scholarly journals Evolution and chemical consequences of lightning-produced NOxobserved in the North Atlantic upper troposphere

2000 ◽  
Vol 105 (D15) ◽  
pp. 19795-19809 ◽  
Author(s):  
J. Crawford ◽  
D. Davis ◽  
J. Olson ◽  
G. Chen ◽  
S. Liu ◽  
...  
2019 ◽  
Vol 19 (10) ◽  
pp. 6621-6636 ◽  
Author(s):  
Thorsten Kaluza ◽  
Daniel Kunkel ◽  
Peter Hoor

Abstract. The evolution of the tropopause inversion layer (TIL) during cyclogenesis in the North Atlantic storm track is investigated using operational meteorological analysis data (Integrated Forecast System from the European Centre for Medium-Range Weather Forecasts). For this a total of 130 cyclones have been analysed during the months August through October between 2010 and 2014 over the North Atlantic. Their paths of migration along with associated flow features in the upper troposphere and lower stratosphere (UTLS) have been tracked based on the mean sea level pressure field. Subsets of the 130 cyclones have been used for composite analysis using minimum sea level pressure to filter the cyclones based on their strength. The composite structure of the TIL strength distribution in connection with the overall UTLS flow strongly resembles the structure of the individual cyclones. Key results are that a strong dipole in TIL strength forms in regions of cyclonic wrap-up of UTLS air masses of different origin and isentropic potential vorticity. These air masses are associated with the cyclonic rotation of the underlying cyclones. The maximum values of enhanced static stability above the tropopause occur north and northeast of the cyclone centre, vertically aligned with outflow regions of strong updraft and cloud formation up to the tropopause, which are situated in anticyclonic flow patterns in the upper troposphere. These regions are co-located with a maximum of vertical shear of the horizontal wind. The strong wind shear within the TIL results in a local minimum of Richardson numbers, representing the possibility for turbulent instability and potential mixing (or air mass exchange) within regions of enhanced static stability in the lowermost stratosphere.


2008 ◽  
Vol 8 (7) ◽  
pp. 1989-2005 ◽  
Author(s):  
S. Y. Kim ◽  
R. Talbot ◽  
H. Mao ◽  
D. Blake ◽  
S. Vay ◽  
...  

Abstract. A case of continental outflow from the United States (US) was examined using airborne measurements from NASA DC-8 flight 13 during the Intercontinental Chemical Transport Experiment – North America (INTEX-NA). Mixing ratios of methane (CH4) and carbon monoxide (CO) at 8–11 km altitude over the North Atlantic were elevated to 1843 ppbv and 134 ppbv respectively, while those of carbon dioxide (CO2) and carbonyl sulfide (COS) were reduced to 372.4 ppmv and 411 pptv respectively. In this region, urban and industrial influences were evidenced by elevated mixing ratios and good linear relationships between urban and industrial tracers compared to North Atlantic background air. Moreover, low mixing ratios and a good correlation between COS and CO2 showed a fingerprint of terrestrial uptake and minimal dilution during rapid transport over a 1–2 day time period. Analysis of synoptic conditions, backward trajectories, and photochemical aging estimates based on C3H8/C2H6 strongly suggested that elevated anthropogenic tracers in the upper troposphere of the flight region were the result of transport via convection and warm conveyor belt (WCB) uplifting of boundary layer air over the southeastern US. This mechanism is supported by the similar slope values of linear correlations between long-lived (months) anthropogenic tracers (e.g., C2Cl4 and CHCl3) from the flight region and the planetary boundary layer in the southeastern US. In addition, the aircraft measurements suggest that outflow from the US augmented the entire tropospheric column at mid-latitudes over the North Atlantic. Overall, the flight 13 data demonstrate a pervasive impact of US anthropogenic emissions on the troposphere over the North Atlantic.


