Identification of long-range transport pathways and potential sources of PM2.5 and PM10 in Beijing from 2014 to 2015

2017 ◽  
Vol 56 ◽  
pp. 214-229 ◽  
Author(s):  
Deping Li ◽  
Jianguo Liu ◽  
Jiaoshi Zhang ◽  
Huaqiao Gui ◽  
Peng Du ◽  
...  
Keyword(s):  
Long Range ◽  
Long Range Transport ◽  
Transport Pathways ◽  
Range Transport ◽  
Potential Sources ◽  
Pm2.5 And Pm10

scholarly journals Concentration Trajectory Route of Air pollution with an Integrated Lagrangian model (C-TRAIL model v1.0) derived from the Community Multiscale Air Quality Modeling (CMAQ model v5.2)

2020 ◽  
Author(s):  
Arman Pouyaei ◽  
Yunsoo Choi ◽  
Jia Jung ◽  
Bavand Sadeghi ◽  
Chul Han Song
Keyword(s):  
Air Pollution ◽  
Air Quality ◽  
Long Range ◽  
Lagrangian Model ◽  
Long Range Transport ◽  
Air Masses ◽  
Range Transport ◽  
Potential Sources ◽  
Model C ◽  
Co Concentrations

Abstract. This paper introduces a reliable and comprehensive Lagrangian output (Concentration Trajectory Route of Air pollution with Integrated Lagrangian model, C-TRAIL version 1.0) from an Eulerian air quality model for validating the source-receptor link by following real polluted air masses. To investigate the concentrations and trajectories of air masses simultaneously, we implement the trajectory-grid (TG) Lagrangian advection scheme in the CMAQ (Community Multiscale Air Quality) Eulerian model version 5.2. The TG algorithm follows the concentrations of representative air packets of species along trajectories determined by the wind field. The generated output from C-TRAIL accurately identifies the origins of pollutants. For validation, we analyzed the results of C-TRAIL during the KORUS-AQ campaign over South Korea. Initially, we implemented C-TRAIL in a simulation of CO concentrations with an emphasis on the long- and short-range transport effect. The output from C-TRAIL reveals that local trajectories were responsible for CO concentrations over Seoul during the stagnant period (May 17–22, 2016) and during the extreme pollution period (May 25–28, 2016), highly polluted air masses from China were distinguished as sources of CO transported to the Seoul Metropolitan Area (SMA). We conclude that long-range transport played a crucial role in high CO concentrations over the receptor area during this period. Furthermore, for May 2016, we find that the potential sources of CO over that SMA were the result of either local transport or long-range transport from the Shandong Peninsula and, in some cases, from north of the SMA. By identifying the trajectories of CO concentrations, one can use the results from C-TRAIL to directly link strong potential sources of pollutants to a receptor in specific regions during various time frames.

scholarly journals Long range transport of mercury to the Arctic and across Canada

2010 ◽  
Vol 10 (2) ◽  
pp. 4673-4717 ◽  
Author(s):  
D. Durnford ◽  
A. Dastoor ◽  
D. Figueras-Nieto ◽  
A. Ryjkov
Keyword(s):  
North America ◽  
Long Range ◽  
Transport Model ◽  
Extensive Study ◽  
Atmospheric Mercury ◽  
The Arctic ◽  
Long Range Transport ◽  
Chemical Transport Model ◽  
Transport Pathways ◽  
Range Transport

Abstract. This study is the most extensive study to date on the transport of mercury to the Arctic. Moreover, it is the first such study to use a fully-coupled, online chemical transport model, Environment Canada's Global/Regional Atmospheric Heavy Metals model (GRAHM), where the meteorology and mercury processes are fully integrated. It is also the only study to date on the transport of mercury across Canada. We determined source attribution from Asia, North America, Russia and Europe at six arctic verification stations, as well as three subarctic and eight midlatitude Canadian stations. We have found that Asia, despite having transport efficiencies that were almost always lower than those of North America and often lower than those of Russia, was the dominant source of gaseous atmospheric mercury at all verification stations: it contributed the most mercury (29–37% at all stations, seasons and levels considered), its concentrations frequently explained nearly 100% of the variability in the concentrations produced by the simulation performed with full global emissions, particularly in the absence of local sources, and it generated the most long range transport (LRT) events, causing 43%, 67% and 75% of the events at the arctic, subarctic and midlatitude stations, respectively. For the Arctic, Russian transport efficiencies tended to be the strongest, as expected, while European and Asian efficiencies were lower and higher, respectively, than those found in the literature. This disagreement is likely produced by mercury's long lifetime relative to that of other pollutants. The accepted springtime preference for the trans-Pacific transport of Asian pollution was evident only in the midlatitude group of stations, being masked in the arctic and subarctic groups by the occurrence of atmospheric mercury depletion events. Some neighbouring arctic stations recorded dissimilar numbers of LRT events; despite their proximity, the behaviour of mercury at these stations was governed by different dynamics and transport pathways. The column burden of GEM in the lowest 5 km of the Northern Hemisphere was largest in summer from Asia, North America and Russia, but in winter from Europe. In the vertical, transport of mercury from all source regions occurred principally in the mid-troposphere.

