Widened Active Temperature Window of a Fe-ZSM-5 Catalyst by an Impregnation Solvent for NH3-SCR of NO

2018 ◽  
Vol 57 (41) ◽  
pp. 13703-13712 ◽  
Author(s):  
Jin Shi ◽  
Yi Zhang ◽  
Zeyun Fan ◽  
Mingxia Chen ◽  
Zhixiang Zhang ◽  
...  
RSC Advances ◽  
2015 ◽  
Vol 5 (10) ◽  
pp. 7597-7603 ◽  
Author(s):  
Yuesong Shen ◽  
Yun Su ◽  
Yifan Ma

The maximum activity is dependent on the number of Lewis acid sites, and the active temperature window is dependent on the acid strength.


RSC Advances ◽  
2019 ◽  
Vol 9 (52) ◽  
pp. 30340-30349 ◽  
Author(s):  
Lvesheng Sun ◽  
Shunxin Cao ◽  
Yun Huang ◽  
Yiming Zhang ◽  
Youhong Xiao ◽  
...  

VOX/TiO2–Ce0.9Zr0.1O2 catalyst exhibits high activity and selectivity in a wide temperature window.


Vacuum ◽  
2021 ◽  
pp. 110384
Author(s):  
Junqiang Xu ◽  
Xianlin Zou ◽  
Guorong Chen ◽  
Yanrong Zhang ◽  
Qiang Zhang ◽  
...  

2021 ◽  
Vol 49 (1) ◽  
pp. 113-120
Author(s):  
Dong-jie YAN ◽  
Tong GUO ◽  
Ya YU ◽  
Zhao-hui CHEN

Catalysts ◽  
2021 ◽  
Vol 11 (1) ◽  
pp. 55
Author(s):  
Katarzyna Świrk ◽  
Ye Wang ◽  
Changwei Hu ◽  
Li Li ◽  
Patrick Da Costa ◽  
...  

Copper and iron promoted ZrO2 catalysts were prepared by one-pot synthesis using urea. The studied catalysts were characterized by XRD, N2 physisorption, XPS, temperature-programmed desorption of NH3 (NH3-TPD), and tested by the selective catalytic reduction by ammonia (NH3-SCR) of NO in the absence and presence of water vapor, under the experimental conditions representative of exhaust gases from stationary sources. The influence of SO2 on catalytic performance was also investigated. Among the studied catalysts, the Fe-Zr sample showed the most promising results in NH3-SCR, being active and highly selective to N2. The addition of SO2 markedly improved NO and NH3 conversions during NH3-SCR in the presence of H2O. The improvement in acidic surface properties is believed to be the cause.


2021 ◽  
Vol 9 (5) ◽  
pp. 106323
Author(s):  
Yuhan Zhou ◽  
Buxin Su ◽  
Shan Ren ◽  
Zhichao Chen ◽  
Zenghui Su ◽  
...  

2017 ◽  
Vol 43 (13-16) ◽  
pp. 1240-1246 ◽  
Author(s):  
Phornphimon Maitarad ◽  
Jin Han ◽  
Supawadee Namuangruk ◽  
Liyi Shi ◽  
Chirawat Chitpakdee ◽  
...  

2021 ◽  
Author(s):  
Nawel Jr ◽  
Thabet Makhlouf ◽  
Gerard Delahay ◽  
Hassib Tounsi

Abstract Copper loaded η-alumina catalysts with different copper contents have been prepared by impregnation/evaporation method. The catalysts were characterized by XRD, FTIR, BET, UV–vis, H2-TPR and evaluated in the selective catalytic reduction of NO by NH3 and in the selective catalytic oxidation of NH3. The characterization techniques showed that the impregnation/evaporation method permits to obtain highly dispersed copper oxide species on the η-alumina surface when low amount of copper is used (1wt. % and 2 wt.%). The wet impregnation method made it possible to reach a well dispersion of the copper species on the surface of the alumina for the low copper contents Cu(1)-Al2O3 and Cu(2)-Al2O3. The latter justifies the similar behavior of Cu(1)-Al2O3) and Cu(2)-Al2O3 in the selective catalytic oxidation of NH3 where these catalysts exhibit a conversion of NH3 to N2 of the order of 100% at T > 500°C.


Author(s):  
Jie Yang ◽  
Shan Ren ◽  
Mingming Wang ◽  
Zhicaho Chen ◽  
Lin Chen ◽  
...  

Ce–Ti catalysts were considered as promising replacement for V–Ti based catalysts for selective catalytic reduction (SCR) of nitrogen oxides (NO and NO2) with NH3. In this work, CeO2/TiO2 catalyst was...


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