2017 ◽  
Vol 30 (17) ◽  
pp. 6629-6643 ◽  
Author(s):  
Dachao Jin ◽  
Zhaoyong Guan

Using the NCEP–NCAR reanalysis and other observational datasets, the authors have investigated the relationship of summer rainfall variations between the Hetao region of northern China and the middle and lower reaches of Yangtze River (MLRYR). The results have demonstrated that rainfall in Hetao varies out of phase with that in MLRYR on the interannual time scales. This phenomenon is referred to as the Hetao–Yangtze rainfall seesaw (HYRS). An HYRS index is defined to reveal both spatial and temporal features of HYRS. It is found that the North Atlantic Oscillation (NAO) affects the HYRS. In years when the NAO is in its positive phase, anomalous divergences in the lower troposphere and anomalous convergences in the upper troposphere are observed in regions of the Mediterranean and eastern Europe. The anomalous convergences in the upper troposphere occur as the positive Rossby wave source excites a circumglobal teleconnection (CGT) in the midlatitudes, exhibiting the eastward propagation of Rossby wave energy along the Asian jet. Meanwhile, the Eurasian–Pacific (EUP) teleconnection also affects the HYRS. Influenced mainly by the CGT pattern, the circulations over Hetao and MLRYR are consequently perturbed. The atmosphere over Hetao converges anomalously in the lower troposphere and diverges anomalously in the upper troposphere, facilitating more than normal rainfall there. At the same time, the atmosphere over MLRYR diverges anomalously in the lower troposphere and converges anomalously in the upper troposphere, resulting in more than normal summer rainfall in MLRYR. In this way, the north–south rainfall seesaw is formed. This NAO-induced rainfall seesaw is potentially useful for summer rainfall predictions in both MLRYR and the Hetao region of northern China.


2018 ◽  
Author(s):  
Thorsten Kaluza ◽  
Daniel Kunkel ◽  
Peter Hoor

Abstract. The variability and similarities in the evolution of the tropopause inversion (TIL) layer during cyclongenesis in the North Atlantic storm track are investigated using operational meteorological analysis data (Integrated Forecast System from the European Centre for Medium-Range Weather Forecasts). For this a total amount of 130 cyclones have been analysed which evolved during the months August through October between 2010–2014 over the North Atlantic. Their paths of migration along with associated flow features in the upper troposphere/lower stratosphere (UTLS) have been tracked using the mean sea level pressure. Subsets of the 130 cyclones have been used for composite analysis using minimum sea level pressure to filter the cyclones based on their strength. The composite structure of the TIL strength distribution in connection with the overall UTLS flow strongly resembles the structure of the individual cyclones. Key results are that a strong dipole in tropopause inversion layer strength forms in regions of cyclonic wrap-up of UTLS air masses of different origin and isentropic potential vorticity. These air masses are associated with the cyclonic rotation of the underlaying cyclones. The maximum values of enhanced static stability above the tropopause occur north and northeast of the cyclone centre, vertically aligned with outflow regions of strong updraft and cloud formation up to the tropopause, which are situated in anticyclonic flow patterns in the upper troposphere. These regions are colocated with a maximum of vertical shear of the horizontal wind. The strong wind shear within the TIL results in a local minimum of Richardson numbers, representing the possibility for turbulent instability and potential mixing (or air mass exchange) within regions of enhanced static stability in the lowermost stratosphere.


2021 ◽  
Vol 21 (10) ◽  
pp. 8213-8232
Author(s):  
Gerald Wetzel ◽  
Felix Friedl-Vallon ◽  
Norbert Glatthor ◽  
Jens-Uwe Grooß ◽  
Thomas Gulde ◽  
...  

Abstract. Measurements of the pollution trace gases ethane (C2H6), ethyne (C2H2), formic acid (HCOOH), and peroxyacetyl nitrate (PAN) were performed in the North Atlantic upper troposphere and lowermost stratosphere (UTLS) region with the airborne limb imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) with high spatial resolution down to cloud top. Observations were made during flights with the German research aircraft HALO (High Altitude and LOng Range Research Aircraft) in the frame of the WISE (Wave-driven ISentropic Exchange) campaign, which was carried out in autumn 2017 from Shannon (Ireland) and Oberpfaffenhofen (Germany). Enhanced volume mixing ratios (VMRs) of up to 2.2 ppbv C2H6, 0.2 ppbv C2H2, 0.9 ppbv HCOOH, and 0.4 ppbv PAN were detected during the flight on 13 September 2017 in the upper troposphere and around the tropopause above the British Isles. Elevated quantities of PAN were measured even in the lowermost stratosphere (locally up to 14 km), likely reflecting the fact that this molecule has the longest lifetime of the four species discussed herein. Backward trajectory calculations as well as global three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS) simulations with artificial tracers of air mass origin have shown that the main sources of the observed pollutant species are forest fires in North America and anthropogenic pollution in South Asia and Southeast Asia uplifted and moved within the Asian monsoon anticyclone (AMA) circulation system. After release from the AMA, these species or their precursor substances are transported by strong tropospheric winds over large distances, depending on their particular atmospheric lifetime of up to months. Observations are compared to simulations with the atmospheric models EMAC (ECHAM5/MESSy Atmospheric Chemistry) and CAMS (Copernicus Atmosphere Monitoring Service). These models are qualitatively able to reproduce the measured VMR enhancements but underestimate the absolute amount of the increase. Increasing the emissions in EMAC by a factor of 2 reduces the disagreement between simulated and measured results and illustrates the importance of the quality of emission databases used in chemical models.


