Modulated Nonlinear Optical Responses and Charge Transfer Transition in Endohedral Fullerene Dimers Na@C60C60@F with n-Fold Covalent Bond (n = 1, 2, 5, and 6) and Long Range Ion Bond

2010 ◽  
Vol 114 (25) ◽  
pp. 11242-11247 ◽  
Author(s):  
Fang Ma ◽  
Zhi-Ru Li ◽  
Zhong-Jun Zhou ◽  
Di Wu ◽  
Ying Li ◽  
...  
2017 ◽  
Vol 19 (47) ◽  
pp. 31958-31964 ◽  
Author(s):  
Feng-Wei Gao ◽  
Hong-liang Xu ◽  
Zhong-Min Su

Different strengths of external electric fields enhance the stability, control the inter-molecular charge transfer and strengthen the nonlinear optical responses of a π-dimer.


2018 ◽  
Vol 20 (27) ◽  
pp. 18699-18706 ◽  
Author(s):  
Feng-Wei Gao ◽  
Hong-Liang Xu ◽  
Shabbir Muhammad ◽  
Zhong-Min Su

External electric fields were found to induce intra- and intermolecular charge transfer and strengthen the second-order nonlinear optical responses of π-dimers.


2020 ◽  
Vol 5 (1) ◽  
Author(s):  
Zhuoliang Ni ◽  
B. Xu ◽  
M.-Á. Sánchez-Martínez ◽  
Y. Zhang ◽  
K. Manna ◽  
...  

AbstractChiral topological semimetals are materials that break both inversion and mirror symmetries. They host interesting phenomena such as the quantized circular photogalvanic effect (CPGE) and the chiral magnetic effect. In this work, we report a comprehensive theoretical and experimental analysis of the linear and nonlinear optical responses of the chiral topological semimetal RhSi, which is known to host multifold fermions. We show that the characteristic features of the optical conductivity, which display two distinct quasi-linear regimes above and below 0.4 eV, can be linked to excitations of different kinds of multifold fermions. The characteristic features of the CPGE, which displays a sign change at 0.4 eV and a large non-quantized response peak of around 160 μA/V2 at 0.7 eV, are explained by assuming that the chemical potential crosses a flat hole band at the Brillouin zone center. Our theory predicts that, in order to observe a quantized CPGE in RhSi, it is necessary to increase the chemical potential as well as the quasiparticle lifetime. More broadly, our methodology, especially the development of the broadband terahertz emission spectroscopy, could be widely applied to study photogalvanic effects in noncentrosymmetric materials and in topological insulators in a contact-less way and accelerate the technological development of efficient infrared detectors based on topological semimetals.


2021 ◽  
pp. 2009476
Author(s):  
Yoshihisa Kosugi ◽  
Masato Goto ◽  
Zhenhong Tan ◽  
Asaya Fujita ◽  
Takashi Saito ◽  
...  

2021 ◽  
Vol 31 (25) ◽  
pp. 2170178
Author(s):  
Yoshihisa Kosugi ◽  
Masato Goto ◽  
Zhenhong Tan ◽  
Asaya Fujita ◽  
Takashi Saito ◽  
...  

1996 ◽  
Vol 104 (15) ◽  
pp. 5821-5833 ◽  
Author(s):  
Oliver Kühn ◽  
Valery Rupasov ◽  
Shaul Mukamel

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