scholarly journals Aerosol optical depth measurements in eastern China and a new calibration method

2010 ◽  
Vol 115 ◽  
Author(s):  
Kwon H. Lee ◽  
Zhanqing Li ◽  
M. C. Cribb ◽  
Jianjun Liu ◽  
Lei Wang ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Eastern China ◽  
Calibration Method

scholarly journals Evaluating Carbon Monoxide and Aerosol Optical Depth Simulations from CAM-Chem Using Satellite Observations

2021 ◽  
Vol 13 (11) ◽  
pp. 2231
Author(s):  
Débora Souza Alvim ◽  
Júlio Barboza Chiquetto ◽  
Monica Tais Siqueira D’Amelio ◽  
Bushra Khalid ◽  
Dirceu Luis Herdies ◽  
...  
Keyword(s):  
Carbon Monoxide ◽  
South America ◽  
Aerosol Optical Depth ◽  
Tropical Forests ◽  
Optical Depth ◽  
Eastern China ◽  
Central Africa ◽  
Central China ◽  
Stratospheric Chemistry ◽  
Tropical Areas

The scope of this work was to evaluate simulated carbon monoxide (CO) and aerosol optical depth (AOD) from the CAM-chem model against observed satellite data and additionally explore the empirical relationship of CO, AOD and fire radiative power (FRP). The simulated seasonal global concentrations of CO and AOD were compared, respectively, with the Measurements of Pollution in the Troposphere (MOPITT) and the Moderate-Resolution Imaging Spectroradiometer (MODIS) satellite products for the period 2010–2014. The CAM-chem simulations were performed with two configurations: (A) tropospheric-only; and (B) tropospheric with stratospheric chemistry. Our results show that the spatial and seasonal distributions of CO and AOD were reasonably reproduced in both model configurations, except over central China, central Africa and equatorial regions of the Atlantic and Western Pacific, where CO was overestimated by 10–50 ppb. In configuration B, the positive CO bias was significantly reduced due to the inclusion of dry deposition, which was not present in the model configuration A. There was greater CO loss due to the chemical reactions, and shorter lifetime of the species with stratospheric chemistry. In summary, the model has difficulty in capturing the exact location of the maxima of the seasonal AOD distributions in both configurations. The AOD was overestimated by 0.1 to 0.25 over desert regions of Africa, the Middle East and Asia in both configurations, but the positive bias was even higher in the version with added stratospheric chemistry. By contrast, the AOD was underestimated over regions associated with anthropogenic activity, such as eastern China and northern India. Concerning the correlations between CO, AOD and FRP, high CO is found during March–April–May (MAM) in the Northern Hemisphere, mainly in China. In the Southern Hemisphere, high CO, AOD, and FRP values were found during August–September–October (ASO) due to fires, mostly in South America and South Africa. In South America, high AOD levels were observed over subtropical Brazil, Paraguay and Bolivia. Sparsely urbanized regions showed higher correlations between CO and FRP (0.7–0.9), particularly in tropical areas, such as the western Amazon region. There was a high correlation between CO and aerosols from biomass burning at the transition between the forest and savanna environments over eastern and central Africa. It was also possible to observe the transport of these pollutants from the African continent to the Brazilian coast. High correlations between CO and AOD were found over southeastern Asian countries, and correlations between FRP and AOD (0.5–0.8) were found over higher latitude regions such as Canada and Siberia as well as in tropical areas. Higher correlations between CO and FRP are observed in Savanna and Tropical forests (South America, Central America, Africa, Australia, and Southeast Asia) than FRP x AOD. In contrast, boreal forests in Russia, particularly in Siberia, show a higher FRP x AOD correlation than FRP x CO. In tropical forests, CO production is likely favored over aerosol, while in temperate forests, aerosol production is more than CO compared to tropical forests. On the east coast of the United States, the eastern border of the USA with Canada, eastern China, on the border between China, Russia, and Mongolia, and the border between North India and China, there is a high correlation of CO x AOD and a low correlation between FRP with both CO and AOD. Therefore, such emissions in these regions are not generated by forest fires but by industries and vehicular emissions since these are densely populated regions.

