scholarly journals Processes influencing ozone levels in Alaskan forest fire plumes during long-range transport over the North Atlantic

2007 ◽  
Vol 112 (D10) ◽  
Author(s):  
E. Real ◽  
K. S. Law ◽  
B. Weinzierl ◽  
M. Fiebig ◽  
A. Petzold ◽  
...  
Keyword(s):  
Long Range ◽  
Forest Fire ◽  
North Atlantic ◽  
Long Range Transport ◽  
The North ◽  
Fire Plumes ◽  
Range Transport ◽  
The North Atlantic ◽  
Ozone Levels

scholarly journals Lagrangian formation pathways of moist anomalies in the trade-wind region during the dry season: two case studies from EUREC<sup>4</sup>A

2021 ◽  
Author(s):  
Leonie Villiger ◽  
Heini Wernli ◽  
Maxi Boettcher ◽  
Martin Hagen ◽  
Franziska Aemisegger
Keyword(s):  
Long Range ◽  
North Atlantic ◽  
Large Scale ◽  
Cold Front ◽  
Trade Wind ◽  
Long Range Transport ◽  
The North ◽  
Range Transport ◽  
The North Atlantic ◽  
The Tropics

Abstract. Shallow clouds in the trade-wind region over the North Atlantic contribute substantially to the global radiative budget. In the vicinity of the Caribbean island Barbados, they appear in different mesoscale organisation patterns with distinct net cloud radiative effects (CRE). Cloud formation processes in this region are typically controlled by the prevailing large-scale subsidence. However, occasionally weather systems from remote origin cause significant disturbances. This study investigates the complex cloud-circulation interactions during the field campaign EUREC4A (Elucidate the Couplings Between Clouds, Convection and Circulation) from 16 January to 20 February 2020, using a combination of Eulerian and Lagrangian diagnostics. Based on observations and ERA5 reanalyses, we identify the relevant processes and characterise the formation pathways of two moist anomalies above the Barbados Cloud Observatory (BCO), one in the lower (~1000–650 hPa) and one in the middle troposphere (~650–300 hPa). These moist anomalies are associated with strongly negative CRE values and with contrasting long-range transport processes from the extratropics and the tropics, respectively. The low-level moist anomaly is characterised by an unusually thick cloud layer, high precipitation totals and a strongly negative CRE. Its formation is connected to an “extratropical dry intrusion” (EDI) that interacts with a trailing cold front. A quasi-climatological (2010–2020) analysis reveals that EDIs lead to different conditions at the BCO depending on how they interact with the associated cold front. Based on this climatology, we discuss the relevance of the strong large-scale forcing by EDIs for the low-cloud patterns near the BCO and the related CRE. The second case study about the mid-tropospheric moist anomaly is associated with an extended and persistent mixed-phase shelf cloud and the lowest daily CRE value observed during the campaign. Its formation is linked to “tropical mid-level detrainment” (TMD), which refers to detrainment from tropical deep convection near the melting layer. The quasi-climatological analysis shows that TMDs consistently lead to mid-tropospheric moist anomalies over the BCO and that the detrainment height controls the magnitude of the anomaly. However, no systematic relationship was found between the amplitude of this mid-tropospheric moist anomaly and the CRE at the BCO. Overall, this study reveals the important impact of the long-range transport, driven by dynamical processes either in the extratropics or the tropics, on the variability of the vertical structure of moisture and clouds, and on the resulting CRE in the North Atlantic winter trades.

scholarly journals Long-range transport of ozone and related pollutants over the North Atlantic in spring and summer

2004 ◽  
Vol 4 (4) ◽  
pp. 4407-4454 ◽  
Author(s):  
S. A. Penkett ◽  
M. J. Evans ◽  
C. E. Reeves ◽  
K. S. Law ◽  
P. S. Monks ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Long Range ◽  
North Atlantic ◽  
Marine Boundary Layer ◽  
Long Range Transport ◽  
Ozone Concentrations ◽  
The North ◽  
Range Transport ◽  
The North Atlantic ◽  
The Uk

