Size Dependence of Excitation-Energy-Related Surface Trapping Dynamics in PbS Quantum Dots

2015 ◽  
Vol 119 (13) ◽  
pp. 7517-7524 ◽  
Author(s):  
Heejae Chung ◽  
Hyekyoung Choi ◽  
Dongho Kim ◽  
Sohee Jeong ◽  
Jiwon Kim
2011 ◽  
Vol 83 (15) ◽  
Author(s):  
Gero Nootz ◽  
Lazaro A. Padilha ◽  
Larissa Levina ◽  
Vlad Sukhovatkin ◽  
Scott Webster ◽  
...  

2004 ◽  
Vol 35 (8) ◽  
pp. 629-633 ◽  
Author(s):  
K Kang ◽  
K Daneshvar ◽  
R Tsu

Nanoscale ◽  
2017 ◽  
Vol 9 (40) ◽  
pp. 15566-15575 ◽  
Author(s):  
Mahfoudh Raissi ◽  
Muhammad T. Sajjad ◽  
Yann Pellegrin ◽  
Thomas Jean Roland ◽  
Stéphane Jobic ◽  
...  

A low driving force (−0.3 eV) is sufficient for PbS quantum dots to inject holes into NiO, and the excitons in PbS decay by both reductive and oxidative quenching.


Photonics ◽  
2020 ◽  
Vol 7 (2) ◽  
pp. 39
Author(s):  
Ivan D. Skurlov ◽  
Evgeniia A. Ponomareva ◽  
Azat O. Ismagilov ◽  
Sergey E. Putilin ◽  
Ilia A. Vovk ◽  
...  

Due to their high resonant third-order nonlinear response, lead sulfide quantum dots (QDs) are potential materials for applications in the field of nonlinear optics. In this paper, we implement the Z-scan method to study the resonant nonlinear response of lead sulfide QDs in colloidal solutions. We managed to measure the purely intrinsic resonant nonlinear response, free of thermal contribution. We report that the lead sulfide QD third-order nonlinear response per QD shows an unconventional increase. A figure of merit for QD nonlinearity grows as a power function with a factor of 2.9.


2020 ◽  
Author(s):  
Iván Mora-Seró ◽  
Sofia Masi ◽  
David Macias-Pinilla ◽  
Carlos Echeverría-Arrondo ◽  
Juan Ignacio Climente

2020 ◽  
Vol 10 (1) ◽  
Author(s):  
Tamara Sloboda ◽  
Sebastian Svanström ◽  
Fredrik O. L. Johansson ◽  
Aneta Andruszkiewicz ◽  
Xiaoliang Zhang ◽  
...  

AbstractTime-resolved photoelectron spectroscopy can give insights into carrier dynamics and offers the possibility of element and site-specific information through the measurements of core levels. In this paper, we demonstrate that this method can access electrons dynamics in PbS quantum dots over a wide time window spanning from pico- to microseconds in a single experiment carried out at the synchrotron facility BESSY II. The method is sensitive to small changes in core level positions. Fast measurements at low pump fluences are enabled by the use of a pump laser at a lower repetition frequency than the repetition frequency of the X-ray pulses used to probe the core level electrons: Through the use of a time-resolved spectrometer, time-dependent analysis of data from all synchrotron pulses is possible. Furthermore, by picosecond control of the pump laser arrival at the sample relative to the X-ray pulses, a time-resolution limited only by the length of the X-ray pulses is achieved. Using this method, we studied the charge dynamics in thin film samples of PbS quantum dots on n-type MgZnO substrates through time-resolved measurements of the Pb 5d core level. We found a time-resolved core level shift, which we could assign to electron injection and charge accumulation at the MgZnO/PbS quantum dots interface. This assignment was confirmed through the measurement of PbS films with different thicknesses. Our results therefore give insight into the magnitude of the photovoltage generated specifically at the MgZnO/PbS interface and into the timescale of charge transport and electron injection, as well as into the timescale of charge recombination at this interface. It is a unique feature of our method that the timescale of both these processes can be accessed in a single experiment and investigated for a specific interface.


2021 ◽  
Vol 546 ◽  
pp. 149086
Author(s):  
Xiangping Pan ◽  
Yanhua Dong ◽  
Ming Jia ◽  
Jianxiang Wen ◽  
Caiyun Su ◽  
...  

2021 ◽  
pp. 1-1
Author(s):  
Aigerim Tankimanova ◽  
Chun Hong Kang ◽  
Omar Alkhazragi ◽  
Haodong Tang ◽  
Meiwei Kong ◽  
...  

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