Fast Photodriven Electron Spin Coherence Transfer: A Quantum Gate Based on a Spin Exchange J-Jump

2012 ◽  
Vol 134 (30) ◽  
pp. 12430-12433 ◽  
Author(s):  
Lukáš Kobr ◽  
Daniel M. Gardner ◽  
Amanda L. Smeigh ◽  
Scott M. Dyar ◽  
Steven D. Karlen ◽  
...  
2015 ◽  
Vol 3 (30) ◽  
pp. 7962-7967 ◽  
Author(s):  
Matthew D. Krzyaniak ◽  
Lukáš Kobr ◽  
Brandon K. Rugg ◽  
Brian T. Phelan ◽  
Eric A. Margulies ◽  
...  

A covalently-linked electron donor–acceptor–acceptor molecule was utilized to study the effect of electron-nuclear hyperfine coupling on the dephasing of the zero quantum coherence in spin correlated radical pairs.


1986 ◽  
Vol 51 (11) ◽  
pp. 2433-2436 ◽  
Author(s):  
Hamza A. Hussain ◽  
Waleed A. A. Kuder

The rate of electron spin exchange in aqueous solution of potassium nitrosodisulphonate K2(SO3)2NO, has been investigated by ESR and found to depend on the dielectric constant of the medium. This observation lead to the calculation of the collision diameter 2 nm which corresponds to bimolecular collisions between species carrying two nagative charges.


2007 ◽  
Vol 75 (20) ◽  
Author(s):  
Wenxian Zhang ◽  
V. V. Dobrovitski ◽  
Lea F. Santos ◽  
Lorenza Viola ◽  
B. N. Harmon

1989 ◽  
Vol 39 (8) ◽  
pp. 3871-3883 ◽  
Author(s):  
Masayoshi Senba ◽  
Donald G. Fleming ◽  
Donald J. Arseneau ◽  
David M. Garner ◽  
Ivan D. Reid

2011 ◽  
Vol 84 (15) ◽  
Author(s):  
M. Syperek ◽  
D. R. Yakovlev ◽  
I. A. Yugova ◽  
J. Misiewicz ◽  
I. V. Sedova ◽  
...  

2010 ◽  
Vol 105 (6) ◽  
Author(s):  
Richard E. George ◽  
Wayne Witzel ◽  
H. Riemann ◽  
N. V. Abrosimov ◽  
N. Nötzel ◽  
...  

2018 ◽  
Vol 52 (4) ◽  
pp. 548-550
Author(s):  
D. R. Yakovlev ◽  
D. H. Feng ◽  
V. V. Pavlov ◽  
A. V. Rodina ◽  
E. V. Shornikova ◽  
...  

1967 ◽  
Vol 22 (6) ◽  
pp. 914-928 ◽  
Author(s):  
D. Stehlik ◽  
K. H. Hausser

In all dynamic nuclear polarisation (DNP) experiments in liquids carried out so far the electronic spin belonged to the paramagnetic molecule while the proton was part of the diamagnetic solvent molecule. In this paper the relaxation and DNP of protons inside free radicals in protonfree solvents is studied.A calculation of the DNP coupling parameter ξ is given for mixed scalar and dipolar intramolecular interaction with simultaneous time dependences by electron spin relaxation, electron spin exchange and molecular motion on the basis of the formalism of ABRAGAM and SOLOMON.Experimental results at 12.5 kGauß were obtained for the t-butyl-protons in the three radicals tri-t-butyl-phenoxyl (TBP), COPPINGER'S Radical (CR) or Galvinoxyl and di-t-butyl-nitroxide (DBNO). The experimental technique differs from the usual NMR-detection in the use of pulse technique and of a dielectric resonator in the microwave equipment.DNP enhancements from high positive to high negative values could be observed corresponding to mixed proton-electron-coupling from dominantly scalar to dominantly dipolar interaction. All results can be at least qualitatively explained by the theory of the intramolecular interaction since the essential parameters and constants of the interaction can be measured with other independent methods.


Sign in / Sign up

Export Citation Format

Share Document