On the Use of Plasmonic Nanoparticle Pairs As a Plasmon Ruler: The Dependence of the Near-Field Dipole Plasmon Coupling on Nanoparticle Size and Shape†

2009 ◽  
Vol 113 (10) ◽  
pp. 1946-1953 ◽  
Author(s):  
Christopher Tabor ◽  
Raghunath Murali ◽  
Mahmoud Mahmoud ◽  
Mostafa A. El-Sayed
Nanophotonics ◽  
2020 ◽  
Vol 9 (7) ◽  
pp. 2097-2105
Author(s):  
Xiaozhuo Qi ◽  
Tsz Wing Lo ◽  
Di Liu ◽  
Lantian Feng ◽  
Yang Chen ◽  
...  

AbstractPlasmonic nanocavities comprised of metal film-coupled nanoparticles have emerged as a versatile nanophotonic platform benefiting from their ultrasmall mode volume and large Purcell factors. In the weak-coupling regime, the particle-film gap thickness affects the photoluminescence (PL) of quantum emitters sandwiched therein. Here, we investigated the Purcell effect-enhanced PL of monolayer MoS2 inserted in the gap of a gold nanoparticle (AuNP)–alumina (Al2O3)–gold film (Au Film) structure. Under confocal illumination by a 532 nm CW laser, we observed a 7-fold PL peak intensity enhancement for the cavity-sandwiched MoS2 at an optimal Al2O3 thickness of 5 nm, corresponding to a local PL enhancement of ∼350 by normalizing the actual illumination area to the cavity’s effective near-field enhancement area. Full-wave simulations reveal a counterintuitive fact that radiation enhancement comes from the non-central area of the cavity rather than the cavity center. By scanning an electric dipole across the nanocavity, we obtained an average radiation enhancement factor of about 65 for an Al2O3 spacer thickness of 4 nm, agreeing well with the experimental thickness and indicating further PL enhancement optimization. Our results indicate the importance of configuration optimization, emitter location and excitation condition when using such plasmonic nanocavities to modulate the radiation properties of quantum emitters.


2011 ◽  
Vol 2 (10) ◽  
pp. 1171-1177 ◽  
Author(s):  
Edward P. O’Brien ◽  
John. E. Straub ◽  
Bernard R. Brooks ◽  
D. Thirumalai

2013 ◽  
Vol 4 ◽  
pp. 632-637 ◽  
Author(s):  
Tsung Sheng Kao ◽  
Yi Guo Chen ◽  
Ming Hui Hong

By utilizing the strongly induced plasmon coupling between discrete nano-antennas and quantitatively controlling the crystalline proportions of an underlying Ge2Sb2Te5 (GST) phase-change thin layer, we show that nanoscale light localizations in the immediate proximity of plasmonic nano-antennas can be spatially positioned. Isolated energy hot-spots at a subwavelength scale can be created and adjusted across the landscape of the plasmonic system at a step resolution of λ/20. These findings introduce a new approach for nano-circuitry, bio-assay addressing and imaging applications.


Nanoscale ◽  
2019 ◽  
Vol 11 (42) ◽  
pp. 19884-19894 ◽  
Author(s):  
Samir A. Belhout ◽  
Frederico R. Baptista ◽  
Stephen J. Devereux ◽  
Anthony W. Parker ◽  
Andrew D. Ward ◽  
...  

The plasmonic properties of composites with controlled AuNP loading are found to be well described by a plasmon ruler equation, and Raman optical tweezer results show the SERS performance in the bulk is dominated by the discrete composite properties.


2015 ◽  
Vol 23 (24) ◽  
pp. 31460 ◽  
Author(s):  
Eleonora Lorek ◽  
Erik Mårsell ◽  
Arthur Losquin ◽  
Miguel Miranda ◽  
Anne Harth ◽  
...  
Keyword(s):  

Nanoscale ◽  
2016 ◽  
Vol 8 (15) ◽  
pp. 7992-8007 ◽  
Author(s):  
Jingchao Li ◽  
Jia'En Jasmine Li ◽  
Jing Zhang ◽  
Xinlong Wang ◽  
Naoki Kawazoe ◽  
...  

2017 ◽  
Vol 28 (6) ◽  
pp. 1791-1800 ◽  
Author(s):  
Jun Yue ◽  
Timothy Joel Feliciano ◽  
Wenlong Li ◽  
Andrew Lee ◽  
Teri W. Odom

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