Dual-Functional Starfish-like P-Doped Co–Ni–S Nanosheets Supported on Nickel Foams with Enhanced Electrochemical Performance and Excellent Stability for Overall Water Splitting

2018 ◽  
Vol 10 (8) ◽  
pp. 7087-7095 ◽  
Author(s):  
Fangfang Zhang ◽  
Yuancai Ge ◽  
Hang Chu ◽  
Pei Dong ◽  
Robert Baines ◽  
...  
2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Xixi Ji ◽  
Yanhong Lin ◽  
Jie Zeng ◽  
Zhonghua Ren ◽  
Zijia Lin ◽  
...  

AbstractDevelopment of excellent and cheap electrocatalysts for water electrolysis is of great significance for application of hydrogen energy. Here, we show a highly efficient and stable oxygen evolution reaction (OER) catalyst with multilayer-stacked hybrid structure, in which vertical graphene nanosheets (VGSs), MoS2 nanosheets, and layered FeCoNi hydroxides (FeCoNi(OH)x) are successively grown on carbon fibers (CF/VGSs/MoS2/FeCoNi(OH)x). The catalyst exhibits excellent OER performance with a low overpotential of 225 and 241 mV to attain 500 and 1000 mA cm−2 and small Tafel slope of 29.2 mV dec−1. Theoretical calculation indicates that compositing of FeCoNi(OH)x with MoS2 could generate favorable electronic structure and decrease the OER overpotential, promoting the electrocatalytic activity. An alkaline water electrolyzer is established using CF/VGSs/MoS2/FeCoNi(OH)x anode for overall water splitting, which generates a current density of 100 mA cm−2 at 1.59 V with excellent stability over 100 h. Our highly efficient catalysts have great prospect for water electrolysis.


2019 ◽  
Vol 7 (3) ◽  
pp. 1083-1091 ◽  
Author(s):  
Lina Liu ◽  
Feng Yan ◽  
Kaiyue Li ◽  
Chunling Zhu ◽  
Ying Xie ◽  
...  

Ultrasmall FeNi3N particles with an exposed active (110) surface anchored on nitrogen-doped graphene as multifunctional electrocatalysts for both overall water splitting and Zn–air batteries exhibited excellent electrochemical performance.


Nanoscale ◽  
2017 ◽  
Vol 9 (13) ◽  
pp. 4409-4418 ◽  
Author(s):  
Jinlong Zheng ◽  
Wei Zhou ◽  
Tong Liu ◽  
Shijie Liu ◽  
Chengbo Wang ◽  
...  

Nanoscale ◽  
2018 ◽  
Vol 10 (45) ◽  
pp. 21019-21024 ◽  
Author(s):  
Liyong Chen ◽  
Yingyue Zhang ◽  
Huifang Wang ◽  
Yanxin Wang ◽  
Dezhi Li ◽  
...  

Cobalt layered double hydroxides (Co-LDHs) obtained by an imidazole-assisted route were used as precursors to prepare dual-functional electrocatalysts CoP/Co2P for water splitting.


Author(s):  
Shuting Wen ◽  
Guangliang Chen ◽  
Wei Chen ◽  
Mengchao Li ◽  
Bo Ouyang ◽  
...  

Nanostructured trimetallic phosphide electrocatalysts are promising for H2 and O2 evolution reactions (HER/OER) that are actively pursued nowadays to achieve commercial hydrogen production. Herein, a dual-functional Nb-doped NiFe phosphide nanosheet...


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