scholarly journals Insight into the Nature of Iron Sulfide Surfaces During the Electrochemical Hydrogen Evolution and CO2 Reduction Reactions

2018 ◽  
Vol 10 (38) ◽  
pp. 32078-32085 ◽  
Author(s):  
Siti N. A. Zakaria ◽  
Nathan Hollingsworth ◽  
Husn U. Islam ◽  
Anna Roffey ◽  
David Santos-Carballal ◽  
...  
2016 ◽  
Vol 120 (29) ◽  
pp. 16200-16210 ◽  
Author(s):  
Takuya Masuda ◽  
Yu Sun ◽  
Hitoshi Fukumitsu ◽  
Hiromitsu Uehara ◽  
Satoru Takakusagi ◽  
...  

Nano Energy ◽  
2016 ◽  
Vol 29 ◽  
pp. 4-28 ◽  
Author(s):  
Juan Herranz ◽  
Julien Durst ◽  
Emiliana Fabbri ◽  
Alexandra Patru ◽  
Xi Cheng ◽  
...  

Nanoscale ◽  
2020 ◽  
Vol 12 (39) ◽  
pp. 20413-20424
Author(s):  
Riming Hu ◽  
Yongcheng Li ◽  
Fuhe Wang ◽  
Jiaxiang Shang

Bilayer single atom catalysts can serve as promising multifunctional electrocatalysts for the HER, ORR, and OER.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Jeremy L. Hitt ◽  
Yuguang C. Li ◽  
Songsheng Tao ◽  
Zhifei Yan ◽  
Yue Gao ◽  
...  

AbstractIn the problem of electrochemical CO2 reduction, the discovery of earth-abundant, efficient, and selective catalysts is essential to enabling technology that can contribute to a carbon-neutral energy cycle. In this study, we adapt an optical high throughput screening method to study multi-metallic catalysts for CO2 electroreduction. We demonstrate the utility of the method by constructing catalytic activity maps of different alloyed elements and use X-ray scattering analysis by the atomic pair distribution function (PDF) method to gain insight into the structures of the most active compositions. Among combinations of four elements (Au, Ag, Cu, Zn), Au6Ag2Cu2 and Au4Zn3Cu3 were identified as the most active compositions in their respective ternaries. These ternary electrocatalysts were more active than any binary combination, and a ca. 5-fold increase in current density at potentials of −0.4 to −0.8 V vs. RHE was obtained for the best ternary catalysts relative to Au prepared by the same method. Tafel plots of electrochemical data for CO2 reduction and hydrogen evolution indicate that the ternary catalysts, despite their higher surface area, are poorer catalysts for the hydrogen evolution reaction than pure Au. This results in high Faradaic efficiency for CO2 reduction to CO.


Nano Research ◽  
2021 ◽  
Author(s):  
Qikang Wu ◽  
Songrui Wang ◽  
Jiahui Guo ◽  
Xueqing Feng ◽  
Han Li ◽  
...  

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