scholarly journals Local Energy Landscape Drives Long-Range Exciton Diffusion in Two-Dimensional Halide Perovskite Semiconductors

2021 ◽  
Vol 12 (16) ◽  
pp. 4003-4011
Author(s):  
Alan Baldwin ◽  
Géraud Delport ◽  
Kai Leng ◽  
Rosemonde Chahbazian ◽  
Krzysztof Galkowski ◽  
...  
ACS Nano ◽  
2020 ◽  
Vol 14 (6) ◽  
pp. 6999-7007 ◽  
Author(s):  
Erika Penzo ◽  
Anna Loiudice ◽  
Edward S. Barnard ◽  
Nicholas J. Borys ◽  
Matthew J. Jurow ◽  
...  

eLight ◽  
2021 ◽  
Vol 1 (1) ◽  
Author(s):  
Pengfei Qi ◽  
Yang Luo ◽  
Beibei Shi ◽  
Wei Li ◽  
Donglin Liu ◽  
...  

AbstractTwo dimensional excitonic devices are of great potential to overcome the dilemma of response time and integration in current generation of electron or/and photon based systems. The ultrashort diffusion length of exciton arising from ultrafast relaxation and low carrier mobility greatly discounts the performance of excitonic devices. Phonon scattering and exciton localization are crucial to understand the modulation of exciton flux in two dimensional disorder energy landscape, which still remain elusive. Here, we report an optimized scheme for exciton diffusion and relaxation dominated by phonon scattering and disorder potentials in WSe2 monolayers. The effective diffusion coefficient is enhanced by > 200% at 280 K. The excitons tend to be localized by disorder potentials accompanied by the steadily weakening of phonon scattering when temperature drops to 260 K, and the onset of exciton localization brings forward as decreasing temperature. These findings identify that phonon scattering and disorder potentials are of great importance for long-range exciton diffusion and thermal management in exciton based systems, and lay a firm foundation for the development of functional excitonic devices.


2021 ◽  
Author(s):  
Stav Rahmany ◽  
Lioz Etgar

Much effort has been made to push the power conversion efficiency of perovskite solar cells (PSCs) towards the theoretical limit. Recent studies have shown that post deposition treatment of barrier...


2021 ◽  
Author(s):  
Arindam Mondal ◽  
Akash Lata ◽  
Aarya Prabhakaran ◽  
Satyajit Gupta

Application of three-dimensional (3D)-halide perovskites (HaP) in photocatalysis encourages the new exercise with two-dimensional (2D) HaP based thin-films for photocatalytic degradation of dye. The reduced dimensionality to 2D-HaPs, with a...


APL Materials ◽  
2021 ◽  
Vol 9 (2) ◽  
pp. 020906
Author(s):  
Tao Zhang ◽  
Qiang Sun ◽  
Xiaoli Zhang ◽  
Yan Shen ◽  
Mingkui Wang

2021 ◽  
Vol 27 (S1) ◽  
pp. 952-954
Author(s):  
Suk Hyun Sung ◽  
Yin Min Goh ◽  
Noah Schnitzer ◽  
Ismail El Baggari ◽  
Kai Sun ◽  
...  

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