Electron and energy transfer mechanisms to switch the luminescence of semiconductor quantum dots

2008 ◽  
Vol 18 (46) ◽  
pp. 5577 ◽  
Author(s):  
Ibrahim Yildiz ◽  
Massimiliano Tomasulo ◽  
Françisco M. Raymo
ACS Nano ◽  
2012 ◽  
Vol 6 (6) ◽  
pp. 5330-5347 ◽  
Author(s):  
Michael H. Stewart ◽  
Alan L. Huston ◽  
Amy M. Scott ◽  
Alexander L. Efros ◽  
Joseph S. Melinger ◽  
...  

Nano Letters ◽  
2010 ◽  
Vol 10 (7) ◽  
pp. 2640-2648 ◽  
Author(s):  
Aliaksandra Rakovich ◽  
Alyona Sukhanova ◽  
Nicolas Bouchonville ◽  
Evgeniy Lukashev ◽  
Vladimir Oleinikov ◽  
...  

2011 ◽  
Vol 115 (44) ◽  
pp. 21535-21545 ◽  
Author(s):  
Eduard I. Zenkevich ◽  
Evgenii I. Sagun ◽  
Valery N. Knyukshto ◽  
Alexander S. Stasheuski ◽  
Victor A. Galievsky ◽  
...  

2010 ◽  
Vol 114 (35) ◽  
pp. 14831-14837 ◽  
Author(s):  
Douglas P. Shepherd ◽  
Kevin J. Whitcomb ◽  
Kenneth K. Milligan ◽  
Peter M. Goodwin ◽  
Martin P. Gelfand ◽  
...  

Nanoscale ◽  
2015 ◽  
Vol 7 (17) ◽  
pp. 7603-7614 ◽  
Author(s):  
Anirban Samanta ◽  
Scott A. Walper ◽  
Kimihiro Susumu ◽  
Chris L. Dwyer ◽  
Igor L. Medintz

2009 ◽  
Author(s):  
Aliaksandra Rakovich ◽  
Alyona Sukhanova ◽  
Nicolas Bouchonville ◽  
Michael Molinari ◽  
Michel Troyon ◽  
...  

2018 ◽  
Vol 232 (9-11) ◽  
pp. 1513-1526 ◽  
Author(s):  
Dzmitry Melnikau ◽  
Thomas Hendel ◽  
Pavel A. Linkov ◽  
Pavel S. Samokhvalov ◽  
Igor R. Nabiev ◽  
...  

Abstract An understanding of the mechanisms of energy transfer and conversion on the nanoscale is one of the key requirements for an implementation of highly efficient photonic nanodevices based on hybrid organic/inorganic nanomaterials. In this work we conduct steady-state and time resolved optical studies of the emission properties of an ensembles and single semiconductor quantum dots and attached organic dye molecules. We revealed that the luminescence intensity of a hybrid structure does not follow the blinking behavior of quantum dots. We also demonstrated an efficient single photon generation from single hybrid nanostructures which involves an energy transfer from donor to acceptor as main excitation source.


Sensors ◽  
2020 ◽  
Vol 20 (10) ◽  
pp. 2909 ◽  
Author(s):  
Anirban Samanta ◽  
Igor L. Medintz

Bioluminescence resonance energy transfer (BRET) is the non-radiative transfer of energy from a bioluminescent protein donor to a fluorophore acceptor. It shares all the formalism of Förster resonance energy transfer (FRET) but differs in one key aspect: that the excited donor here is produced by biochemical means and not by an external illumination. Often the choice of BRET source is the bioluminescent protein Renilla luciferase, which catalyzes the oxidation of a substrate, typically coelenterazine, producing an oxidized product in its electronic excited state that, in turn, couples with a proximal fluorophore resulting in a fluorescence emission from the acceptor. The acceptors pertinent to this discussion are semiconductor quantum dots (QDs), which offer some unrivalled photophysical properties. Amongst other advantages, the QD’s large Stokes shift is particularly advantageous as it allows easy and accurate deconstruction of acceptor signal, which is difficult to attain using organic dyes or fluorescent proteins. QD-BRET systems are gaining popularity in non-invasive bioimaging and as probes for biosensing as they don’t require external optical illumination, which dramatically improves the signal-to-noise ratio by avoiding background auto-fluorescence. Despite the additional advantages such systems offer, there are challenges lying ahead that need to be addressed before they are utilized for translational types of research.


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