Abstract. This paper presents strong experimental evidence for a major perturbation in ozone concentrations over large parts of the North Atlantic Ocean from the surface to 8 km associated with continental pollutants. The evidence was gathered in the course of 7 flights by the UK Meteorological Office C-130 aircraft based on the Azores, and 4 ferry flights between the UK to the Azores in spring and summer 1997 as a component of the NERC-funded ACSOE project. The total latitude range covered was approximately 55°N–25°N, and the longitude range was approximately 0° to 40°W. Many profiles were made between the sea surface and altitudes up to 9 km to survey the composition of the marine atmosphere. The C-130 aircraft was comprehensively equipped to measure many chemical and physical parameters along with standard meteorological instrumentation. Thus it was able to measure ozone and speciated NOy, along with tracers including water vapour, carbon monoxide and condensation nuclei, in near real time. The overall "picture" of the troposphere over large parts of the North Atlantic is of layers of pollution from the continents of different ages interspersed with layers of air uplifted from the marine boundary layer. The lowest ozone concentrations were recorded in the marine boundary layer where there is evidence for extensive ozone destruction in summer. Flights were made to penetrate the outflow of hurricane Erica, to determine the southerly extent of polluted air in summer, to examine the impact of frontal systems on the composition of remote marine air, and to trace long-range pollution from the west coast of the USA interspersed with air with a stratospheric origin. In one of the spring flights it is possible that a plume of polluted air with high ozone and NOy, and with an origin in southeast Asia, was intercepted off the coast of Portugal. The concentrations of NOx, in this plume were sufficient for ozone formation to be continuing along its track from west to east. The instrument to measure NOy almost certainly was only measuring the sum of organic nitrates (mostly in the form of PAN) plus NOx. The high correlation between NOy and ozone under these conditions strongly suggests a non-stratospheric source for most of the ozone encountered over large parts of the atmosphere upwind of Europe. There was a marked seasonal variation in the NOy with about twice as much present in the spring flights than in the summer flights. The overall ozone levels in both spring and summer were somewhat similar although the highest ozone concentration encountered (~100 ppbv) was observed in summer in some polluted layers in mid Atlantic with an origin in the boundary layer over the southeastern USA. The bulk of the pollutants, ozone, CO, and NOy, were in the free troposphere at altitudes between 3 and 8 km. The only instances of pollution at lower levels were in the form of ship plumes, which were encountered several times. The data therefore strongly support the need for more in-situ aircraft experiments to quantify and understand the phenomenon of long-range transport of pollution from continent to continent. Observations at ground-based stations are inadequate for this purpose and satellite data is incomplete both in terms of its altitude detail and in the extent of chemical speciation, particularly for ascertaining whether chemical production and destruction processes for ozone are occurring.

GLAS long-range transport observation of the 2003 California forest fire plumes to the northeastern US

2005 ◽  
Vol 32 (22) ◽  
pp. n/a-n/a ◽  
Author(s):  
R. M. Hoff ◽  
S. P. Palm ◽  
J. A. Engel-Cox ◽  
J. Spinhirne
Keyword(s):  
Long Range ◽  
Forest Fire ◽  
Long Range Transport ◽  
Fire Plumes ◽  
Range Transport

scholarly journals Transport and fate of hexachlorocyclohexanes in the oceanic air and surface seawater

2011 ◽  
Vol 8 (3) ◽  
pp. 5537-5562 ◽  
Author(s):  
Z. Xie ◽  
B. P. Koch ◽  
A. Möller ◽  
R. Sturm ◽  
R. Ebinghaus
Keyword(s):  
Southern Ocean ◽  
Long Range ◽  
Water Exchange ◽  
Exchange Process ◽  
Lower Atmosphere ◽  
Long Range Transport ◽  
Surface Seawater ◽  
The North ◽  
Range Transport ◽  
Long Term Trends

