Molecule Self-Assembly Synthesis of Porous Few-Layer Carbon Nitride for Highly Efficient Photoredox Catalysis

2019 ◽  
Vol 141 (6) ◽  
pp. 2508-2515 ◽  
Author(s):  
Yuting Xiao ◽  
Guohui Tian ◽  
Wei Li ◽  
Ying Xie ◽  
Baojiang Jiang ◽  
...  
Keyword(s):  
Self Assembly ◽  
Carbon Nitride ◽  
Photoredox Catalysis ◽  
Highly Efficient

Micro-scale hollow nanosphere as highly efficient ORR electrocatalyst derived from the self-assembly of triblock copolymer (L64)

Ionics ◽  
2021 ◽  
Vol 27 (4) ◽  
pp. 1611-1618
Author(s):  
Xiaowen Ge ◽  
Xiaomei Du ◽  
Yin Sun ◽  
Junjie Zhang ◽  
Zhongyu Qiu ◽  
...  
Keyword(s):  
Self Assembly ◽  
Triblock Copolymer ◽  
The Self ◽  
Hollow Nanosphere ◽  
Micro Scale ◽  
Highly Efficient

Photoinduced Self‐Assembly of Carbon Nitride Quantum Dots

2021 ◽  
Author(s):  
Zheng Xing ◽  
Kaituo Dong ◽  
Nick G Pavlopoulos ◽  
Yuexing Chen ◽  
Lilac Amirav
Keyword(s):  
Quantum Dots ◽  
Self Assembly ◽  
Carbon Nitride

scholarly journals Carbon nitride nanotubes with in situ grafted hydroxyl groups for highly efficient spontaneous H2O2 production

2021 ◽  
Vol 288 ◽  
pp. 119993
Author(s):  
Liang Zhou ◽  
Juying Lei ◽  
Fuchen Wang ◽  
Lingzhi Wang ◽  
Michael R. Hoffmann ◽  
...  
Keyword(s):  
Carbon Nitride ◽  
H2o2 Production ◽  
Hydroxyl Groups ◽  
Highly Efficient

scholarly journals Band Engineering and Morphology Control of Oxygen-Incorporated Graphitic Carbon Nitride Porous Nanosheets for Highly Efficient Photocatalytic Hydrogen Evolution

2021 ◽  
Vol 13 (1) ◽  
Author(s):  
Yunyan Wu ◽  
Pan Xiong ◽  
Jianchun Wu ◽  
Zengliang Huang ◽  
Jingwen Sun ◽  
...  
Keyword(s):  
Surface Area ◽  
Hydrogen Evolution ◽  
Carbon Nitride ◽  
Separation Efficiency ◽  
Physical Adsorption ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
Photocatalytic Hydrogen Evolution ◽  
Band Engineering ◽  
Highly Efficient

AbstractGraphitic carbon nitride (g-C3N4)-based photocatalysts have shown great potential in the splitting of water. However, the intrinsic drawbacks of g-C3N4, such as low surface area, poor diffusion, and charge separation efficiency, remain as the bottleneck to achieve highly efficient hydrogen evolution. Here, a hollow oxygen-incorporated g-C3N4 nanosheet (OCN) with an improved surface area of 148.5 m2 g−1 is fabricated by the multiple thermal treatments under the N2/O2 atmosphere, wherein the C–O bonds are formed through two ways of physical adsorption and doping. The physical characterization and theoretical calculation indicate that the O-adsorption can promote the generation of defects, leading to the formation of hollow morphology, while the O-doping results in reduced band gap of g-C3N4. The optimized OCN shows an excellent photocatalytic hydrogen evolution activity of 3519.6 μmol g−1 h−1 for ~ 20 h, which is over four times higher than that of g-C3N4 (850.1 μmol g−1 h−1) and outperforms most of the reported g-C3N4 catalysts.

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