scholarly journals Estimating ground-level PM<sub>2.5</sub> in Eastern China using aerosol optical depth determined from the GOCI Satellite Instrument

2015 ◽  
Vol 15 (12) ◽  
pp. 17251-17281 ◽  
Author(s):  
J. Xu ◽  
R. V. Martin ◽  
A. van Donkelaar ◽  
J. Kim ◽  
M. Choi ◽  
...  
Keyword(s):  
Organic Matter ◽  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Transport Model ◽  
Eastern China ◽  
Ground Level ◽  
East China ◽  
Chemical Transport Model ◽  
Near Surface ◽  
Significant Agreement

Abstract. We determine and interpret fine particulate matter (PM2.5) concentrations in East China for January to December 2013 at a horizontal resolution of 6 km from aerosol optical depth (AOD) retrieved from the Korean Geostationary Ocean Color Imager (GOCI) satellite instrument. We implement a set of filters to minimize cloud contamination in GOCI AOD. Evaluation of filtered GOCI AOD with AOD from the Aerosol Robotic Network (AERONET) indicates significant agreement with mean fractional bias (MFB) in Beijing of 6.7 % and northern Taiwan of −1.2 %. We use a global chemical transport model (GEOS-Chem) to relate the total column AOD to the near-surface PM2.5. The simulated PM2.5/AOD ratio exhibits high consistency with ground-based measurements (MFB = −0.52–8.0 %). We evaluate the satellite-derived PM2.5 vs. the ground-level PM2.5 in 2013 measured by the China Environmental Monitoring Center. Significant agreement is found between GOCI-derived PM2.5 and in-situ observations in both annual averages (r = 0.81, N = 494) and monthly averages (MFB = 13.1 %), indicating GOCI provides valuable data for air quality studies in Northeast Asia. The GEOS-Chem simulated chemical speciation of GOCI-derived PM2.5 reveals that secondary inorganics (SO42−, NO3−, NH4+) and organic matter are the most significant components. Biofuel emissions in northern China for heating are responsible for an increase in the concentration of organic matter in winter. The population-weighted GOCI-derived PM2.5 over East China for 2013 is 53.8 μg m−3, threatening the health and life expectancy of its 600 million residents.

scholarly journals The spatiotemporal relationship between PM<sub>2.5</sub> and aerosol optical depth in China: influencing factors and implications for satellite PM<sub>2.5</sub> estimations using MAIAC aerosol optical depth

2021 ◽  
Vol 21 (24) ◽  
pp. 18375-18391
Author(s):  
Qingqing He ◽  
Mengya Wang ◽  
Steve Hung Lam Yim
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Spatial Scales ◽  
Pearson Correlation ◽  
Eastern China ◽  
Atmospheric Correction ◽  
Mainland China ◽  
Ground Level ◽  
Central China ◽  
The Relationship

