Phase and Energy Relaxation of Vibrational Motion and Its Manifestation in Femtosecond Pump−Probe Experiments on I2in Rare Gas Environments

2001 ◽  
Vol 105 (32) ◽  
pp. 7501-7507 ◽  
Author(s):  
V. A. Ermoshin ◽  
V. Engel ◽  
A. K. Kazansky
1997 ◽  
Vol 101 (27) ◽  
pp. 4852-4859 ◽  
Author(s):  
G. Knopp ◽  
M. Schmitt ◽  
A. Materny ◽  
W. Kiefer

2007 ◽  
Vol 21 (13n14) ◽  
pp. 2439-2448
Author(s):  
M. BAER ◽  
G. BOUSQUET ◽  
P. M. DINH ◽  
F. FEHRER ◽  
P.-G. REINHARD ◽  
...  

We investigate the dynamics of Na clusters embedded in Ar matrices. We use a hierarchical approach, accounting microscopically for the cluster's degrees of freedom and more coarsely for the matrix. The dynamical polarizability of the Ar atoms and the strong Pauli-repulsion exerted by the Ar -electrons are taken into account. We discuss the impact of the matrix on the cluster gross properties and on its optical response. We then consider a realistic case of irradiation by a moderately intense laser and discuss the impact of the matrix on the hindrance of the explosion, as well as a possible pump probe scenario for analyzing dynamical responses.


ChemInform ◽  
2010 ◽  
Vol 28 (39) ◽  
pp. no-no
Author(s):  
G. KNOPP ◽  
M. SCHMITT ◽  
A. MATERNY ◽  
W. KIEFER

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