scholarly journals Modeling of light scattering in cirrus clouds with inhomogeneous hexagonal monocrystals. Comparison with in-situ and ADEOS-POLDER measurements

2000 ◽  
Vol 27 (1) ◽  
pp. 113-116 ◽  
Author(s):  
Laurent C. -Labonnote ◽  
Gérard Brogniez ◽  
Marie Doutriaux-Boucher ◽  
Jean-Claude Buriez ◽  
Jean-François Gayet ◽  
...  
Keyword(s):  
Light Scattering ◽  
Cirrus Clouds

Modeling of polarized light scattering in cirrus clouds: validation with in-situ measurements and ADEOS-POLDER reflectance observations

1999 ◽  
Author(s):  
Laurent C. Labonnote ◽  
Gerard Brogniez ◽  
Jean-Francois Gayet ◽  
Jean-Claude Buriez ◽  
Marie Doutriaux-Boucher
Keyword(s):  
Light Scattering ◽  
Polarized Light ◽  
In Situ Measurements ◽  
Cirrus Clouds

In-Situ Dual-Wavelength Ellipsometry and Light Scattering Monitoring of Si/Si1−xGex Heterostructures and Multiuantum Wells

1993 ◽  
Vol 324 ◽  
Author(s):  
C. Pickering ◽  
D.A.O. Hope ◽  
W.Y. Leong ◽  
D.J. Robbins ◽  
R. Greef
Keyword(s):  
Growth Rate ◽  
Light Scattering ◽  
Laser Light ◽  
Growth Period ◽  
Laser Light Scattering ◽  
Heterojunction Bipolar Transistor ◽  
Dual Wavelength ◽  
Multi Quantum Well ◽  
Refractive Index Data

AbstractIn-situ dual-wavelength ellipsometry and laser light scattering have been used to monitor growth of Si/Si1−x,Gex heterojunction bipolar transistor and multi-quantum well (MQW) structures. The growth rate of B-doped Si0 8Ge0.2 has been shown to be linear, but that of As-doped Si is non-linear, decreasing with time. Refractive index data have been obtained at the growth temperature for x = 0.15, 0.20, 0.25. Interface regions ∼ 6-20Å thickness have been detected at hetero-interfaces and during interrupted alloy growth. Period-to-period repeatability of MQW structures has been shown to be ±lML.

First global assessment of modelled aerosol hygroscopicity in the context of other aerosol optical properties

2021 ◽  
Author(s):  
Maria Ángeles Burgos Simón ◽  
Elisabeth Andrews ◽  
Gloria Titos ◽  
Angela Benedetti ◽  
Huisheng Bian ◽  
...  
Keyword(s):  
Optical Properties ◽  
Light Scattering ◽  
Relative Humidity ◽  
Water Uptake ◽  
Chem Phys ◽  
Earth System ◽  
Aerosol Optical Properties ◽  
System Models ◽  
Earth System Models

<p>The particle hygroscopic growth impacts the optical properties of aerosols and, in turn, affects the aerosol-radiation interaction and calculation of the Earth’s radiative balance. The dependence of particle light scattering on relative humidity (RH) can be described by the scattering enhancement factor f(RH), defined as the ratio between the particle light scattering coefficient at a given RH divided by its dry value.</p><p>The first effort of the AeroCom Phase III – INSITU experiment was to develop an observational dataset of scattering enhancement values at 26 sites to study the uptake of water by atmospheric aerosols, and evaluate f(RH) globally (Burgos et al., 2019). Model outputs from 10 Earth System Models (CAM, CAM-ATRAS, CAM-Oslo, GEOS-Chem, GEOS-GOCART, MERRAero, TM5, OsloCTM3, IFS-AER, and ECMWF) were then evaluated against this in-situ dataset. Building on these results, we investigate f(RH) in the context of other aerosol optical and chemical properties, making use of the same 10 Earth System Models (ESMs) and in-situ measurements as in Burgos et al. (2020) and Titos et al. (2021).</p><p>Given the difficulties of deploying and maintaining instrumentation for long-term, accurate and comprehensive f(RH) observations, it is desirable to find an observational proxy for f(RH). This observation-based proxy would also need to be reproduced in modelling space. Our aim here is to evaluate how ESMs currently represent the relationship between f(RH), scattering Ångström exponent (SAE), and single scattering albedo (SSA). This work helps to identify current challenges in modelling water-uptake by aerosols and their impact on aerosol optical properties within Earth system models.</p><p>We start by analyzing the behavior of SSA with RH, finding the expected increase with RH for all site types and models. Then, we analyze the three variables together (f(RH)-SSA-SAE relationship). Results show that hygroscopic particles tend to be bigger and scatter more than non-hygroscopic small particles, though variability within models is noticeable. This relationship can be further studied by relating SAE to model chemistry, by selecting those grid points dominated by a single chemical component (mass mixing ratios > 90%). Finally, we analyze model performance at three specific sites representing different aerosol types: Arctic, marine and rural. At these sites, the model data can be exactly temporally and spatially collocated with the observations, which should help to identify the models which exhibit better agreement with measurements and for which aerosol type.</p><p> </p><p>Burgos, M.A. et al.: A global view on the effect of water uptake on aerosol particle light scattering. Sci Data 6, 157. https://doi.org/10.1038/s41597-019-0158-7, 2019.</p><p>Burgos, M.A. et al.: A global model–measurement evaluation of particle light scattering coefficients at elevated relative humidity, Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, 2020.</p><p>Titos, G. et al.: A global study of hygroscopicity-driven light scattering enhancement in the context of other in-situ aerosol optical properties, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2020-1250, in review, 2020.</p>

