In situ measurements of the NOxdistribution and variability over the eastern North Atlantic

1999 ◽  
Vol 104 (D13) ◽  
pp. 16021-16032 ◽  
Author(s):  
H. Ziereis ◽  
H. Schlager ◽  
P. Schulte ◽  
I. Köhler ◽  
R. Marquardt ◽  
...  
2008 ◽  
Vol 113 (C3) ◽  
Author(s):  
Andrés Cianca ◽  
Peer Helmke ◽  
Beatriz Mouriño ◽  
María José Rueda ◽  
Octavio Llinás ◽  
...  

1999 ◽  
Vol 65 (6) ◽  
pp. 2585-2591 ◽  
Author(s):  
Nyree J. West ◽  
David J. Scanlan

ABSTRACT The in situ community structure of Prochlorococcuspopulations in the eastern North Atlantic Ocean was examined by analysis of Prochlorococcus 16S rDNA sequences with three independent approaches: cloning and sequencing, hybridization to specific oligonucleotide probes, and denaturing gradient gel electrophoresis (DGGE). The hybridization of high-light (HL) and low-light (LL) Prochlorococcus genotype-specific probes to two depth profiles of PCR-amplified 16S rDNA sequences revealed that in these two stratified water columns, an obvious niche-partitioning ofProchlorococcus genotypes occurred. In each water column a shift from the HL to the LL genotype was observed, a transition correlating with the depth of the surface mixed layer (SML). Only the HL genotype was found in the SML in each water column, whereas the LL genotype was distributed below the SML. The range of in situ irradiance to which each genotype was subjected within these distinct niches was consistent with growth irradiance studies of cultured HL- and LL-adapted Prochlorococcus strains. DGGE analysis and the sequencing of Prochlorococcus 16S rDNA clones were in full agreement with the genotype-specific oligonucleotide probe hybridization data. These observations of a partitioning ofProchlorococcus genotypes in a stratified water column provide a genetic basis for the dim and brightProchlorococcus populations observed in flow cytometric signatures in several oceanic provinces.


2016 ◽  
Vol 16 (7) ◽  
pp. 4251-4269 ◽  
Author(s):  
Yenny González ◽  
Matthias Schneider ◽  
Christoph Dyroff ◽  
Sergio Rodríguez ◽  
Emanuel Christner ◽  
...  

Abstract. We present two years of in situ measurements of water vapour (H2O) and its isotopologue ratio (δD, the standardized ratio between H216O and HD16O), made at two remote mountain sites on Tenerife in the subtropical North Atlantic. We show that the data – if measured during night-time – are well representative for the lower/middle free troposphere. We use the measured H2O-δD pairs, together with dust measurements and back trajectory modelling for analysing the moisture pathways to this region. We can identify four principally different transport pathways. The air mass transport from high altitudes and high latitudes shows two different scenarios. The first scenario brings dry air masses to the stations, as the result of condensation events occurring at low temperatures. The second scenario brings humid air masses to the stations, due to cross-isentropic mixing with lower-level and more humid air during transport since last condensation (LC). The third pathway is transportation from lower latitudes and lower altitudes, whereby we can identify rain re-evaporation as an occasional source of moisture. The fourth pathway is linked to the African continent, where during summer, dry convection processes over the Sahara very effectively inject humidity from the boundary layer to higher altitudes. This so-called Saharan Air Layer (SAL) is then advected westward over the Atlantic and contributes to moisten the free troposphere. We demonstrate that the different pathways leave distinct fingerprints on the measured H2O-δD pairs.


Author(s):  
Andrés Cianca ◽  
Peer Helmke ◽  
Beatriz Mouriño ◽  
María José Rueda ◽  
Octavio Llinás ◽  
...  

2018 ◽  
Vol 18 (23) ◽  
pp. 17191-17206 ◽  
Author(s):  
Gary Lloyd ◽  
Thomas W. Choularton ◽  
Keith N. Bower ◽  
Martin W. Gallagher ◽  
Jonathan Crosier ◽  
...  

Abstract. A key challenge for numerical weather prediction models is representing boundary layer clouds in cold air outbreaks (CAOs). One important aspect is the evolution of microphysical properties as stratocumulus transitions to open cellular convection. Abel et al. (2017) have shown, for the first time from in situ field observations, that the break-up in CAOs over the eastern Atlantic may be controlled by the development of precipitation in the cloud system while the boundary layer becomes decoupled. This paper describes that case and examines in situ measurements from three more CAOs. Flights were conducted using the UK Facility for Airborne Atmospheric Measurements (FAAM) British Aerospace-146 (BAe-146) aircraft in the North Atlantic region around the UK, making detailed microphysical measurements in the stratiform boundary layer. As the cloudy boundary layer evolves prior to break-up, increasing liquid water paths (LWPs) and drop sizes and the formation of liquid precipitation are observed. Small numbers of ice particles, typically a few per litre, are also observed. Eventually LWPs reduce significantly due to loss of water from the stratocumulus cloud (SC) layer. In three of the cases, aerosols are removed from the boundary layer across the transition. This process appears to be similar to those observed in warm clouds and pockets of open cells (POCs) in the subtropics. After break-up, deeper convective clouds form with bases warm enough for secondary ice production (SIP), leading to rapid glaciation. It is concluded that the precipitation is strongly associated with the break-up, with both weakening of the capping inversion and boundary layer decoupling also observed.