2020 ◽  
Author(s):  
Gerald Wetzel ◽  
Felix Friedl-Vallon ◽  
Norbert Glatthor ◽  
Jens-Uwe Grooß ◽  
Thomas Gulde ◽  
...  

Abstract. Measurements of the pollution trace gases ethane (C2H6), ethyne (C2H2), formic acid (HCOOH), and peroxyacetyl nitrate (PAN) were performed in the North Atlantic upper troposphere and lowermost stratosphere (UTLS) region with the airborne limb imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) with high spatial resolution down to cloud top. Observations were made during flights with the German research aircraft HALO (High Altitude and LOng Range Research Aircraft) in the frame of the WISE (Wave-driven ISentropic Exchange) campaign, which was carried out in autumn 2017 from Shannon (Ireland) and Oberpfaffenhofen (Germany). Enhanced volume mixing ratios (VMR) of up to 2.2 ppbv C2H6, 0.2 ppbv C2H2, 0.9 ppbv HCOOH, and 0.4 ppbv PAN were detected during the flight on 13 September 2017 in the upper troposphere and around the tropopause above the British Isles. Since PAN has the longest lifetime of this foursome, elevated quantities of this molecule could be measured even in the lowermost stratosphere (locally up to 14 km). Backward trajectory calculations as well as global three-dimensional CLaMS simulations with artificial tracers of air mass origin have shown that the main sources of the observed pollutant species are forest fires in North America and anthropogenic pollution in South and Southeast Asia uplifted and moved within the Asian monsoon anticyclone (AMA) circulation system. After release from the AMA, these species or their precursor substances are transported by strong tropospheric winds over large distances, depending on their particular atmospheric lifetime of up to months. Observations are compared to simulations with the atmospheric models EMAC (ECHAM5/MESSy Atmospheric Chemistry) and CAMS (Copernicus Atmosphere Monitoring Service). These models are qualitatively able to reproduce the measured VMR enhancements but underestimate the absolute amount of the increase. Increasing the emissions in EMAC by a factor of 2 reduces the disagreement between simulated and measured results and illustrates the importance of the quality of emission databases used in chemical models.


2008 ◽  
Vol 21 (18) ◽  
pp. 4680-4690 ◽  
Author(s):  
Jian Li ◽  
Rucong Yu ◽  
Tianjun Zhou

Abstract Analysis of the monthly NCEP–NCAR reanalysis data and station data reveals a teleconnection pattern (NAULEA) that links climate changes over the North Atlantic and Eurasia. The NAULEA pattern has five action centers. It extends from the North Atlantic to northwestern Europe, and then stretches eastward to the Urals, with its eastern end over North China. Certain climate changes over East Asia, such as the cooling changes in both the upper troposphere and surface in the last few decades of the twentieth century, can be attributed to the NAULEA pattern anomalies and traced upstream to the North Atlantic. The NAULEA pattern is suggested to be another NAO-related teleconnection pattern. Compared with the pattern with the Asian jet waveguide path, which leads to temperature anomalies over northeastern Asia, the NAULEA pattern with a high-latitude path exerts stronger influences on the climate of southwestern China.


