It’s a Gas: Oxidative Dehydrogenation of Propane over Boron Nitride Catalysts

2021 ◽  
Vol 125 (10) ◽  
pp. 5623-5634
Author(s):  
Peter Kraus ◽  
Rune Peter Lindstedt
Keyword(s):  
Boron Nitride ◽  
Oxidative Dehydrogenation ◽  
Oxidative Dehydrogenation Of Propane

Nonmetal oxygen vacancies confined under boron nitride for enhanced oxidative dehydrogenation of propane to propene

2021 ◽  
Vol 537 ◽  
pp. 147927
Author(s):  
Qiuwen Liu ◽  
Cheng Chen ◽  
Qiang Liu ◽  
Yawei Wu ◽  
Fangshu Xing ◽  
...  
Keyword(s):  
Boron Nitride ◽  
Oxidative Dehydrogenation ◽  
Oxygen Vacancies ◽  
Oxidative Dehydrogenation Of Propane

scholarly journals It's a Gas: Oxidative Dehydrogenation of Propane over Boron Nitride Catalysts

2020 ◽  
Author(s):  
Peter Kraus ◽  
R. Peter Lindstedt
Keyword(s):  
Low Temperature ◽  
Boron Nitride ◽  
Gas Phase ◽  
Oxidative Dehydrogenation ◽  
Hexagonal Boron Nitride ◽  
Combustion Model ◽  
Low Temperature Combustion ◽  
Oxidative Dehydrogenation Of Propane ◽  
Temperature Combustion

We investigate the role of gas-phase phenomena in the heterogeneous oxidative dehydrogenation of propane over hexagonal boron nitride. We apply a recently developed gas-phase combustion model for low-temperature combustion of propane and couple it with several surface microkinetic mechanisms to probe the selectivity limits using the open-source flame solver Cantera. We show that while the conversion of propane is surface-driven, the selectivities are significantly influenced by the gas-phase, especially when dilute catalyst beds are used.<br>

scholarly journals Edge-hydroxylated Boron Nitride for Oxidative Dehydrogenation of Propane to Propylene

ChemCatChem ◽  
2017 ◽  
Vol 9 (10) ◽  
pp. 1720-1720 ◽  
Author(s):  
Lei Shi ◽  
Dongqi Wang ◽  
Wei Song ◽  
Dan Shao ◽  
Wei-Ping Zhang ◽  
...  
Keyword(s):  
Boron Nitride ◽  
Oxidative Dehydrogenation ◽  
Oxidative Dehydrogenation Of Propane

O2 Activation and Oxidative Dehydrogenation of Propane on Hexagonal Boron Nitride: Mechanism Revisited

2019 ◽  
Vol 123 (4) ◽  
pp. 2256-2266 ◽  
Author(s):  
Hongping Li ◽  
Jinrui Zhang ◽  
Peiwen Wu ◽  
Suhang Xun ◽  
Wei Jiang ◽  
...  
Keyword(s):  
Boron Nitride ◽  
Oxidative Dehydrogenation ◽  
Hexagonal Boron Nitride ◽  
Oxidative Dehydrogenation Of Propane ◽  
O2 Activation

scholarly journals It's a Gas: Oxidative Dehydrogenation of Propane over Boron Nitride Catalysts

2021 ◽  
Author(s):  
Peter Kraus ◽  
R. Peter Lindstedt
Keyword(s):  
Low Temperature ◽  
Boron Nitride ◽  
Gas Phase ◽  
Oxidative Dehydrogenation ◽  
Hexagonal Boron Nitride ◽  
Combustion Model ◽  
Low Temperature Combustion ◽  
Oxidative Dehydrogenation Of Propane ◽  
Temperature Combustion

We investigate the role of gas-phase phenomena in the heterogeneous oxidative dehydrogenation of propane over hexagonal boron nitride. We apply a recently developed gas-phase combustion model for low-temperature combustion of propane and couple it with several surface microkinetic mechanisms to probe the selectivity limits using the open-source flame solver Cantera. We show that while the conversion of propane is surface-driven, the selectivities are significantly influenced by the gas-phase, especially when dilute catalyst beds are used.<br>

scholarly journals Oxidative dehydrogenation of propane on the oxygen adsorbed edges of boron nitride nanoribbons

2020 ◽  
Vol 10 (15) ◽  
pp. 5181-5195
Author(s):  
Biplab Rajbanshi ◽  
Supriya Saha ◽  
Charles Fricke ◽  
Salai Cheettu Ammal ◽  
Andreas Heyden
Keyword(s):  
Boron Nitride ◽  
Oxidative Dehydrogenation ◽  
Active Site ◽  
Oxidative Dehydrogenation Of Propane ◽  
Type Site ◽  
Boron Nitride Nanoribbons

A N2O/NOx-type site on the boron nitride nanoribbon edge is proposed as highly selective, active site for the oxidative dehydrogenation of propane.

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