Abstract. Satellite aerosol retrievals have been a popular alternative to monitoring the surface-based PM2.5 concentration due to their extensive spatial and temporal coverage. Satellite-derived PM2.5 estimations strongly rely on an accurate representation of the relationship between ground-level PM2.5 and satellite aerosol optical depth (AOD). Due to the limitations of satellite AOD data, most studies have examined the relationship at a coarse resolution (i.e., ≥ 10 km); thus, more effort is still needed to better understand the relationship between “in situ” PM2.5 and AOD at finer spatial scales. While PM2.5 and AOD could have obvious temporal variations, few studies have examined the diurnal variation in their relationship. Therefore, considerable uncertainty still exists in satellite-derived PM2.5 estimations due to these research gaps. Taking advantage of the newly released fine-spatial-resolution satellite AOD data derived from the Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm and real-time ground aerosol and PM2.5 measurements, this study explicitly explored the relationship between PM2.5 and AOD as well as its plausible impact factors, including meteorological parameters and topography, in mainland China during 2019, at various spatial and temporal scales. The coefficient of variation, the Pearson correlation coefficient and the slope of the linear regression model were used. Spatially, stronger correlations mainly occurred in northern and eastern China, and the linear slope was larger on average in northern inland regions than in other areas. Temporally, the PM2.5–AOD correlation peaked at noon and in the afternoon, and reached a maximum in winter. Simultaneously, considering relative humidity (RH) and the planetary boundary layer height (PBLH) in the relationship can improve the correlation, but the effect of RH and the PBLH on the correlation varied spatially and temporally with respect to both strength and direction. In addition, the largest correlation occurred at 400–600 m primarily in basin terrain such as the Sichuan Basin, the Shanxi–Shaanxi basins and the Junggar Basin. MAIAC 1 km AOD can better represent the ground-level fine particulate matter in most domains with exceptions, such as in very high terrain (i.e., Tibetan Plateau) and northern central China (i.e., Qinghai and Gansu). The findings of this study have useful implications for satellite-based PM2.5 monitoring and will further inform the understanding of the aerosol variation and PM2.5 pollution status of mainland China.

scholarly journals Retrieving High-Resolution Aerosol Optical Depth from GF-4 PMS Imagery in Eastern China

2021 ◽  
Vol 13 (18) ◽  
pp. 3752
Author(s):  
Zhendong Sun ◽  
Jing Wei ◽  
Ning Zhang ◽  
Yulong He ◽  
Yu Sun ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Zenith Angle ◽  
Rural Areas ◽  
Urban Areas ◽  
Eastern China ◽  
Practical Significance ◽  
Retrieval Algorithm ◽  
Transfer Model ◽  
Surface Reflectance

Gaofen 4 (GF-4) is a geostationary satellite, with a panchromatic and multispectral sensor (PMS) onboard, and has great potential in observing atmospheric aerosols. In this study, we developed an aerosol optical depth (AOD) retrieval algorithm for the GF-4 satellite. AOD retrieval was realized based on the pre-calculated surface reflectance database and 6S radiative transfer model. We customized the unique aerosol type according to the long time series aerosol parameters provided by the Aerosol Robotic Network (AERONET) site. The solar zenith angle, relative azimuth angle, and satellite zenith angle of the GF-4 panchromatic multispectral sensor image were calculated pixel-by-pixel. Our 1 km AOD retrievals were validated against AERONET Version 3 measurements and compared with MOD04 C6 AOD products at different resolutions. The results showed that our GF-4 AOD algorithm had a good robustness in both bright urban areas and dark rural areas. A total of 71.33% of the AOD retrievals fell within the expected errors of ±(0.05% + 20%); root-mean-square error (RMSE) and mean absolute error (MAE) were 0.922 and 0.122, respectively. The accuracy of GF-4 AOD in rural areas was slightly higher than that in urban areas. In comparison with MOD04 products, the accuracy of GF-4 AOD was much higher than that of MOD04 3 km and 10 km dark target AOD, but slightly worse than that of MOD04 10 km deep blue AOD. For different values of land surface reflectance (LSR), the accuracy of GF-4 AOD gradually deteriorated with an increase in the LSR. These results have theoretical and practical significance for aerosol research and can improve retrieval algorithms using the GF-4 satellite.

scholarly journals Aerosol radiative forcings induced by substantial changes in anthropogenic emissions in China from 2008 to 2016

2021 ◽  
Vol 21 (8) ◽  
pp. 5965-5982
Author(s):  
Mingxu Liu ◽  
Hitoshi Matsui
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Forcing ◽  
Eastern China ◽  
Radiation Budget ◽  
Anthropogenic Emissions ◽  
Radiative Forcings ◽  
The Past ◽  
Positive Direct ◽  
Aerosol Radiative

