scholarly journals Bacterial diversity in snow from mid-latitude mountain areas: Alps, Eastern Anatolia, Karakoram and Himalaya

2018 ◽  
Vol 59 (77) ◽  
pp. 10-20 ◽  
Author(s):  
Roberto Sergio Azzoni ◽  
Ilario Tagliaferri ◽  
Andrea Franzetti ◽  
Christoph Mayer ◽  
Astrid Lambrecht ◽  
...  
Keyword(s):  
Microbial Communities ◽  
Bacterial Communities ◽  
The Arctic ◽  
Eastern Anatolia ◽  
Mountain Areas ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses ◽  
Operational Taxonomic Units ◽  
High Throughput Dna Sequencing

ABSTRACTSnow can be considered an independent ecosystem that hosts active microbial communities. Snow microbial communities have been extensively investigated in the Arctic and in the Antarctica, but rarely in mid-latitude mountain areas. In this study, we investigated the bacterial communities of snow collected in four glacierized areas (Alps, Eastern Anatolia, Karakoram and Himalaya) by high-throughput DNA sequencing. We also investigated the origin of the air masses that produced the sampled snowfalls by reconstructing back-trajectories. A standardized approach was applied to all the analyses in order to ease comparison among different communities and geographical areas. The bacterial communities hosted from 25 to 211 Operational Taxonomic Units (OTUs), and their structure differed significantly between geographical areas. This suggests that snow bacterial communities may largely derive from ‘local’ air bacteria, maybe by deposition of airborne particulate of local origin that occurs during snowfall. However, some evidences suggest that a contribution of bacteria collected during air mass uplift to snow communities cannot be excluded, particularly when the air mass that originated the snow event is particularly rich in dust.

scholarly journals Measurements of aerosol and CCN properties in the Mackenzie River delta (Canadian Arctic) during spring–summer transition in May 2014

2018 ◽  
Vol 18 (7) ◽  
pp. 4477-4496 ◽  
Author(s):  
Paul Herenz ◽  
Heike Wex ◽  
Silvia Henning ◽  
Thomas Bjerring Kristensen ◽  
Florian Rubach ◽  
...  
Keyword(s):  
Particle Number ◽  
Oil Field ◽  
River Delta ◽  
The Arctic ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses ◽  
North East ◽  
The North ◽  
Mackenzie River

Abstract. Within the framework of the RACEPAC (Radiation–Aerosol–Cloud Experiment in the Arctic Circle) project, the Arctic aerosol, arriving at a ground-based station in Tuktoyaktuk (Mackenzie River delta area, Canada), was characterized during a period of 3 weeks in May 2014. Basic meteorological parameters and particle number size distributions (PNSDs) were observed and two distinct types of air masses were found. One type were typical Arctic haze air masses, termed accumulation-type air masses, characterized by a monomodal PNSD with a pronounced accumulation mode at sizes above 100 nm. These air masses were observed during a period when back trajectories indicate an air mass origin in the north-east of Canada. The other air mass type is characterized by a bimodal PNSD with a clear minimum around 90 nm and with an Aitken mode consisting of freshly formed aerosol particles. Back trajectories indicate that these air masses, termed Aitken-type air masses, originated from the North Pacific. In addition, the application of the PSCF receptor model shows that air masses with their origin in active fire areas in central Canada and Siberia, in areas of industrial anthropogenic pollution (Norilsk and Prudhoe Bay Oil Field) and the north-west Pacific have enhanced total particle number concentrations (NCN). Generally, NCN ranged from 20 to 500 cm−3, while cloud condensation nuclei (CCN) number concentrations were found to cover a range from less than 10 up to 250 cm−3 for a supersaturation (SS) between 0.1 and 0.7 %. The hygroscopicity parameter κ of the CCN was determined to be 0.23 on average and variations in κ were largely attributed to measurement uncertainties. Furthermore, simultaneous PNSD measurements at the ground station and on the Polar 6 research aircraft were performed. We found a good agreement of ground-based PNSDs with those measured between 200 and 1200 m. During two of the four overflights, particle number concentrations at 3000 m were found to be up to 20 times higher than those measured below 2000 m; for one of these two flights, PNSDs measured above 2000 m showed a different shape than those measured at lower altitudes. This is indicative of long-range transport from lower latitudes into the Arctic that can advect aerosol from different regions in different heights.