2020 ◽  
Vol 33 (24) ◽  
pp. 10523-10537
Author(s):  
Sijie Huang ◽  
Xiuzhen Li ◽  
Zhiping Wen

AbstractThe characteristics and possible energy sources of the South Asian jet wave train in winter are analyzed, with the intraseasonal signal emphasized. The wave train is equivalently barotropic and strongest in the upper troposphere, with its daily evolution dominated by the intraseasonal (10–30 day) time scale. Along the wave train, the propagation of disturbances from the North Atlantic to the western North Pacific takes around 8 days, which is much faster than the eastward migration of activity centers. The energy sources of the intraseasonal wave train are complicated and can be separated into three categories depending on the role of the North Atlantic Oscillation (NAO). When NAO− precedes the wave train, it is northwest–southeast oriented. The energy is rooted in the lower troposphere over the high-latitude North Atlantic, and excites the Rossby wave source (RWS) over the western Mediterranean Sea via vortex stretching by abnormal divergence. When NAO+ precedes the wave train, it is southwest–northeast oriented. The energy rooted in the northeastern activity center excites RWS over the eastern Mediterranean Sea. Additionally, disturbances from the western North Atlantic and southwestern activity center of NAO+ excite the RWS over the western Mediterranean Sea. Hence, both NAO− and NAO+ can excite the same wave train, but with different orientation and via different paths. Without the NAO, the wave train can also be stimulated by enhanced disturbances over the midlatitude central North Atlantic. The signal lies mainly in the middle-upper troposphere, which might be related to atmospheric internal dynamic processes, such as kinetic energy conversion from synoptic disturbances.


2021 ◽  
Author(s):  
Chao Xu ◽  
Yaoming Ma ◽  
Jiehua Ma ◽  
Chao You ◽  
Huijun Wang

<p>Dust is a major component of atmospheric aerosol worldwide, greatly affecting regional and global climate. A dust belt can be clearly found at altitudes higher than 6 km over the downwind direction of the TP at latitudes of around 30°–40°N, crossing the Pacific Ocean and extending to North America during spring. Dust is uplifted to the midtroposphere over the source regions; then, frequent, deep, dry convection prevailing over the TP during spring can cause convective overshooting that uplifts the dust aerosols to the upper troposphere. The TP thus acts as a channel for transporting dust from the lower atmosphere to the upper troposphere, enabling the long-range zonal transport of dust around the Northern Hemisphere. Estimated spring dust mass flux (DMF) showed a significant declining trend over the TP during 2007-2019. The total spring DMF across the TP was mainly affected by DMFs over the Tarim Basin, while the spring DMF across the TP in the mid-troposphere was also connected with DMFs over the northwest Indian Peninsula and Central Asia. Inter-annual variability of spring DMF across the TP was strongly correlated with the North Atlantic winter sea surface temperature (SST) tripole. The North Atlantic winter SST tripole anomalies persist into the subsequent spring, and induce a corresponding atmosphere response. A strong positive North Atlantic winter SST tripole anomaly strengthens the upper-level westerly jets, enhancing air flow towards the TP mid-troposphere; together, these circulation patterns cause anomalous cyclonic conditions in the lower troposphere, especially over the Tarim Basin, via the eastwards propagation of a Rossby wave train. These atmospheric circulation conditions are likely to increase the frequency of dust occurrence and promote the transport of dust onto the TP.</p>


1961 ◽  
Vol 14 (4) ◽  
pp. 432-445
Author(s):  
A. F. Crossley

From an inspection of upper-air contour charts for 300 and 200 mb., the location of the axis of jet streams of 80 kt. or more has been assessed once daily over the two years 1957–8. Results are presented for each of the four seasons by means of isopleths of frequency (Fig. 1) and also by means of frequency-roses in areas of 5 degrees of latitude by 10 degrees of longitude (Figs. 2–5); each rose shows the number of occasions of direction of the axis from the eight compass points. The area covered extends from latitude 30° N. to 70° N., and from longitude 60° W. to 30° E. An Appendix contains some discussion of the technique of locating the axis of jet streams on contour charts.The characteristics of jet streams were described in a paper by Chambers in this Journal for July/October 1959. The present paper goes a stage further by giving the number of occurrences of jet streams per season over a two-year period in an area from the North Atlantic to the Mediterranean. The number of occurrences depends very much on the chosen definition, about which there is no general agreement. Whilst a jet stream may be fairly described as a fast-moving stream of air in the upper troposphere with great extension in the direction of the wind and persistence of the order of days, for statistical purposes it is necessary to be more precise. In this paper a critical speed of 80 kt. is required at the 300- or 200-mb. level in order that the stream shall qualify as a jet stream. Further discussion of this point is given in the Appendix, but any definition is largely subjective and it does not matter a great deal what definition is used provided the reader is aware of the limits to which the statistics refer.


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