Abstract. Anthropogenic emissions in China play an important role in altering the global radiation budget. Over the past decade, the strong clean-air policies in China have resulted in substantial reductions of anthropogenic emissions of sulfur dioxide (SO2) and primary particulate matter, and air quality in China has consequently improved. However, the resultant aerosol radiative forcings have been poorly understood. In this study, we used an advanced global climate model integrated with the latest localized emission inventory to quantify the aerosol radiative forcings by the changes of anthropogenic emissions in China between 2008 and 2016. By comparing with multiple observation datasets, our simulations reproduced the considerable reductions of sulfate and black carbon (BC) mass loadings reasonably well over eastern China (the key region subject to stringent emission controls) during the period and accordingly showed a clear decline in both aerosol optical depth and absorption aerosol optical depth. The results revealed a regional annual mean positive direct radiative forcing (DRF) of +0.29 W m−2 at the top of the atmosphere (TOA) due to the reduction of SO2 emissions. This positive aerosol radiative forcing was comprised of diminished sulfate scattering (+0.58 W m−2), enhanced nitrate radiative effects (−0.29 W m−2), and could be completely offset by the concurrent reduction of BC emissions that induced a negative BC DRF of −0.33 W m−2. Despite the small net aerosol DRF (−0.05 W m−2) at the TOA, aerosol–radiation interactions could explain the surface brightening in China over the past decade. The overall reductions in aerosol burdens and associated optical effects mainly from BC and sulfate enhanced the regional annual mean downward solar radiation flux at the surface by +1.0 W m−2 between 2008 and 2016. The enhancement was in general agreement with a long-term observational record of surface energy fluxes in China. We also estimated that aerosol effects on cloud radiative forcings may have played a dominant role in the net aerosol radiative forcings at the TOA in China and over the northern Pacific Ocean during the study period. This study will facilitate more informed assessment of climate responses to projected emissions in the future as well as to sudden changes in human activities (e.g., the COVID-19 lockdown).

scholarly journals Large contribution of meteorological factors to inter-decadal changes in regional aerosol optical depth

2019 ◽  
Author(s):  
Huizheng Che ◽  
Ke Gui ◽  
Xiangao Xia ◽  
Yaqiang Wang ◽  
Brent N. Holben ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Meteorological Parameters ◽  
Eastern China ◽  
Meteorological Parameter ◽  
Emission Factors ◽  
Dominant Factor ◽  
Large Contribution ◽  
Anthropogenic Aerosol

Abstract. Aerosol optical depth (AOD) has become a crucial metric for assessing global climate change. Although global and regional AOD trends have been studied extensively, it remains unclear what factors are driving the inter-decadal variations in regional AOD and how to quantify the relative contribution of each dominant factor. This study used a long-term (1980–2016) aerosol dataset from the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis, along with two satellite-based AOD datasets (MODIS/Terra and MISR) from 2001 to 2016, to investigate the long-term trends in global and regional aerosol loading. Statistical models based on emission factors and meteorological parameters were developed to identify the main factors driving the inter-decadal changes of regional AOD and to quantify their contribution. Evaluation of the MERRA-2 AOD with the combined in-situ measurements of AERONET and the China Aerosol Remote Sensing Network indicated significant spatial agreement on the global scale (r = 0.84, RMSE = 0.14, and MAE = 0.07). In general, MERRA-2 was able to quantitatively reproduce the annual and seasonal AOD trends on both regional and global scales, as observed by MODIS/Terra, albeit some differences were found when compared to MISR. Over the 37-year period in this study, significant decreasing trends were observed over Europe and the eastern United States. In contrast, eastern China and South Asia showed AOD increases, but the increasing trend of the former reversed sharply in the most recent decade. The statistical analyses suggested that the meteorological parameters explained a larger proportion of the AOD variability (20.4 %–72.8 %) over almost all regions of interest (ROIs) during 1980–2014 when compared with emission factors (0 %–56 %). Further analysis also showed that SO2 was the dominant emission factor, explaining 12.7 %–32.6 % of the variation in AOD over anthropogenic aerosol–dominant regions, while BC or OC was the leading factor over the biomass burning–dominant (BBD) regions, contributing 24.0 %–27.7 % of the variation. Additionally, wind speed was found to be the leading meteorological parameter, explaining 11.8 %–30.3 % of the variance over the mineral dust–dominant regions, while ambient humidity (including soil moisture and relative humidity) was the top meteorological parameter over the BBD regions, accounting for 11.7 %–35.5 % of the variation. The results of this study indicate that the variation in meteorological parameters is a key factor in determining the inter-decadal change in regional AOD.