scholarly journals Measurements of aerosol and CCN properties in the Mackenzie River delta (Canadian Arctic) during Spring-Summer transition in May 2014

2017 ◽  
Author(s):  
Paul Herenz ◽  
Heike Wex ◽  
Silvia Henning ◽  
Thomas Bjerring Kristensen ◽  
Florian Rubach ◽  
...  
Keyword(s):  
Particle Number ◽  
Cloud Condensation Nuclei ◽  
River Delta ◽  
The Arctic ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses ◽  
North East ◽  
The North ◽  
Mackenzie River

Abstract. Within the framework of the RACEPAC (Radiation-Aerosol-Cloud Experiment in the Arctic Circle) project, the Arctic aerosol, arriving at a ground based station in Tuktoyaktuk (Mackenzie River delta area, Canada), was characterized during a period of 3 weeks in May 2014. The observations of basic meteorological parameters and particle number size distributions (PNSDs) were indicative for the rapid transition from Arctic spring to summer that took place during the measurement period. Two distinct types of air masses were found. One type were typical Arctic haze air masses, termed as spring-type air masses, characterized by a mono-modal PNSD with a pronounced accumulation mode at sizes above 100 nm. These air masses were observed during a period when back trajectories indicate an air mass origin in the north east of Canada. The other air mass type is characterized by a bi-modal PNSD with a clear minimum around 90 nm, and with an Aitken mode consisting of freshly formed aerosol particles. Back trajectories indicate that these air masses, termed as summer-type air masses, originated from the northern Pacific. Generally total particle number concentrations (NCN) ranged from 20 to 500 cm−3, while cloud condensation nuclei (CCN) number concentrations were found to cover a range between less than 10 up to 250 cm−3 for a supersaturation (SS) between 0.1 and 0.7 %. The hygroscopicity parameter κ of the CCN was determined to be 0.23 on average and variations in kappa were largely attributed to measurement uncertainties. Furthermore, simultaneous PNSD measurements at the ground station and on the Polar 6 research aircraft were performed. We found a good agreement of ground based PNSDs with those measured between 200 and 1200 m. During two of the four overflights, particle number concentrations at 3000 m were found to be up to twenty times higher than those measured below 2000 m, and for one of these two flights, PNSDs measured above 2000 m showed a different shape than those measured at lower altitudes. This is indicative for long range transport from lower latitudes into the Arctic that can advect aerosol from different regions in different heights.

scholarly journals Identification of the Aerosol Types over Athens, Greece: The Influence of Air-Mass Transport

2010 ◽  
Vol 2010 ◽  
pp. 1-15 ◽  
Author(s):  
D. G. Kaskaoutis ◽  
P. G. Kosmopoulos ◽  
H. D. Kambezidis ◽  
P. T. Nastos
Keyword(s):  
Winter Season ◽  
Saharan Dust ◽  
Dust Particles ◽  
Hysplit Model ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses ◽  
Local Pollution ◽  
Coarse Mode ◽  
Aerosol Types

Aerosol optical depth at 550 nm () and fine-mode (FM) fraction data from Terra-MODIS were obtained over the Greater Athens Area covering the period February 2000–December 2005. Based on both and FM values three main aerosol types have been discriminated corresponding to urban/industrial aerosols, clean maritime conditions, and coarse-mode, probably desert dust, particles. Five main sectors were identified for the classification of the air-mass trajectories, which were further used in the analysis of the ( and FM data for the three aerosol types). The HYSPLIT model was used to compute back trajectories at three altitudes to investigate the relation between -FM and wind sector depending on the altitude. The accumulation of local pollution is favored in spring and corresponds to air masses at lower altitudes originating from Eastern Europe and the Balkan. Clean maritime conditions are rare over Athens, limited in the winter season and associated with air masses from the Western or Northwestern sector. The coarse-mode particles origin seems to be more complicated proportionally to the season. Thus, in summer the Northern sector dominates, while in the other seasons, and especially in spring, the air masses belong to the Southern sector enriched with Saharan dust aerosols.

scholarly journals Aerosol Characteristics in the Three Poles of the Earth Observed by CALIPSO

