Wavelength- and Time-Dependent Two-Photon Photoemission Spectroscopy of Dye-Coated Silicon Surface

2000 ◽  
Vol 104 (47) ◽  
pp. 11248-11252 ◽  
Author(s):  
A. Samokhvalov ◽  
R. Naaman
Keyword(s):  
Silicon Surface ◽  
Time Dependent ◽  
Photoemission Spectroscopy ◽  
Two Photon

Characterization of Molecular Modified Surface States by Wavelength- and Time-Dependent Two-Photon Photoemission Spectroscopy

1997 ◽  
Vol 101 (20) ◽  
pp. 4085-4089 ◽  
Author(s):  
A. Kadyshevitch ◽  
R. Naaman ◽  
R. Cohen ◽  
D. Cahen ◽  
J. Libman ◽  
...  
Keyword(s):  
Surface States ◽  
Time Dependent ◽  
Photoemission Spectroscopy ◽  
Two Photon ◽  
Modified Surface

Bisporphyrin connected by tetrathiafulvalene

2009 ◽  
Vol 13 (01) ◽  
pp. 114-121 ◽  
Author(s):  
Kazuya Ogawa ◽  
Yasunori Nagatsuka
Keyword(s):  
Cross Section ◽  
Density Functional ◽  
Polar Solvent ◽  
Soret Band ◽  
Oxidation Potential ◽  
Time Dependent ◽  
Photon Absorption ◽  
Functional Theory ◽  
Two Photon Absorption ◽  
Two Photon

A new porphyrintetrathiafulvalene composite, where two porphyrins are bridged by te trathiafulvalene (TTF) using acetylene bonds was synthesized. The Q-band of the monomeric porphyrin appears at 590 nm whereas that of the composite is red-shifted to 620 nm and intensified. The Soret band is also red-shifted from 427 nm to 435 nm and much broadened, indicating the expansion of π-conjugation over the porphyrin and tetrathiafulvalene units. The HOMOs and LUMOs were calculated using time-dependent density functional theory. Voltammetric experiments revealed that the first oxidation potential of the TTF moiety in the composite was shifted by +155 mV compa red with TTF in the absence of composite. The effective two-photon absorption (2PA) cross section values were measured by using a nanosecond open aperture Z-scan method. The maximum effective 2PA cross section values were obtained at 760 nm, as 7300 GM in benzonitrile and 5900 GM in toluene. The values obtained in the polar solvent were 1.2 to 1.5 times larger than those in the nonpolar solvent.

scholarly journals Atom-atom entanglement in a not-resonant two-photon Tavis-Cummings model

2019 ◽  
Vol 220 ◽  
pp. 03018
Author(s):  
Marya O. Guslyannikova ◽  
Eugene K. Bashkirov
Keyword(s):  
Exact Solution ◽  
Density Matrix ◽  
Thermal Field ◽  
Time Dependent ◽  
Two Photon ◽  
Atomic States ◽  
Dependent Density

The entanglement between two two-level atoms (qubits) interacting not-resonantly with a one mode of thermal field in a lossless cavity via effective degenerate two-photon transitions is investigated. Based on the exact solution for the time-dependent density matrix of the system under consideration, negativity is calculated as a measure of the entanglement of atoms. The influence of a detuning on the dynamics of entanglement of atoms for separable and entangled initial atomic states and thermal cavity state is investigated.

Electronic structures of GaP(100) surface reconstructions probed with two-photon photoemission spectroscopy

2014 ◽  
Vol 89 (16) ◽  
Author(s):  
Philipp Sippel ◽  
Oliver Supplie ◽  
Matthias M. May ◽  
Rainer Eichberger ◽  
Thomas Hannappel
Keyword(s):  
Electronic Structures ◽  
Photoemission Spectroscopy ◽  
Two Photon ◽  
Surface Reconstructions
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