scholarly journals Investigating sources of gaseous oxidized mercury in dry deposition at three sites across Florida, USA

2012 ◽  
Vol 12 (19) ◽  
pp. 9201-9219 ◽  
Author(s):  
M. Sexauer Gustin ◽  
P. S. Weiss-Penzias ◽  
C. Peterson
Keyword(s):  
United States ◽  
Long Range ◽  
Dry Deposition ◽  
Passive Sampling ◽  
Point Sources ◽  
Long Range Transport ◽  
Range Transport ◽  
Potential Sources ◽  
Sampling Systems ◽  
Surrogate Surfaces

Abstract. During 2009–2010, the State of Florida established a series of air quality monitoring stations to collect data for development of a statewide total maximum daily load (TMDL) for mercury (Hg). At three of these sites, located near Ft. Lauderdale (DVE), Pensacola (OLF), and Tampa Bay (TPA), passive samplers for the measurement of air Hg concentrations and surrogate surfaces for measurement of Hg dry deposition were deployed. While it is known that Hg in wet deposition in Florida is high compared to the rest of the United States, there is little information on Hg dry deposition. The objectives of the work were to: (1) investigate the utility of passive sampling systems for Hg in an area with low and consistent air concentrations as measured by the Tekran® mercury measurement system, (2) estimate dry deposition of gaseous oxidized Hg, and (3) investigate potential sources. This paper focuses on Objective 3. All sites were situated within 15 km of 1000 MW electricity generating plants (EGPs) and major highways. Bi-weekly dry deposition and passive sampler Hg uptake were not directly correlated with the automated Tekran® system measurements, and there was limited agreement between these systems for periods of high deposition. Using diel, biweekly, and seasonal Hg observations, and ancillary data collected at each site, the potential sources of Hg deposited to surrogate surfaces were investigated. With this information, we conclude that there are three major processes/sources contributing to Hg dry deposition in Florida, with these varying as a function of location and time of year. These include: (1) in situ oxidation of locally and regionally derived Hg facilitated by mobile source emissions, (2) indirect and direct inputs of Hg from local EGPs, and (3) direct input of Hg associated with long range transport of air from the northeastern United States. Based on data collected with the surrogate surface sampling system, natural background dry deposition for Florida is estimated to be 0.03 ng m−2 h−1. Deposition associated with mobile sources is 0.10 ng m−2 h−1 at TPA and DVE, and 0.03 ng m−2 h−1 at OLF. Long range transport contributes 0.8 ng m−2 h−1 in the spring. At DVE ~0.10 ng m−2 h−1 is contributed directly or indirectly from local point sources. We also suggest based on the data collected with the Tekran® and passive sampling systems that different chemical forms of GOM are associated with each of these sources.

scholarly journals Atmospheric speciated mercury concentrations on an island between China and Korea: sources and transport pathways

2015 ◽  
Vol 15 (22) ◽  
pp. 32931-32966 ◽  
Author(s):  
G.-S. Lee ◽  
P.-R. Kim ◽  
Y.-J. Han ◽  
T. M. Holsen ◽  
Y.-S. Seo ◽  
...  
Keyword(s):  
Long Range ◽  
Probability Function ◽  
Long Range Transport ◽  
Back Trajectory ◽  
Transport Pathways ◽  
Relative Significance ◽  
Secondary Formation ◽  
Range Transport ◽  
Global Pollutant ◽  
Conditional Probability Function

Abstract. As a global pollutant, mercury (Hg) is of particular concern in East Asia where anthropogenic emissions are the largest. In this study, speciated Hg concentrations were measured in the western most island in Korea, located between China and the Korean mainland to identify the importance of local, regional and distant Hg sources. Various tools including correlations with other pollutants, conditional probability function, and back-trajectory based analysis consistently indicated that Korean sources were important for gaseous oxidized mercury (GOM) whereas, for total gaseous mercury (TGM) and particulate bound mercury (PBM), long-range and regional transport were also important. A trajectory cluster based approach considering both Hg concentration and the fraction of time each cluster was impacting the site was developed to quantify the effect of Korean sources and out-of-Korean source. This analysis suggests that Korean sources contributed approximately 55 % of the GOM and PBM while there were approximately equal contributions from Korean and out-of-Korean sources for the TGM measured at the site. The ratio of GOM / PBM decreased when the site was impacted by long-range transport, suggesting that this ratio may be a useful tool for identifying the relative significance of local sources vs. long-range transport. The secondary formation of PBM through gas-particle partitioning with GOM was found to be important at low temperatures and high relative humidity.

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