How much can the vertical distribution of black carbon affect its global direct radiative forcing?

2010 ◽  
Vol 37 (20) ◽  
pp. n/a-n/a ◽  
Author(s):  
Colin M. Zarzycki ◽  
Tami C. Bond
Keyword(s):  
Vertical Distribution ◽  
Black Carbon ◽  
Radiative Forcing ◽  
Direct Radiative Forcing ◽  
The Vertical Distribution

scholarly journals Impacts of East Asian Summer and Winter Monsoon on Interannual Variations of Mass Concentrations and Direct Radiative Forcing of Black Carbon over Eastern China

2016 ◽  
Author(s):  
Yu Hao Mao ◽  
Hong Liao
Keyword(s):  
Black Carbon ◽  
Radiative Forcing ◽  
Southern China ◽  
East Asian ◽  
Eastern China ◽  
Northern China ◽  
Winter Monsoon ◽  
Interannual Variations ◽  
Direct Radiative Forcing ◽  
Asian Summer

Abstract. We applied a global three-dimensional chemical transport model (GEOS-Chem) to examine the impacts of the East Asian monsoon on the interannual variations of mass concentrations and direct radiative forcing (DRF) of black carbon (BC) over eastern China (110–125° E, 20–45° N). With emissions fixed at the year 2010 levels, model simulations were driven by the Goddard Earth Observing System (GEOS-4) meteorological fields for 1986–2006 and the Modern Era Retrospective-analysis for Research and Applications (MERRA) meteorological fields for 1980–2010. During the period of 1986–2006, simulated JJA and DJF surface BC concentrations were higher in MERRA than in GEOS-4 by 0.30 µg m−3 (44 %) and 0.77 µg m−3 (54 %), respectively, because of the generally weaker precipitation in MERRA. We found that the strength of the East Asian summer monsoon (EASM, (East Asian winter monsoon, EAWM)) negatively correlated with simulated JJA (DJF) surface BC concentrations (r = –0.7 (–0.7) in GEOS-4 and –0.4 (–0.7) in MERRA), mainly by the changes in atmospheric circulation. Relative to the five strongest EASM years, simulated JJA surface BC concentrations in the five weakest monsoon years were higher over northern China (110–125° E, 28–45° N) by 0.04–0.09 µg m−3 (3–11 %), but lower over southern China (110–125° E, 20–27° N) by 0.03–0.04 µg m−3 (10–11 %). Compared to the five strongest EAWM years, simulated DJF surface BC concentrations in the five weakest monsoon years were higher by 0.13–0.15 µg m−3 (5–8 %) in northern China and by 0.04–0.10 µg m−3 (3–12 %) in southern China. The resulting JJA (DJF) mean all-sky DRF of BC at the top of the atmosphere were 0.04 W m−2 (3 %, (0.03 W m−2, 2 %)) higher in northern China but 0.06 W m−2 (14 %, (0.03 W m−2, 3 %)) lower in southern China. In the weakest monsoon years, the weaker vertical convection led to the lower BC concentrations above 1–2 km in southern China, and therefore the lower BC DRF in the region. The differences in vertical profiles of BC between the weakest and strongest EASM years (1998–1997) and EAWM years (1990–1996) reached up to –0.09 µg m−3 (–46 %) and –0.08 µg m−3 (–11 %) at 1–2 km in eastern China.

scholarly journals Markedly enhanced absorption and direct radiative forcing of black carbon under polluted urban environments

2016 ◽  
Vol 113 (16) ◽  
pp. 4266-4271 ◽  
Author(s):  
Jianfei Peng ◽  
Min Hu ◽  
Song Guo ◽  
Zhuofei Du ◽  
Jing Zheng ◽  
...  
Keyword(s):  
Developing Countries ◽  
Black Carbon ◽  
Radiative Forcing ◽  
Urban Environments ◽  
Absorption Enhancement ◽  
Ambient Conditions ◽  
Climatic Impact ◽  
Atmospheric Aging ◽  
Enhanced Absorption ◽  
Direct Radiative Forcing

Black carbon (BC) exerts profound impacts on air quality and climate because of its high absorption cross-section over a broad range of electromagnetic spectra, but the current results on absorption enhancement of BC particles during atmospheric aging remain conflicting. Here, we quantified the aging and variation in the optical properties of BC particles under ambient conditions in Beijing, China, and Houston, United States, using a novel environmental chamber approach. BC aging exhibits two distinct stages, i.e., initial transformation from a fractal to spherical morphology with little absorption variation and subsequent growth of fully compact particles with a large absorption enhancement. The timescales to achieve complete morphology modification and an absorption amplification factor of 2.4 for BC particles are estimated to be 2.3 h and 4.6 h, respectively, in Beijing, compared with 9 h and 18 h, respectively, in Houston. Our findings indicate that BC under polluted urban environments could play an essential role in pollution development and contribute importantly to large positive radiative forcing. The variation in direct radiative forcing is dependent on the rate and timescale of BC aging, with a clear distinction between urban cities in developed and developing countries, i.e., a higher climatic impact in more polluted environments. We suggest that mediation in BC emissions achieves a cobenefit in simultaneously controlling air pollution and protecting climate, especially for developing countries.