2020 ◽  
Author(s):  
Yikun Yang ◽  
Chuanfeng Zhao ◽  
Quan Wang ◽  
Zhiyuan Cong ◽  
Xingchuan Yang ◽  
...  
Keyword(s):  
South Asia ◽  
Ross Sea ◽  
Temporal Trends ◽  
Arctic Region ◽  
The Arctic ◽  
Hysplit Model ◽  
Back Trajectories ◽  
Air Masses ◽  
Spatial And Seasonal Variation ◽  
The Antarctic

Abstract. To better understand the aerosol properties over the Arctic, Antarctic, and Tibetan Plateau (TP), the aerosol optical properties were investigated using 13 years CALIPSO L3 data, and the back trajectories for air masses were also simulated using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. The results show that the aerosol optical depth (AOD) has obvious spatial and seasonal variation characteristics, and the aerosol loading over Eurasia, Ross Sea, and South Asia is relatively large. The annual average AOD in the Arctic, Antarctic, and TP are 0.046, 0.025, and 0.098, respectively. The Arctic and Antarctic regions have larger AOD values in winter and spring, while the TP in spring and summer. There are no significant temporal trends of AOD anomalies in the three study regions. Clean marine and dust-related aerosols are the dominant types over ocean and land respectively in both the Arctic and Antarctic, while dust-related aerosol types have greater occurrence frequency (OF) over the TP. The OF of dust-related and elevated smoke is large for a broad range of heights, indicating that they are likely transported aerosols, while other types of aerosols mainly occurred at heights below 2 km in the Antarctic and Arctic. The maximum OF of dust-related aerosols mainly occurs at 6 km altitude over the TP. The analysis of back trajectories of the air masses shows large differences among different regions and seasons. The Arctic region is more vulnerable to mid-latitude pollutants than the Antarctic region, especially in winter and spring, while the air masses in the TP are mainly from the Iranian Plateau, Tarim Basin, and South Asia.

scholarly journals In situ measurements of aerosols optical properties and number size distributions in a subarctic coastal region of Norway

2011 ◽  
Vol 11 (12) ◽  
pp. 32921-32964
Author(s):  
S. Mogo ◽  
V. E. Cachorro ◽  
J. F. Lopez ◽  
E. Montilla ◽  
B. Torres ◽  
...  
Keyword(s):  
Optical Properties ◽  
Single Scattering ◽  
Mean Value ◽  
The Arctic ◽  
Optical Parameters ◽  
Size Distributions ◽  
Air Mass ◽  
Air Masses ◽  
Particle Sizer

Abstract. In situ measurements of aerosol optical properties were made in the summer of 2008 at the ALOMAR station facility (69°16 N, 16°00 E), located at a rural site in the north of the island of Andøya (Vesterålen archipelago), approximately 300 km north of the Arctic Circle. The extended three-month campaign was part of the POLARCAT Project (Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols, and Transport) of the International Polar Year (IPY-2007-2008). Its goal was to characterize the aerosols of this sub-Arctic area, which are frequently transported to the Arctic region. The ambient light-scattering coefficient, σs (550 nm), at ALOMAR had a measured hourly mean value of 5.41 Mm−1 (StD = 3.55 Mm−1), and the light-absorption coefficient, σa (550 nm), had a measured hourly mean value of 0.40 Mm−1 (StD = 0.27 Mm−1). The scattering/absorption Ångström exponents, αs,a, are used for a detailed analysis of the variations of the spectral shape of σs,a. Whereas αs demonstrates the presence of two particle sizes corresponding to two types of aerosols, the αa demonstrates only one type of absorbing aerosol particles. Values of αa above 1 were not observed. The single-scattering albedo, ω0, ranged from 0.62 to 0.99 (mean = 0.91, StD = 0.05), and the relationships of this property to the absorption/scattering coefficients and the Ångström exponents are presented. The concentration of the particles was monitored using a scanning mobility particle sizer (SMPS), an aerodynamic particle sizer (APS) and an ultrafine condensation particle counter (UCPC). The shape of the median size distribution of the particles in the submicrometer fraction was bimodal, and the submicrometer, micrometer and total concentrations presented hourly mean values of 1277 cm3 (StD = 1563 cm3), 1 cm3 (StD = 1 cm3) and 2463 cm3 (StD = 4251 cm3), respectively. The modal correlations were investigated, and the concentration of particles sized between 30 and 100 nm (Aitken mode) are presented as a function of the concentration of the particles sized between 100 and 390 nm (accumulation mode). The optical and the microphysical parameters are related to each other, and the results are presented. The origins and pathways of air masses were examined by computing the back-trajectories in a trajectory model (HYSPLIT). Six geographical sectors were defined to classify the air masses, and, based on the sector classification, the linkage between the air mass origin and the optical parameters was established. Aerosol size distributions were also evaluated in relation to the air masses. The relationships between the air mass origins and other parameters, especially those related to the single scattering albedo, allow us to describe two characteristic situations: northern and western air masses, which had predominantly marine aerosols, presented lower optical parameter values, indicating predominantly coarser and non-absorbent particles; and eastern and southern air masses, in which continental aerosols were predominant, presented higher values for all optical parameters, indicating the presence of smaller absorbent particles.

