Probing the smallest soot particles in low-sooting premixed flames using laser-induced incandescence

2015 ◽  
Vol 35 (2) ◽  
pp. 1843-1850 ◽  
Author(s):  
Henrik Bladh ◽  
Nils-Erik Olofsson ◽  
Thomas Mouton ◽  
Johan Simonsson ◽  
Xavier Mercier ◽  
...  
1997 ◽  
Author(s):  
K. McManus ◽  
M. Allen ◽  
W. Rawlins ◽  
K. McManus ◽  
M. Allen ◽  
...  

2005 ◽  
Vol 6 (1) ◽  
pp. 21-42 ◽  
Author(s):  
H Kosaka ◽  
T Aizawa ◽  
T Kamimoto

The processes of ignition and formation of soot precursor and soot particles in a diesel spray flame achieved in a rapid compression machine (RCM) were imaged two-dimensionally using the laser sheet techniques. For the two-dimensional imaging of time and of location where ignition first occurs in a diesel spray, planar laser-induced fluorescence (PLIF) of formaldehyde was applied to a diesel spray in an RCM. Formaldehyde has been hypothesized to be one of the stable intermediate species marking the start of oxidation reactions in a transient spray under compression ignition conditions. In this study, the laser-induced fluorescence (LIF) images of the formaldehyde formed in a diesel fuel spray during the ignition process have been obtained by exciting formaldehyde with the third harmonic of a neodymium-doped yttrium aluminium garnet (Nd:YAG) laser. The LIF images of formaldehyde in a spray revealed that the time when the first fluorescence is detected is almost identical with the time when the total heat release due to low-temperature oxidation reactions equals the heat absorption by fuel vaporization in the spray. The formaldehyde level rose steadily until the high-temperature reaction phase of diesel spray ignition. At the start of this ‘hot-ignition’ phase, the formaldehyde concentration fell rapidly, thus signalling the end of the low-temperature ignition phase. Increases in the initial ambient gas temperatures advanced the hot-ignition starting time. The first hot ignition occurred in the periphery of spray head at initial ambient gas temperatures between 580 and 660 K. When the ambient gas temperature was increased to 790 K, the position of the first ignition moved to the central region of the spray head. For the investigation of soot formation processes in a diesel spray flame, simultaneous imaging of the soot precursor and soot particles in a transient spray flame in an RCM was conducted by PLIF and by planar laser-induced incandescence (PLII) techniques. The third harmonic (355 nm) and the fundamental (1064 nm) laser pulses from an Nd:YAG laser, between which a delay of 44 ns was imposed by 13.3 m of optical path difference, were used to excite LIF from the soot precursor and laser-induced incandescence (LII) from soot particles in the spray flame. The LIF and the LII were separately imaged by two image-intensified charge-coupled device cameras with identical detection wavelengths of 400 nm and bandwidths of 80 nm. The LIF from the soot precursor was mainly located in the central region of the spray flame between 40 and 55 mm (between 270 and 370 times the nozzle orifice diameter d°) from the nozzle orifice. The LII from soot particles was observed to surround the soot precursor LIF region and to extend downstream. The first appearance of the LIF from the soot precursor in the spray flame preceded the appearance of the LII from soot particles. The intensity of the LIF from the soot precursor reached its maximum immediately after rich premixed combustion. In contrast, the intensity of the LII from soot particles increased gradually and reached its maximum after the end of injection. Measured LIF spectra, of the soot precursor in the spray flame, were very broad with the peak between 430 and 460 nm.


Author(s):  
Aritra Chakraborty ◽  
Satya R. Chakravarthy

This paper reports an investigation of soot formation in ethylene-air partially premixed flames over a wide range of premixedness. An axisymmetric co-flow configuration is chosen to establish partially premixed flames from the fully non-premixed to fully premixed conditions. Reducing the fuel flow rate as a percentage of the maximum from the core stream and supplying the same to the annular stream leads to stratification of the reactant concentrations. The thermal power, overall equivalence ratio, and the average velocity in the both streams are maintained constant under all conditions. The soot volume fraction is estimated by light attenuation method, and laser induced incandescence is performed to map the soot distribution in the flow field. The soot volume fraction is observed to exhibit a ‘S’-type trend as the conditions are traversed from near the premixed to the non-premixed regimes. That is, when traversing from the non-premixed to near-premixed regime, below 60% fuel flow rate in core, the soot volume fraction drops drastically. The onset of sooting in the partially premixed flames is clearly seen to be at the tip of the rich-premixed flame branch of their triple flame structure, which advances upstream towards the base of the flame as the premixing is reduced. The ‘S’-type variation is clearly the effect of partial premixing, more specifically due to the presence of the lean premixed flame branch of the triple flame. Laser induced incandescence intensities are insufficient to capture the upstream advance of the soot onset with decreased premixedness. So, a quick and inexpensive technique to isolate soot luminescence through flame imaging is presented in the paper involving quasi-simultaneous imaging with a 650 nm and a BG-3 filter using a normal color camera.


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