Radical cations of hexamethylprismane: ab initio calculations and nuclear spin polarization results

1989 ◽  
Vol 111 (18) ◽  
pp. 7132-7136 ◽  
Author(s):  
Krishnan Raghavachari ◽  
Heinz D. Roth
Author(s):  
M. M. Glazov

The transfer of nonequilibrium spin polarization between the electron and nuclear subsystems is studied in detail. Usually, a thermal orientation of nuclei in magnetic field is negligible due to their small magnetic moments, but if electron spins are optically oriented, efficient nuclear spin polarization can occur. The microscopic approach to the dynamical nuclear polarization effect based on the kinetic equation method, along with a phenomenological but very powerful description of dynamical nuclear polarization in terms of the nuclear spin temperature concept is given. In this way, one can account for the interaction between neighbouring nuclei without solving a complex many-body problem. The hyperfine interaction also induces the feedback of polarized nuclei on the electron spin system giving rise to a number of nonlinear effects: bistability of nuclear spin polarization and anomalous Hanle effect, dragging and locking of optical resonances in quantum dots. Theory is illustrated by experimental data on dynamical nuclear polarization.


2016 ◽  
Vol 93 (8) ◽  
Author(s):  
F. Heisterkamp ◽  
E. Kirstein ◽  
A. Greilich ◽  
E. A. Zhukov ◽  
T. Kazimierczuk ◽  
...  

2006 ◽  
Vol 965 ◽  
Author(s):  
Helder Sousa Domingos

ABSTRACTClassical and ab-initio calculations were carried out on bulk defects and surfaces of the carbon allotrope Fcc-C22. The results revealed a number of possible defects with spin polarization and one with antiferromagnetic character. The surfaces were shown to be able to host magnetic polarization. Extrinsic light dopants (H and N) were shown to introduce spin polarization for small dopant concentration and to metallize the systems for large concentrations.


1982 ◽  
Vol 104 (22) ◽  
pp. 5878-5883 ◽  
Author(s):  
Richard S. Hutton ◽  
Heinz D. Roth ◽  
Marcia L. Manion Schilling ◽  
Anthony M. Trozzolo ◽  
Thomas M. Leslie

2014 ◽  
Vol 31 (10) ◽  
pp. 2278 ◽  
Author(s):  
Sung Jong Park ◽  
Taeksu Shin ◽  
Ju Hahn Lee ◽  
Gi Dong Kim ◽  
Yong Kyun Kim

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