scholarly journals Long-Range Transport of Water Channelized through the Southern Subtropical Jet

Atmosphere ◽  
2018 ◽  
Vol 9 (10) ◽  
pp. 374 ◽  
Author(s):  
Eliane Larroza ◽  
Philippe Keckhut ◽  
Jean-Luc Baray ◽  
Walter Nakaema ◽  
Hélène Vérèmes ◽  
...  
Keyword(s):  
Satellite Observation ◽  
Sao Paulo ◽  
Cloud Formation ◽  
Physical Parameters ◽  
Cirrus Cloud ◽  
São Paulo ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses ◽  
Subtropical Jet

In this study, an air mass (containing a cirrus cloud) was detected by light detection and ranging (lidar) above São Paulo (Brazil) in June 2007 and tracked around the globe, thanks to Lagrangian calculations as well as ground-based and satellite observations. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data were also used to provide locations of occurrence of cirrus around the globe and extract their respective macro physical parameters (altitude and temperature). An analysis of the air mass history based on Lagrangian trajectories reveals that water coming from the Equator is channelized through the southern subtropical jet for weeks. In this case, the back-trajectories showed that the cirrus cloud detected at São Paulo was a mixture of air masses from two different locations: (1) the active convective area located around the Equator, with transport into the upper troposphere that promotes cirrus cloud formation; and (2) the South Pacific Ocean, with transport that follows the subtropical jet stream (STJ). Air masses coming from equatorial convective regions are trapped by the jet, which contributes to maintaining the lifetime of the cirrus cloud for a few days. The cloud disappears near the African continent, due to a southern excursion and warmer temperatures, then reappears and is detected again by the lidar system in São Paulo after 12 days. The observed cloud is located at a similar altitude, revealing that sedimentation is small or compensated by radiative uplift.

scholarly journals Air mass origins influencing TTL chemical composition over West Africa during 2006 summer monsoon

2010 ◽  
Vol 10 (22) ◽  
pp. 10753-10770 ◽  
Author(s):  
K. S. Law ◽  
F. Fierli ◽  
F. Cairo ◽  
H. Schlager ◽  
S. Borrmann ◽  
...  
Keyword(s):  
West Africa ◽  
Summer Monsoon ◽  
Large Scale ◽  
Lower Stratosphere ◽  
Deep Convection ◽  
Lower Troposphere ◽  
Trace Gas ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses

