Thermally Stable Amine-Grafted Adsorbent Prepared by Impregnating 3-Aminopropyltriethoxysilane on Mesoporous Silica for CO2 Capture

2016 ◽  
Vol 55 (29) ◽  
pp. 7842-7852 ◽  
Author(s):  
Dang Viet Quang ◽  
T. Alan Hatton ◽  
Mohammad R. M. Abu-Zahra
Keyword(s):  
Mesoporous Silica ◽  
Co2 Capture ◽  
Thermally Stable

Thermally stable amine-functionalized silica sorbents using one-pot synthesis method for CO2 capture at low temperature

2020 ◽  
Vol 37 (12) ◽  
pp. 2317-2325
Author(s):  
Seong Bin Jo ◽  
Ho Jin Chae ◽  
Tae Young Kim ◽  
Jeom-In Baek ◽  
Dhanusuraman Ragupathy ◽  
...  
Keyword(s):  
Low Temperature ◽  
Co2 Capture ◽  
Synthesis Method ◽  
Functionalized Silica ◽  
Thermally Stable ◽  
One Pot ◽  
One Pot Synthesis ◽  
Amine Functionalized

scholarly journals Evaluation on the Stability of Amine-Mesoporous Silica Adsorbents used for CO2 Capture

2020 ◽  
Vol 36 (1) ◽  
Author(s):  
Dang Viet Quang ◽  
Dao Van Duong ◽  
Vu Thi Hong Ha ◽  
Dao Sy Duc ◽  
Tran Thi Ngoc Dung ◽  
...  
Keyword(s):  
Mesoporous Silica ◽  
Co2 Capture ◽  
Capture Process ◽  
Silica Substrate ◽  
Humid Condition ◽  
Silica Adsorbents ◽  
Reduction Of Energy Consumption ◽  
The Stability ◽  
Co2 Adsorption Capacity ◽  
Co2 Capture Capacity

Amine-mesoporous silica has been considered as a promising CO2 adsorbent with high potential for the reduction of energy consumption and CO2 capture cost; however, its stability could greatly vary with synthetic method. In this study, adsorbents prepared by impregnating different amines including polyethylenimine (PEI) and 3-aminopropyltriethoxysilane (APTES) onto mesoporous silica were used to evaluate the effect of amines selection on the stability of adsorbents used in CO2 capture process. Results revealed that APTES impregnated mesoporous silica (APTES-MPS) is more stable than PEI-impregnated mesoporous silica (PEI-MPS); APTES-MPS was thermally decomposed at ≈280 oC, while PEI-MPS was thermally decomposed at ≈180 oC only. PEI-MPS was particularly less stable when operating under dry condition; its CO2 adsorption capacity reduced by 22.1% after 10 adsorption/regeneration cycles, however, the capacity can be significantly improved in humid condition. APTES-MPS showed a greater stability with no significant reduction in CO2 capture capacity after 10 adsorption/regeneration cycles. In general, APTES-MPS adsorbent possesses a higher stability compared to PEI-MPS thanks to the formation of chemical bonds between amino-functional groups and mesoporous silica substrate. Keywords: Mesoporous silica; CO2 capture; Adsorption; Regeneration; Emission.

CO2 capture and MWCNTs synthesis using mesoporous silica and zeolite 13X collectively prepared from bottom ash

2012 ◽  
Vol 190 (1) ◽  
pp. 15-22 ◽  
Author(s):  
Ji-Eun Park ◽  
Han-Kyol Youn ◽  
Seung-Tae Yang ◽  
Wha-Seung Ahn
Keyword(s):  
Mesoporous Silica ◽  
Co2 Capture ◽  
Bottom Ash ◽  
Zeolite 13X

One-pot synthesis of thermally stable gold@mesoporous silica core-shell nanospheres with catalytic activity

Nano Research ◽  
2013 ◽  
Vol 6 (12) ◽  
pp. 871-879 ◽  
Author(s):  
Junchen Chen ◽  
Renyuan Zhang ◽  
Lu Han ◽  
Bo Tu ◽  
Dongyuan Zhao
Keyword(s):  
Catalytic Activity ◽  
Mesoporous Silica ◽  
Core Shell ◽  
Thermally Stable ◽  
One Pot ◽  
One Pot Synthesis ◽  
Silica Core

Incorporation of monoethanolamine (MEA), diethanolamine (DEA) and methyldiethanolamine (MDEA) in mesoporous silica: An alternative to CO2 capture

2016 ◽  
Vol 4 (4) ◽  
pp. 4514-4524 ◽  
Author(s):  
Simone G. de Ávila ◽  
Marco A. Logli ◽  
Luís Carlos C. Silva ◽  
Márcia C.A. Fantini ◽  
Jivaldo R. Matos
Keyword(s):  
Mesoporous Silica ◽  
Co2 Capture
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