MoS2 Quantum Dots with a Tunable Work Function for High-Performance Organic Solar Cells

2016 ◽  
Vol 8 (40) ◽  
pp. 26916-26923 ◽  
Author(s):  
Wang Xing ◽  
Yusheng Chen ◽  
Xinlong Wang ◽  
Lei Lv ◽  
Xinhua Ouyang ◽  
...  
2021 ◽  
Vol 13 (1) ◽  
Author(s):  
Juanyong Wan ◽  
Yonggao Xia ◽  
Junfeng Fang ◽  
Zhiguo Zhang ◽  
Bingang Xu ◽  
...  

AbstractNonfullerene organic solar cells (OSCs) have achieved breakthrough with pushing the efficiency exceeding 17%. While this shed light on OSC commercialization, high-performance flexible OSCs should be pursued through solution manufacturing. Herein, we report a solution-processed flexible OSC based on a transparent conducting PEDOT:PSS anode doped with trifluoromethanesulfonic acid (CF3SO3H). Through a low-concentration and low-temperature CF3SO3H doping, the conducting polymer anodes exhibited a main sheet resistance of 35 Ω sq−1 (minimum value: 32 Ω sq−1), a raised work function (≈ 5.0 eV), a superior wettability, and a high electrical stability. The high work function minimized the energy level mismatch among the anodes, hole-transporting layers and electron-donors of the active layers, thereby leading to an enhanced carrier extraction. The solution-processed flexible OSCs yielded a record-high efficiency of 16.41% (maximum value: 16.61%). Besides, the flexible OSCs afforded the 1000 cyclic bending tests at the radius of 1.5 mm and the long-time thermal treatments at 85 °C, demonstrating a high flexibility and a good thermal stability.


Solar RRL ◽  
2021 ◽  
Author(s):  
Weiqiang Miao ◽  
Chuanhang Guo ◽  
Donghui Li ◽  
Teng Li ◽  
Pang Wang ◽  
...  

2013 ◽  
Vol 15 (43) ◽  
pp. 18973 ◽  
Author(s):  
Miaomiao Li ◽  
Wang Ni ◽  
Bin Kan ◽  
Xiangjian Wan ◽  
Long Zhang ◽  
...  

Nanomaterials ◽  
2021 ◽  
Vol 11 (6) ◽  
pp. 1464
Author(s):  
Kwang Hyun Park ◽  
Sunggyeong Jung ◽  
Jungmo Kim ◽  
Byoung-Min Ko ◽  
Wang-Geun Shim ◽  
...  

The design of photoactive materials and interface engineering between organic/inorganic layers play a critical role in achieving enhanced performance in energy-harvesting devices. Two-dimensional transitional dichalcogenides (TMDs) with excellent optical and electronic properties are promising candidates in this regard. In this study, we demonstrate the fabrication of size-controlled MoS2 quantum dots (QDs) and present fundamental studies of their optical properties and their application as a hole-transport layer (HTL) in organic solar cells (OSCs). Optical and structural analyses reveal that the as-prepared MoS2 QDs show a fluorescence mechanism with respect to the quantum confinement effect and intrinsic/extrinsic states. Moreover, when incorporated into a photovoltaic device, the MoS2 QDs exhibit a significantly enhanced performance (5/10-nanometer QDs: 8.30%/7.80% for PTB7 and 10.40%/10.17% for PTB7-Th, respectively) compared to those of the reference device (7.24% for PTB7 and 9.49% for PTB7-Th). We confirm that the MoS2 QDs clearly offer enhanced transport characteristics ascribed to higher hole-mobility and smoother root mean square (Rq) as a hole-extraction material. This approach can enable significant advances and facilitate a new avenue for realizing high-performance optoelectronic devices.


2021 ◽  
Author(s):  
Tingting Zhang ◽  
Qiu Zhang ◽  
Yumeng Wang ◽  
Fengyan Li ◽  
Lin Xu

The preparation of low cost H3PW12O40 (PW12)/CoS2 complex is used as a counter electrode (CE) to combine with sandwich quantum dots sensitized cells (QDSSCs) composed of TiO2/CdS/CdSe/ZnS photoanode and polysulfide...


2019 ◽  
Vol 12 (11) ◽  
pp. 3400-3411 ◽  
Author(s):  
Fei Pan ◽  
Chenkai Sun ◽  
Yingfen Li ◽  
Dianyong Tang ◽  
Yingping Zou ◽  
...  

Solution-processable n-doped graphene-containing cathode interfacial material with a low work function demonstrates 16.52% power conversion efficiency in organic solar cells.


2021 ◽  
pp. 129768
Author(s):  
Dou Luo ◽  
Xue Lai ◽  
Nan Zheng ◽  
Chenghao Duan ◽  
Zhaojin Wang ◽  
...  

2021 ◽  
Vol 60 (16) ◽  
pp. 8813-8817
Author(s):  
Shuting Pang ◽  
Zhiqiang Wang ◽  
Xiyue Yuan ◽  
Langheng Pan ◽  
Wanyuan Deng ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Zhenrong Jia ◽  
Shucheng Qin ◽  
Lei Meng ◽  
Qing Ma ◽  
Indunil Angunawela ◽  
...  

AbstractTandem organic solar cells are based on the device structure monolithically connecting two solar cells to broaden overall absorption spectrum and utilize the photon energy more efficiently. Herein, we demonstrate a simple strategy of inserting a double bond between the central core and end groups of the small molecule acceptor Y6 to extend its conjugation length and absorption range. As a result, a new narrow bandgap acceptor BTPV-4F was synthesized with an optical bandgap of 1.21 eV. The single-junction devices based on BTPV-4F as acceptor achieved a power conversion efficiency of over 13.4% with a high short-circuit current density of 28.9 mA cm−2. With adopting BTPV-4F as the rear cell acceptor material, the resulting tandem devices reached a high power conversion efficiency of over 16.4% with good photostability. The results indicate that BTPV-4F is an efficient infrared-absorbing narrow bandgap acceptor and has great potential to be applied into tandem organic solar cells.


Sign in / Sign up

Export Citation Format

Share Document