Kinetics of oxidation of cyclohexanone in a jet-stirred reactor: Experimental and modeling

2015 ◽  
Vol 35 (1) ◽  
pp. 507-514 ◽  
Author(s):  
Z. Serinyel ◽  
C. Togbé ◽  
A. Zaras ◽  
G. Dayma ◽  
P. Dagaut
2010 ◽  
Vol 24 (3) ◽  
pp. 1668-1676 ◽  
Author(s):  
H. P. Ramirez L. ◽  
K. Hadj-Ali ◽  
P. Diévart ◽  
G. Moréac ◽  
P. Dagaut

2010 ◽  
Vol 24 (9) ◽  
pp. 4904-4911 ◽  
Author(s):  
A. Mzé-Ahmed ◽  
K. Hadj-Ali ◽  
P. Diévart ◽  
P. Dagaut

Author(s):  
Philippe Dagaut ◽  
Sandro Gai¨l

The oxidation of kerosene and bio-kerosene (kerosene-rapeseed oil methyl esters 80/20 in mole) was studied experimentally in a jet-stirred reactor at 10 atm and constant residence time, over the high temperature range 740-1200 K, and for variable equivalence ratios in the range 0.5–1.5. Concentration profiles of reactants, stable intermediates, and final products were obtained by probe sampling followed by on-line and off-line GC analyses. The oxidation of these fuels in these conditions was modeled using a detailed kinetic reaction mechanism consisting of 2027 reversible reactions and 263 species. The surrogate bio-kerosene model-fuel used consisted of a mixture of n-hexadecane, n-propylcyclohexane, n-propylbenzene, and n-decane. For bio-kerosene, the methyl ester fraction was simply represented by n-hexadecane. The proposed kinetic reaction mechanism used in the modeling yielded a good representation of the kinetics of oxidation of kerosene and bio-kerosene under JSR conditions. The data and the model showed the bio-kerosene (Jet A-1/RME mixture) has a slightly higher reactivity than Jet A-1 whereas not major modification of the products distribution was observed besides the formation of small methyl esters from RME’s oxidation.


2019 ◽  
Vol 37 (1) ◽  
pp. 381-388 ◽  
Author(s):  
Sébastien Thion ◽  
Casimir Togbé ◽  
Philippe Dagaut ◽  
Guillaume Dayma ◽  
Zeynep Serinyel

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