Enhanced Charge Transport in Two-Dimensional Materials through Light–Matter Strong Coupling

ACS Nano ◽  
2021 ◽  
Author(s):  
Pooja Bhatt ◽  
Kuljeet Kaur ◽  
Jino George
2020 ◽  
Vol 4 (1) ◽  
pp. 9
Author(s):  
Vasilios Karanikolas ◽  
Ioannis Thanopulos ◽  
Emmanuel Paspalakis

Two-dimensional materials allow for extreme light confinement, thus becoming important candidates for all optical application platforms.  [...]


2022 ◽  
Author(s):  
Ye Ming Qing ◽  
Yongze Ren ◽  
Dangyuan Lei ◽  
Hui Feng Ma ◽  
Tie Jun Cui

Abstract Strong interaction between electromagnetic radiation and matter leads to the formation of hybrid light-matter states, making the absorption and emission behavior different from those of the uncoupled states. Strong coupling effect results in the famous Rabi splitting and the emergence of new polaritonic eigenmodes, exhibiting spectral anticrossing behavior and unique energy-transfer properties. In recent years, there has been a rapidly increasing number of works focusing on strong coupling between nanostructures and two-dimensional materials (2DMs), because of the exceptional properties and applications they demonstrate. Here, we review the significant recent advances and important developments of strong light-matter interactions in 2DMs-based nanostructures. We adopt the coupled oscillator model to describe the strong coupling and give an overview of various hybrid nanostructures to realize this regime, including graphene-based nanostructures, black phosphorus-based nanostructures, transition-metal dichalcogenides-based nanostructures, etc. In addition, we discuss potential applications that can benefit from these effects and conclude our review with a perspective on the future of this rapidly emerging field.


2021 ◽  
Vol 4 (12) ◽  
pp. 893-905
Author(s):  
Erik Piatti ◽  
Adrees Arbab ◽  
Francesco Galanti ◽  
Tian Carey ◽  
Luca Anzi ◽  
...  

RSC Advances ◽  
2015 ◽  
Vol 5 (15) ◽  
pp. 11392-11396 ◽  
Author(s):  
Yuewen Mu ◽  
Feng Ding ◽  
Haigang Lu

The Dirac point and cones make some two-dimensional materials (e.g., graphene, silicone and graphyne) exhibit ballistic charge transport and enormously high carrier mobilities.


2019 ◽  
Author(s):  
Simil Thomas ◽  
Hong Li ◽  
Raghunath R. Dasari ◽  
Austin Evans ◽  
William Dichtel ◽  
...  

<p>We have considered three two-dimensional (2D) π-conjugated polymer networks (i.e., covalent organic frameworks, COFs) materials based on pyrene, porphyrin, and zinc-porphyrin cores connected <i>via</i> diacetylenic linkers. Their electronic structures, investigated at the density functional theory global-hybrid level, are indicative of valence and conduction bands that have large widths, ranging between 1 and 2 eV. Using a molecular approach to derive the electronic couplings between adjacent core units and the electron-vibration couplings, the three π-conjugated 2D COFs are predicted to have ambipolar charge-transport characteristics with electron and hole mobilities in the range of 65-95 cm<sup>2</sup>V<sup>-1</sup>s<sup>-1</sup>. Such predicted values rank these 2D COFs among the highest-mobility organic semiconductors. In addition, we have synthesized the zinc-porphyrin based 2D COF and carried out structural characterization via powder X-ray diffraction and surface area analysis, which demonstrates the feasability of these electroactive networks.</p>


2018 ◽  
Author(s):  
Penny Perlepe ◽  
Rodolphe Clérac ◽  
Itziar Oyarzabal ◽  
Corine Mathonière

Sign in / Sign up

Export Citation Format

Share Document