Distribution and direct radiative forcing of black carbon aerosols over Korean Peninsula

2012 ◽  
Vol 58 ◽  
pp. 45-55 ◽  
Author(s):  
Min Young Kim ◽  
Seung-Bok Lee ◽  
Gwi-Nam Bae ◽  
Seung Shik Park ◽  
Kyung Man Han ◽  
...  
Keyword(s):  
Black Carbon ◽  
Korean Peninsula ◽  
Radiative Forcing ◽  
Direct Radiative Forcing ◽  
Carbon Aerosols ◽  
Black Carbon Aerosols

scholarly journals Impacts of East Asian summer and winter monsoons on interannual variations of mass concentrations and direct radiative forcing of black carbon over eastern China

2017 ◽  
Vol 17 (7) ◽  
pp. 4799-4816 ◽  
Author(s):  
Yu-Hao Mao ◽  
Hong Liao ◽  
Hai-Shan Chen
Keyword(s):  
Black Carbon ◽  
Radiative Forcing ◽  
Southern China ◽  
East Asian ◽  
Eastern China ◽  
Northern China ◽  
Interannual Variations ◽  
Direct Radiative Forcing ◽  
Asian Summer ◽  
Mass Concentrations

Abstract. We applied a global three-dimensional chemical transport model (GEOS-Chem) to examine the impacts of the East Asian monsoon on the interannual variations of mass concentrations and direct radiative forcing (DRF) of black carbon (BC) over eastern China (110–125° E, 20–45° N). With emissions fixed at the year 2010 levels, model simulations were driven by the Goddard Earth Observing System (GEOS-4) meteorological fields for 1986–2006 and the Modern Era Retrospective-analysis for Research and Applications (MERRA) meteorological fields for 1980–2010. During the period of 1986–2006, simulated June–July–August (JJA) and December–January–February (DJF) surface BC concentrations were higher in MERRA than in GEOS-4 by 0.30 µg m−3 (44 %) and 0.77 µg m−3 (54 %), respectively, because of the generally weaker precipitation in MERRA. We found that the strength of the East Asian summer monsoon (EASM; East Asian winter monsoon, EAWM) negatively correlated with simulated JJA (DJF) surface BC concentrations (r = −0. 7 (−0.7) in GEOS-4 and −0.4 (−0.7) in MERRA), mainly by the changes in atmospheric circulation. Relative to the 5 strongest EASM years, simulated JJA surface BC concentrations in the 5 weakest monsoon years were higher over northern China (110–125° E, 28–45° N) by 0.04–0.09 µg m−3 (3–11 %), but lower over southern China (110–125° E, 20–27° N) by 0.03–0.04 µg m−3 (10–11 %). Compared to the 5 strongest EAWM years, simulated DJF surface BC concentrations in the 5 weakest monsoon years were higher by 0.13–0.15 µg m−3 (5–8 %) in northern China and by 0.04–0.10 µg m−3 (3–12 %) in southern China. The resulting JJA (DJF) mean all-sky DRF of BC at the top of the atmosphere was 0.04 W m−2 (3 %; 0.03 W m−2, 2 %) higher in northern China but 0.06 W m−2 (14 %; 0.03 W m−2, 3 %) lower in southern China. In the weakest monsoon years, the weaker vertical convection at the elevated altitudes led to the lower BC concentrations above 1–2 km in southern China, and therefore the lower BC DRF in the region. The differences in vertical profiles of BC between the weakest and strongest EASM years (1998–1997) and EAWM years (1990–1996) reached up to −0.09 µg m−3 (−46 %) and −0.08 µg m−3 (−11 %) at 1–2 km in eastern China.

scholarly journals The vertical distribution of ozone instantaneous radiative forcing from satellite and chemistry climate models

