Ultrafast Photodissociation Dynamics of Acetone at 195 nm:  II. Unraveling Complex Three-Body Dissociation Dynamics by Femtosecond Time-Resolved Photofragment Translational Spectroscopy

2005 ◽  
Vol 109 (31) ◽  
pp. 6818-6829 ◽  
Author(s):  
Wei-Kan Chen ◽  
Po-Yuan Cheng
2016 ◽  
Vol 18 (21) ◽  
pp. 14644-14653 ◽  
Author(s):  
Adam S. Chatterley ◽  
Florian Lackner ◽  
Daniel M. Neumark ◽  
Stephen R. Leone ◽  
Oliver Gessner

Using femtosecond time-resolved extreme ultraviolet absorption spectroscopy, the dissociation dynamics of the haloalkane 1,2-dibromoethane (DBE) have been explored following strong field ionization by femtosecond near infrared pulses at intensities between 7.5 × 1013 and 2.2 × 1014 W cm−2.


2013 ◽  
Vol 117 (15) ◽  
pp. 3176-3182 ◽  
Author(s):  
Hong-Kai Li ◽  
Lei Xia ◽  
Xian-Jin Zeng ◽  
Shan Xi Tian

2001 ◽  
Vol 114 (19) ◽  
pp. 8436-8444 ◽  
Author(s):  
Todd G. Clements ◽  
A. Khai Luong ◽  
Hans-Jürgen Deyerl ◽  
Robert E. Continetti

2015 ◽  
Vol 6 (1) ◽  
Author(s):  
Chan La-o-vorakiat ◽  
Teddy Salim ◽  
Jeannette Kadro ◽  
Mai-Thu Khuc ◽  
Reinhard Haselsberger ◽  
...  

Abstract Apart from broadband absorption of solar radiation, the performance of photovoltaic devices is governed by the density and mobility of photogenerated charge carriers. The latter parameters indicate how many free carriers move away from their origin, and how fast, before loss mechanisms such as carrier recombination occur. However, only lower bounds of these parameters are usually obtained. Here we independently determine both density and mobility of charge carriers in a perovskite film by the use of time-resolved terahertz spectroscopy. Our data reveal the modification of the free carrier response by strong backscattering expected from these heavily disordered perovskite films. The results for different phases and different temperatures show a change of kinetics from two-body recombination at room temperature to three-body recombination at low temperatures. Our results suggest that perovskite-based solar cells can perform well even at low temperatures as long as the three-body recombination has not become predominant.


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