Photoelectron angular distributions from single oriented molecules: Past, present and future

2015 ◽  
Vol 200 ◽  
pp. 247-256 ◽  
Author(s):  
Akira Yagishita
Keyword(s):  
Angular Distributions ◽  
Oriented Molecules ◽  
Photoelectron Angular Distributions

scholarly journals Photoelectron angular distributions from strong-field ionization of oriented molecules

2010 ◽  
Vol 6 (6) ◽  
pp. 428-432 ◽  
Author(s):  
Lotte Holmegaard ◽  
Jonas L. Hansen ◽  
Line Kalhøj ◽  
Sofie Louise Kragh ◽  
Henrik Stapelfeldt ◽  
...  
Keyword(s):  
Strong Field ◽  
Angular Distributions ◽  
Field Ionization ◽  
Strong Field Ionization ◽  
Oriented Molecules ◽  
Photoelectron Angular Distributions

MULTIPLE SCATTERING THEORY OF PHOTOELECTRON ANGULAR DISTRIBUTIONS FROM ORIENTED DIATOMIC MOLECULES

2002 ◽  
Vol 09 (02) ◽  
pp. 1213-1217 ◽  
Author(s):  
R. DÍEZ MUIÑO ◽  
D. ROLLES ◽  
F. J. GARCÍA DE ABAJO ◽  
C. S. FADLEY ◽  
M. A. VAN HOVE
Keyword(s):  
Gas Phase ◽  
Multiple Scattering ◽  
Electron Scattering ◽  
Scattering Theory ◽  
Angular Distributions ◽  
Spherically Symmetric ◽  
Photoelectron Diffraction ◽  
Oriented Molecules ◽  
Scattering Matrices ◽  
Photoelectron Angular Distributions

We use multiple scattering photoelectron diffraction (MSPD) theory to calculate the angular patterns of electrons photoemitted from the K-shell of CO and N 2 gas-phase oriented molecules, as recently measured by several groups. For low (E < 50 eV ) kinetic energies of the photoemitted electron, the electron scattering cannot be adequately represented by spherically symmetric potentials. We thus include nonspherical scattering potentials in our formalism through nondiagonal scattering matrices. We show that intramolecular scattering and interference are responsible for the experimentally measured patterns. This MSPD approach represents a more accurate and versatile method for dealing with such angular distributions as compared to prior calculations of these effects.

scholarly journals Anomaly in photoelectron angular distributions

2007 ◽  
Vol 76 (1) ◽  
Author(s):  
Jingtao Zhang ◽  
L. D. van Woerkom ◽  
Dong-Sheng Guo ◽  
R. R. Freeman
Keyword(s):  
Angular Distributions ◽  
Photoelectron Angular Distributions

Modeling Valence-Band Images from Synchrotron-Radiation Studies Using Display Analyzers: Lithium Fluoride and Graphite

1994 ◽  
Vol 375 ◽  
Author(s):  
Eric L. Shirley ◽  
Louis J. Terminello ◽  
John E. Klepeis ◽  
F. J. Himpsel
Keyword(s):  
Synchrotron Radiation ◽  
Band Structure ◽  
Lithium Fluoride ◽  
State Energy ◽  
Bragg Diffraction ◽  
Angular Distributions ◽  
Initial State ◽  
Statistical Comparison ◽  
Photoelectron Angular Distributions ◽  
Initial Crystal

AbstractWe present simulated photoelectron angular distributions (PAD's) for LiF and graphite. The results describe electron photocurrent versus photon energy, electron initial-state energy, and emission angles (leading to identification of two, or three, components of a valence electron's initial crystal momentum). Results are displayed in a fashion greatly facilitated by display analyzers. Earlier experimental results for LiF are confirmed in great detail. We discuss statistical comparison of theoretical and experimental PAD's. Effects of Bragg- diffraction on outgoing photoelectrons and uncertainty in crystal momentum normal to a surface are analyzed. In graphite, the observed lowering of symmetry, from that in a periodic-zone band structure to that seen in the PAD's, is modeled and explained.

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