Aqueous solubilization of hydrophobic supramolecular metal–organic nanocapsules

2014 ◽  
Vol 5 (6) ◽  
pp. 2554-2559 ◽  
Author(s):  
H. Kumari ◽  
S. R. Kline ◽  
J. L. Atwood
Keyword(s):  
Light Scattering ◽  
Dynamic Light Scattering ◽  
Neutron Scattering ◽  
Metal Organic

Micelles of surfactant solubilized metal-seamed pyrogallol[4]arene based organic nanocapsules are synthesized and characterized using in situ neutron scattering and dynamic light scattering techniques, which show trends in sizes as a function of alkyl tails of pyrogallols and surfactants.

Dynamic Processes in Cirrus Clouds: Concepts and Models

Cirrus ◽  
2002 ◽  
Author(s):  
David O’C. Starr ◽  
Markus Quante
Keyword(s):  
Cirrus Clouds ◽  
Radiative Properties ◽  
Cirrus Cloud ◽  
Early Model ◽  
Minimum Requirement ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Cloud Models ◽  
New Concepts

Advancement in the understanding of cirrus clouds and their life cycle comes through symbiotic use of models, observations, and related concepts (fig. 18.1). Models of cirrus clouds represent an integration of our knowledge of cirrus cloud properties and processes. They provide a capacity to extend knowledge and enhance understanding in ways that complement existing observational capabilities. Models can be used to develop new theories, such as parameterizations, and focus science issues and observational requirements and developments. For example, early model results of Starr and Cox (1985a) and Starr (1987b) predicted that fine cellular structure (~lkm or less) would be found in the upper part of extended stratiform cirrus clouds. This prediction was confirmed when high-frequency sensors were deployed both for active remote sensing (Sassen et al. 1990a, 1995) and later for in-situ measurements (Quante and Brown 1992; Gultepe et al. 1995; Quante et al. 1996). Sampling rates of 10Hz, or better, are now accepted as a minimum requirement for resolving cirrus cloud internal structure and circulation where 1-Hz or coarser measurements were previously used. Similarly, discrepancies between observed cloud radiative properties and calculations (theory) based on corresponding in-situ observations of cloud microphysical properties (Sassen et al. 1990b) led to the development of improved observing capabilities for small ice crystals (Arnott et al. 1994; Miloshevich and Heymsfield 1997; Lawson et al. 1998). Such sensors are now regarded as part of the standard complement when doing in-situ microphysical measurements in cirrus. At the same time, observations are absolutely essential in developing and evaluating cloud models. No cloud modeler wants to apply a model or theory too far beyond the limits of what can be observationally confirmed, at least in gross terms. The third aspect of this triad is concepts. Although models and observations can lead to predictions or diagnosis of unexpected relationships, they are each limited by the concepts that were used in their design and/or implementation. In the end, new concepts arising from analogy to other phenomena and/or from synergistic integration of existing knowledge can lead to new understanding, new models, new instruments, and new sampling strategies (fig. 18.1). Chapter 17 focuses on observations of internal cloud circulation and structure.

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