Abstract. Trace gas and aerosol data collected in the tropical tropopause layer (TTL) between 12–18.5 km by the M55 Geophysica aircraft as part of the SCOUT-AMMA campaign over West Africa during the summer monsoon in August 2006 have been analysed in terms of their air mass origins. Analysis of domain filling back trajectories arriving over West Africa, and in the specific region of the flights, showed that the M55 flights were generally representative of air masses arriving over West Africa during the first 2 weeks of August, 2006. Air originating from the mid-latitude lower stratosphere was under-sampled (in the mid-upper TTL) whilst air masses uplifted from central Africa (into the lower TTL) were over-sampled in the latter part of the campaign. Signatures of recent (previous 10 days) origins were superimposed on the large-scale westward flow over West Africa. In the lower TTL, air masses were impacted by recent local deep convection over Africa at the level of main convective outflow (350 K, 200 hPa) and on certain days up to 370 K (100 hPa). Estimates of the fraction of air masses influenced by local convection vary from 10 to 50% depending on the method applied and from day to day during the campaign. The analysis shows that flights on 7, 8 and 11 August were more influenced by local convection than on 4 and 13 August allowing separation of trace gas and aerosol measurements into "convective" and "non-convective" flights. Strong signatures, particularly in species with short lifetimes (relative to CO2) like CO, NO and fine-mode aerosols were seen during flights most influenced by convection up to 350–365 K. Observed profiles were also constantly perturbed by uplift (as high as 39%) of air masses from the mid to lower troposphere over Asia, India, and oceanic regions resulting in import of clean oceanic (e.g. O3-poor) or polluted air masses from Asia (high O3, CO, CO2) into West Africa. Thus, recent uplift of CO2 over Asia may contribute to the observed positive CO2 gradients in the TTL over West Africa. This suggests a more significant fraction of younger air masses in the TTL and needs to taken into consideration in derivations of mean age of air. Transport of air masses from the mid-latitude lower stratosphere had an impact from the mid-TTL upwards (20–40% above 370 K) during the campaign period importing air masses with high O3 and NOy. Ozone profiles show a less pronounced lower TTL minimum than observed previously by regular ozonesondes at other tropical locations. Concentrations are less than 100 ppbv in the lower TTL and vertical gradients less steep than in the upper TTL. The air mass origin analysis and simulations of in-situ net photochemical O3 production, initialised with observations, suggest that the lower TTL is significantly impacted by uplift of O3 precursors (over Africa and Asia) leading to positive production rates (up to 2 ppbv per day) in the lower and mid TTL even at moderate NOx levels. Photochemical O3 production increases with higher NOx and H2O in air masses with O3 less than 150 ppbv.

scholarly journals Dynamics of gaseous oxidized mercury at Villum Research Station during the High Arctic summer

2021 ◽  
Author(s):  
Jakob Boyd Pernov ◽  
Bjarne Jensen ◽  
Andreas Massling ◽  
Daniel Charles Thomas ◽  
Henrik Skov
Keyword(s):  
Meteorological Data ◽  
High Arctic ◽  
Atmospheric Mercury ◽  
The Arctic ◽  
Research Station ◽  
Cold Temperatures ◽  
Air Mass ◽  
Back Trajectories ◽  
Arctic Summer ◽  
Gaseous Oxidized Mercury

Abstract. While much research has been devoted to the subject of gaseous elemental mercury (GEM) and gaseous oxidized mercury (GOM) in the Arctic spring, during atmospheric mercury depletion events, few studies have examined the behavior of GOM in the High Arctic summer. GOM, once introduced into the ecosystem, can pose a threat to human and wildlife health, though there remain large uncertainties regarding the transformation, deposition, and assimilation of mercury into the ecosystem. Therefore, to further our understanding of the dynamics of gaseous oxidized mercury in the High Arctic during the late summer, we performed measurements of GEM and GOM along with meteorological parameters, atmospheric constituents, and air mass history during two summer campaigns in 2019 and 2020 at Villum Research Station (Villum) in Northeastern Greenland. Five events of enhanced GOM concentrations were identified and investigated in greater detail. The origin of these events was identified, through analysis of air mass back-trajectories, associated meteorological data, and other atmospheric constituents, to be the cold, dry free troposphere. These events were associated with low RH, limited precipitation, cold temperatures, and intense sunlight along the trajectory path. Events were positively correlated with ozone, aerosol particle number, and black carbon mass concentration, which were interpreted as an indication of tropospheric air masses. This work aims to provide a better understanding of the dynamics of GOM during the High Arctic summer.

scholarly journals Changes in aerosol properties during spring-summer period in the Arctic troposphere

2007 ◽  
Vol 7 (1) ◽  
pp. 1215-1260 ◽  
Author(s):  
A.-C. Engvall ◽  
R. Krejci ◽  
J. Ström ◽  
R. Treffeisen ◽  
R. Scheele ◽  
...  
Keyword(s):  
Mass Transport ◽  
Time Window ◽  
Rapid Change ◽  
Chemical Properties ◽  
Anthropogenic Sources ◽  
The Arctic ◽  
Data Set ◽  
Air Mass ◽  
Back Trajectories ◽  
Aerosol Properties