2007 ◽  
Vol 25 (11) ◽  
pp. 2247-2257 ◽  
Author(s):  
C. Jamet ◽  
C. Moulin ◽  
N. Lefèvre

Abstract. Automated instruments on board Volunteer Observing Ships (VOS) have provided high-frequency pCO2 measurements over basin-wide regions for a decade or so. In order to estimate regional air-sea CO2 fluxes, it is necessary to interpolate between in-situ measurements to obtain maps of the marine pCO2. Such an interpolation remains, however, a difficult task because VOS lines are too distant from each other to capture the high pCO2 variability. Relevant physical parameters available at large scale are thus necessary to serve as a guide to estimate the pCO2 values between the VOS lines. Satellites do not measure pCO2 but they give access to parameters related to the processes that control its variability, such as sea surface temperature (SST). In this paper we developed a method to compute pCO2 maps using satellite data (SST and CHL, the chlorophyll concentration), combined with a climatology of the mixed-layer depth (MLD). Using 15 401 measurements of surface pCO2 acquired in the North Atlantic between UK and Jamaica, between June 1994 and August 1995, we show that the parameterization of pCO2 as a function of SST, CHL and MLD yields more realistic pCO2 values than parameterizations that have been widely used in the past, based on SST, latitude, longitude or SST only. This parameterization was then used to generate seasonal maps of pCO2 over the North Atlantic. Results show that our approach yields the best marine pCO2 estimates, both in terms of absolute accuracy, when compared with an independent data set, and of geographical patterns, when compared to the climatology of Takahashi et al. (2002). This suggests that monitoring the seasonal variability of pCO2 over basin-wide regions is possible, provided that sufficient VOS lines are available.


2018 ◽  
Vol 18 (15) ◽  
pp. 11303-11322 ◽  
Author(s):  
Qianqian Song ◽  
Zhibo Zhang ◽  
Hongbin Yu ◽  
Seiji Kato ◽  
Ping Yang ◽  
...  

Abstract. In this study, we integrate recent in situ measurements with satellite retrievals of dust physical and radiative properties to quantify dust direct radiative effects on shortwave (SW) and longwave (LW) radiation (denoted as DRESW and DRELW, respectively) in the tropical North Atlantic during the summer months from 2007 to 2010. Through linear regression of the CERES-measured top-of-atmosphere (TOA) flux versus satellite aerosol optical depth (AOD) retrievals, we estimate the instantaneous DRESW efficiency at the TOA to be -49.7±7.1 W m−2 AOD−1 and -36.5±4.8 W m−2 AOD−1 based on AOD from MODIS and CALIOP, respectively. We then perform various sensitivity studies based on recent measurements of dust particle size distribution (PSD), refractive index, and particle shape distribution to determine how the dust microphysical and optical properties affect DRE estimates and its agreement with the above-mentioned satellite-derived DREs. Our analysis shows that a good agreement with the observation-based estimates of instantaneous DRESW and DRELW can be achieved through a combination of recently observed PSD with substantial presence of coarse particles, a less absorptive SW refractive index, and spheroid shapes. Based on this optimal combination of dust physical properties we further estimate the diurnal mean dust DRESW in the region of −10 W m−2 at TOA and −26 W m−2 at the surface, respectively, of which ∼ 30 % is canceled out by the positive DRELW. This yields a net DRE of about −6.9 and −18.3 W m−2 at TOA and the surface, respectively. Our study suggests that the LW flux contains useful information on dust particle size, which could be used together with SW observations to achieve a more holistic understanding of the dust radiative effect.


2010 ◽  
Vol 40 (8) ◽  
pp. 1881-1893 ◽  
Author(s):  
Jan D. Zika ◽  
Trevor J. McDougall ◽  
Bernadette M. Sloyan

Abstract The tracer-contour inverse method is used to infer mixing and circulation in the eastern North Atlantic. Solutions for the vertical mixing coefficient D, the along-isopycnal mixing coefficient K, and a geostrophic streamfunction Ψ are all direct outputs of the method. The method predicts a vertical mixing coefficient O(10−5 m2 s−1) in the upper 1000 m of the water column, consistent with in situ observations. The method predicts a depth-dependent along-isopycnal mixing coefficient that decreases from O(1000 m2 s−1) close to the mixed layer to O(100 m2 s−1) in the interior, which is also consistent with observations and previous hypotheses. The robustness of the result is tested with a rigorous sensitivity analysis including the use of two independently constructed datasets. This study confirms the utility of the tracer-contour inverse method. The results presented support the hypothesis that vertical mixing is small in the thermocline of the subtropical Atlantic Ocean. A strong depth dependence of the along-isopycnal mixing coefficient is also demonstrated, supporting recent parameterizations for coarse-resolution ocean models.


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