Mechanism of DNA Adsorption and Desorption on Graphene Oxide

Langmuir ◽  
2014 ◽  
Vol 30 (42) ◽  
pp. 12587-12595 ◽  
Author(s):  
Joon Soo Park ◽  
Nam-In Goo ◽  
Dong-Eun Kim
RSC Advances ◽  
2014 ◽  
Vol 4 (102) ◽  
pp. 58778-58787 ◽  
Author(s):  
Weifan Chen ◽  
Linlin Wang ◽  
Mingpeng Zhuo ◽  
Yiping Wang ◽  
Sulei Fu ◽  
...  

Schematic diagram of Y(iii) adsorption and desorption on graphene oxide nanosheets in colloidal suspensions loaded in a dialysis bag.


2006 ◽  
Vol 21 (11) ◽  
pp. 2137-2145 ◽  
Author(s):  
Andrew L. Hook ◽  
Helmut Thissen ◽  
Jason P. Hayes ◽  
Nicolas H. Voelcker

Langmuir ◽  
2011 ◽  
Vol 27 (6) ◽  
pp. 2731-2738 ◽  
Author(s):  
Marissa Wu ◽  
Ravindra Kempaiah ◽  
Po-Jung Jimmy Huang ◽  
Vivek Maheshwari ◽  
Juewen Liu

Coatings ◽  
2020 ◽  
Vol 10 (3) ◽  
pp. 289 ◽  
Author(s):  
Sebastian Muraru ◽  
Cosmin G. Samoila ◽  
Emil I. Slusanschi ◽  
Jorge S. Burns ◽  
Mariana Ionita

Graphene and its functionalised derivatives are transforming the development of biosensors that are capable of detecting nucleic acid hybridization. Using a Molecular Dynamics (MD) approach, we explored single-stranded or double-stranded deoxyribose nucleic acid (ssDNA or dsDNA) adsorption on two graphenic species: graphene oxide (GO) and reduced graphene oxide functionalized with aminated polyethylene glycol (rGO-PEG-NH2). Innovatively, we included chloride (Cl−) and magnesium (Mg2+) ions that influenced both the ssDNA and dsDNA adsorption on GO and rGO-PEG-NH2 surfaces. Unlike Cl−, divalent Mg2+ ions formed bridges between the GO surface and DNA molecules, promoting adsorption through electrostatic interactions. For rGO-PEG-NH2, the Mg2+ ions were repulsed from the graphenic surface. The subsequent ssDNA adsorption, mainly influenced by electrostatic forces and hydrogen bonds, could be supported by π–π stacking interactions that were absent in the case of dsDNA. We provide a novel insight for guiding biosensor development.


2018 ◽  
Vol 18 (9) ◽  
pp. 6364-6368
Author(s):  
Hyun Jin Yoo ◽  
Changyoon Baek ◽  
Donghyun Lee ◽  
Junhong Min

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