scholarly journals Large contribution of meteorological factors to inter-decadal changes in regional aerosol optical depth

2019 ◽  
Vol 19 (16) ◽  
pp. 10497-10523 ◽  
Author(s):  
Huizheng Che ◽  
Ke Gui ◽  
Xiangao Xia ◽  
Yaqiang Wang ◽  
Brent N. Holben ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Meteorological Parameters ◽  
Eastern China ◽  
Meteorological Parameter ◽  
Emission Factors ◽  
Dominant Factor ◽  
Large Contribution ◽  
Gross Error

Abstract. Aerosol optical depth (AOD) has become a crucial metric for assessing global climate change. Although global and regional AOD trends have been studied extensively, it remains unclear what factors are driving the inter-decadal variations in regional AOD and how to quantify the relative contribution of each dominant factor. This study used a long-term (1980–2016) aerosol dataset from the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis, along with two satellite-based AOD datasets (MODIS/Terra and MISR) from 2001 to 2016, to investigate the long-term trends in global and regional aerosol loading. Statistical models based on emission factors and meteorological parameters were developed to identify the main factors driving the inter-decadal changes of regional AOD and to quantify their contribution. Evaluation of the MERRA-2 AOD with the ground-based measurements of AERONET indicated significant spatial agreement on the global scale (r= 0.85, root-mean-square error = 0.12, mean fractional error = 38.7 %, fractional gross error = 9.86 % and index of agreement = 0.94). However, when AOD observations from the China Aerosol Remote Sensing Network (CARSNET) were employed for independent verification, the results showed that MERRA-2 AODs generally underestimated CARSNET AODs in China (relative mean bias = 0.72 and fractional gross error =-34.3 %). In general, MERRA-2 was able to quantitatively reproduce the annual and seasonal AOD trends on both regional and global scales, as observed by MODIS/Terra, although some differences were found when compared to MISR. Over the 37-year period in this study, significant decreasing trends were observed over Europe and the eastern United States. In contrast, eastern China and southern Asia showed AOD increases, but the increasing trend of the former reversed sharply in the most recent decade. The statistical analyses suggested that the meteorological parameters explained a larger proportion of the AOD variability (20.4 %–72.8 %) over almost all regions of interest (ROIs) during 1980–2014 when compared with emission factors (0 %–56 %). Further analysis also showed that SO2 was the dominant emission factor, explaining 12.7 %–32.6 % of the variation in AOD over anthropogenic-aerosol-dominant regions, while black carbon or organic carbon was the leading factor over the biomass-burning-dominant (BBD) regions, contributing 24.0 %–27.7 % of the variation. Additionally, wind speed was found to be the leading meteorological parameter, explaining 11.8 %–30.3 % of the variance over the mineral-dust-dominant regions, while ambient humidity (including soil moisture and relative humidity) was the top meteorological parameter over the BBD regions, accounting for 11.7 %–35.5 % of the variation. The results of this study indicate that the variation in meteorological parameters is a key factor in determining the inter-decadal change in regional AOD.

Correlation between PM concentrations and aerosol optical depth in eastern China

2009 ◽  
Vol 43 (37) ◽  
pp. 5876-5886 ◽  
Author(s):  
Jian-Ping Guo ◽  
Xiao-Ye Zhang ◽  
Hui-Zheng Che ◽  
Sun-Ling Gong ◽  
Xingqin An ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Eastern China
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