2011 ◽  
Vol 116 (D1) ◽  
Author(s):  
A. M. Aghedo ◽  
K. W. Bowman ◽  
H. M. Worden ◽  
S. S. Kulawik ◽  
D. T. Shindell ◽  
...  
Keyword(s):  
Vertical Distribution ◽  
Radiative Forcing ◽  
Climate Models ◽  
The Vertical Distribution

scholarly journals The Observation Path Problems and the Formation Conditions of the Elevated Layer of Black Carbon Aerosol

2020 ◽  
Author(s):  
Lianji Jin ◽  
Liang Lin ◽  
Deping Ding ◽  
Delong Zhao ◽  
Bin Zhu ◽  
...  
Keyword(s):  
Vertical Distribution ◽  
Black Carbon ◽  
Simulation Analysis ◽  
Mixing Layer ◽  
Horizontal Distribution ◽  
Free Atmosphere ◽  
Observation Area ◽  
Formation Conditions ◽  
Black Carbon Aerosol ◽  
The Vertical Distribution

Studies on the detection of layers with elevated black carbon aerosol (BC) concentrations and the formation conditions of these layers help understand the vertical distribution of BC concentrations, which will provide a basis for the assessment of climate effects and early BC pollution warnings. By using the Weather Research and Forecasting with Chemistry (WRF-Chem) numerical model, we performed a numerical simulation analysis on the authenticity of strong elevated BC concentration layers that were detected by an aircraft in the mixing layer over Harbin, China, which is a high-emission area, on a clear sunny afternoon in the early heating period of 2016. We then discuss possible problems and solutions when non-vertical paths are used to detect the vertical distribution of BC concentrations. Finally, we discuss the favorable conditions for the formation of elevated BC concentration layers by weak vertical flow. The results show that the horizontal variability of BC concentration in the mixing layer in the observation area in Harbin was sufficiently large during the measurement. This produced a false elevated layer, as detected by the aircraft during one round of spiral flight in the mixing layer. The root mean square of the horizontal distribution of BC concentration did not change with height in the mixing layer during the daytime, but it decreased with the thickness of the mixing layer and was higher in the mixing layer than in the free atmosphere. Therefore, the thinner the mixing layer, in which the vertical distribution of the BC concentration is detected in an inclined path, the stronger interference of the horizontal variability on the detected results. When a spiral flight detection path is used, the aircraft should fly at least two rounds in the mixing layer. In the daytime, due to strong turbulence in the mixing layer, weak vertical uplift is not favorable for the occurrence of elevated BC concentration layers in the mixing layer. In the nighttime, if weak vertical uplift is well matched with the BC concentration or its vertical gradient, elevated BC concentration layers can be formed in the atmosphere. Compared with upper layers far from the ground, nighttime elevated layers are easier to form in lower layers near the ground because high BC concentrations or large vertical gradients are more likely to occur in the lower layers. Both cases facilitate the occurrence of large vertical upward transport rates of BC.

scholarly journals Processes controlling the vertical aerosol distribution in marine stratocumulus regions – a sensitivity study using the climate model NorESM1-M

2021 ◽  
Vol 21 (1) ◽  
pp. 577-595
Author(s):  
Lena Frey ◽  
Frida A.-M. Bender ◽  
Gunilla Svensson
Keyword(s):  
Vertical Distribution ◽  
Radiative Forcing ◽  
Climate Model ◽  
Cloud Microphysics ◽  
Aerosol Extinction ◽  
Shallow Convection ◽  
Marine Stratocumulus ◽  
Aerosol Emission ◽  
Aerosol Distribution ◽  
The Vertical Distribution

Abstract. The vertical distribution of aerosols plays an important role in determining the effective radiative forcing from aerosol–radiation and aerosol–cloud interactions. Here, a number of processes controlling the vertical distribution of aerosol in five subtropical marine stratocumulus regions in the climate model NorESM1-M are investigated, with a focus on the total aerosol extinction. A comparison with satellite lidar data (CALIOP, Cloud–Aerosol Lidar with Orthogonal Polarization) shows that the model underestimates aerosol extinction throughout the troposphere, especially elevated aerosol layers in the two regions where they are seen in observations. It is found that the shape of the vertical aerosol distribution is largely determined by the aerosol emission and removal processes in the model, primarily through the injection height, emitted particle size, and wet scavenging. In addition, the representation of vertical transport related to shallow convection and entrainment is found to be important, whereas alterations in aerosol optical properties and cloud microphysics parameterizations have smaller effects on the vertical aerosol extinction distribution. However, none of the alterations made are sufficient for reproducing the observed vertical distribution of aerosol extinction, neither in magnitude nor in shape. Interpolating the vertical levels of CALIOP to the corresponding model levels leads to better agreement in the boundary layer and highlights the importance of the vertical resolution.

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