Abstract. The change in aerosol properties during the transition from the more polluted spring to the clean summer Arctic troposphere was studied. A six year data set of observations from Ny-Ålesund, Svalbard, covering the months April through June serve as the basis for the characterisation of this time period. In addition four-day-back trajectories were used to describe air mass histories. The observed transition in aerosol properties from an accumulation mode dominated to an Aitken mode dominated size distribution is discussed with respect to long-range transport and influences from natural and anthropogenic sources of aerosols and pertinent trace gases. Our study shows that the air-mass transport is an important factor modulating the physical and chemical properties observed. However, the air-mass transport cannot alone explain the yearly repeatable systematic and rather rapid change in aerosol properties, occurring within a limited time window of approximately 10 days. With a simplified phenomenological model, which delivers the nucleation potential for new particle formation, we suggest that the rapid shift in aerosol microphysical properties between the Arctic spring and summer is mainly driven by the incoming solar radiation in concert with transport of precursor gases and changes in condensational sink.

scholarly journals Air mass origins influencing TTL chemical composition over West Africa during 2006 summer monsoon

2010 ◽  
Vol 10 (6) ◽  
pp. 15485-15536 ◽  
Author(s):  
K. S. Law ◽  
F. Fierli ◽  
F. Cairo ◽  
H. Schlager ◽  
S. Borrmann ◽  
...  
Keyword(s):  
West Africa ◽  
Summer Monsoon ◽  
Large Scale ◽  
Lower Stratosphere ◽  
Deep Convection ◽  
Lower Troposphere ◽  
Trace Gas ◽  
Air Mass ◽  
Back Trajectories ◽  
Air Masses

Abstract. Trace gas and aerosol data collected in the tropical tropopause layer (TTL) between 12–18.5 km by the M55 Geophysica aircraft as part of the SCOUT-AMMA campaign over West Africa during the summer monsoon in August 2006 have been analysed in terms of their air mass origins. Analysis of domain filling back trajectories arriving over West Africa, and in the specific region of the flights, showed that the M55 flights were generally representative of air masses arriving over West Africa during the first 2 weeks of August, 2006. Air originating from the mid-latitude lower stratosphere was under-sampled (in the mid-upper TTL) whilst air masses uplifted from central Africa (into the lower TTL) were over-sampled in the latter part of the campaign. Signatures of recent (previous 10 days) origins were superimposed on the large-scale westerly flow over West Africa. In the lower TTL, air masses were impacted by recent local deep convection over Africa at the level of main convective outflow (350 K, 200 hPa) and on certain days up to 370 K (100 hPa). Estimates of the fraction of air masses influenced by local convection vary from 10 to 50% depending on the method applied and from day to day during the campaign. The analysis shows that flights on 7, 8 and 11 August were more influenced by local convection than on 4 and 13 August allowing separation of trace gas and aerosol measurements into ''convective'' and ''non-convective'' flights. Strong signatures, particularly in short-lived species like CO, NO and fine-mode aerosols were seen during flights most influenced by convection up to 350–365 K. Observed profiles were also constantly perturbed by uplift (as high as 39%) of air masses from the mid to lower troposphere over Asia, India, and oceanic regions resulting in import of clean oceanic (e.g., O3-poor) or polluted air masses from Asia (high O3, CO, CO2) into West Africa. Thus, recent uplift of CO2 over Asia may contribute to the observed positive CO2 gradients in the TTL over West Africa. This suggests a more significant fraction of younger air masses in the TTL making it difficult to derive mean age of air from average gradients. Transport of air masses from the mid-latitude lower stratosphere had an impact from the mid-TTL upwards (20–40% above 370 K) during the campaign period importing air masses with high O3 and NOy. Ozone profiles show a less pronounced lower TTL minimum than observed previously by regular ozonesondes at other tropical locations. Concentrations are less than 100 ppbv in the lower TTL and vertical gradients less steep than in the upper TTL. The air mass origin analysis and simulations of in-situ net photochemical O3 production, initialised with observations, suggest that the lower TTL is significantly impacted by uplift of O3 precursors (over Africa and Asia) leading to positive production rates (up to 2 ppbv per day) in the lower and mid TTL even at moderate NOx levels. Photochemical O3 production increases with higher NOx and H2O in air masses with O3 less than 150 ppbv.

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