Abstract. Hexachlorocyclohexanes (HCHs) are ubiquitous organic pollutants derived from pesticide application. They are subject to long-range transport, persistent in the environment, and capable of accumulation in biota. Shipboard measurements of HCH isomers (α-, γ- and β-HCH) in surface seawater and boundary layer atmospheric samples were conducted in the Atlantic and the Southern Ocean in October to December of 2008. ΣHCHs concentrations (the sum of α-, γ- and β-HCH) in the lower atmosphere ranged from 11.8 to 36.9 pg m−3 (mean: 26.6 ± 11.0 pg m−3) in the Northern Hemisphere (NH), and from 1.5 to 4.0 pg m−3 (mean: 2.8 ± 1.1 pg m−3) in the Southern Hemisphere (SH), respectively. Water concentrations were: α-HCH 0.33–46.8 pg l−1, γ-HCH 0.02–33.2 pg l−1 and β-HCH 0.11–2 pg l−1. HCH concentrations decreased from the North Atlantic to the Southern Ocean, indicating historical use of HCHs in the NH. Spatial distribution showed increasing concentrations from the equator towards North and South latitudes illustrating the concept of cold condensation and less interhemispheric mixing process. In comparison to concentrations measured in 1987–1999/2000, gaseous HCHs were slightly lower, while dissolved HCHs decreased by factor of 2–3 orders of magnitude. Air-water exchange gradients suggested net deposition for α-HCH (mean: 3759 pg m−2 day−1) and γ-HCH (mean: 1987 pg m−2 day−1), whereas β-HCH varied between equilibrium (volatilization: <0–12 pg m−2 day−1) and net deposition (range: 6–687 pg m−2 day−1), indicating a multi-hopper transport behavior. Climate change may significantly accelerate the releasing process of "old" HCHs from continental storage (e.g. soil, vegetation and high mountains) and drive long-range transport from sources to deposition in the open oceans. Biological productivities may interfere with the air-water exchange process as well. Consequently, further investigation is necessary to elucidate the long term trends and the biogeochemical turnover of HCHs in the oceanic environment.

scholarly journals Quantification of chemical and physical processes influencing ozone during long-range transport using a trajectory ensemble

2012 ◽  
Vol 12 (15) ◽  
pp. 7015-7039 ◽  
Author(s):  
M. Cain ◽  
J. Methven ◽  
E. J. Highwood
Keyword(s):  
Long Range ◽  
Long Range Transport ◽  
Mass Composition ◽  
Physical Parameters ◽  
Physical Processes ◽  
Air Mass ◽  
Mixing Ratios ◽  
The North ◽  
Range Transport ◽  
Physical Processing

Abstract. During long-range transport, many distinct processes – including photochemistry, deposition, emissions and mixing – contribute to the transformation of air mass composition. Partitioning the effects of different processes can be useful when considering the sensitivity of chemical transformation to, for example, a changing environment or anthropogenic influence. However, transformation is not observed directly, since mixing ratios are measured, and models must be used to relate changes to processes. Here, four cases from the ITCT-Lagrangian 2004 experiment are studied. In each case, aircraft intercepted a distinct air mass several times during transport over the North Atlantic, providing a unique dataset and quantifying the net changes in composition from all processes. A new framework is presented to deconstruct the change in O3 mixing ratio (Δ O3) into its component processes, which were not measured directly, taking into account the uncertainty in measurements, initial air mass variability and its time evolution. The results show that the net chemical processing (Δ O3chem) over the whole simulation is greater than net physical processing (Δ O3phys) in all cases. This is in part explained by cancellation effects associated with mixing. In contrast, each case is in a regime of either net photochemical destruction (lower tropospheric transport) or production (an upper tropospheric biomass burning case). However, physical processes influence O3 indirectly through addition or removal of precursor gases, so that changes to physical parameters in a model can have a larger effect on Δ O3chem than Δ O3phys. Despite its smaller magnitude, the physical processing distinguishes the lower tropospheric export cases, since the net photochemical O3 change is −5 ppbv per day in all three cases. Processing is quantified using a Lagrangian photochemical model with a novel method for simulating mixing through an ensemble of trajectories and a background profile that evolves with them. The model is able to simulate the magnitude and variability of the observations (of O3, CO, NOy and some hydrocarbons) and is consistent with the time-average OH following air-masses inferred from hydrocarbon measurements alone (by Arnold et al., 2007). Therefore, it is a useful new method to simulate air mass evolution and variability, and its sensitivity to process parameters.

The Evaluation and Use of the Dectra Navigation System

1958 ◽  
Vol 11 (4) ◽  
pp. 377-384
Author(s):  
E. W. Hare
Keyword(s):  
Long Range ◽  
North Atlantic ◽  
Navigation System ◽  
Radio Navigation ◽  
The North ◽  
Radio Navigation System ◽  
Accurate Position ◽  
The North Atlantic

Dectra is a long-range radio navigation system designed to give accurate position fixing coverage over specific areas, and in particular over long trans-oceanic crossings. The position of an aircraft or ship equipped with a Dectra receiver is continuously available in the form of dial indications relating to coordinates of a Dectra lattice, and in addition this information can be presented pictorially on a normal Decca flight log. The system is at present functioning over the North Atlantic, and flight trials have been in progress since May 1957. This paper discusses the experience gained and the results obtained in the trials.

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