Molecular strong field ionization and high harmonic generation: A selection of computational illustrations

2013 ◽  
Vol 414 ◽  
pp. 10-19 ◽  
Author(s):  
Michael Spanner ◽  
Serguei Patchkovskii
Keyword(s):  
Harmonic Generation ◽  
Strong Field ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Field Ionization ◽  
Strong Field Ionization ◽  
Selection Of

scholarly journals The sensitivities of high-harmonic generation and strong-field ionization to coupled electronic and nuclear dynamics

2014 ◽  
Vol 171 ◽  
pp. 113-132 ◽  
Author(s):  
Denitsa Baykusheva ◽  
Peter M. Kraus ◽  
Song Bin Zhang ◽  
Nina Rohringer ◽  
Hans Jakob Wörner
Keyword(s):  
Harmonic Generation ◽  
Strong Field ◽  
Stimulated Raman Scattering ◽  
High Harmonic ◽  
Simultaneous Detection ◽  
High Harmonic Generation ◽  
Field Ionization ◽  
Nuclear Dynamics ◽  
Strong Field Ionization ◽  
Electronic Dynamics

The sensitivities of high-harmonic generation (HHG) and strong-field ionization (SFI) to coupled electronic and nuclear dynamics are studied, using the nitric oxide (NO) molecule as an example. A coherent superposition of electronic and rotational states of NO is prepared by impulsive stimulated Raman scattering and probed by simultaneous detection of HHG and SFI yields. We observe a fourfold higher sensitivity of high-harmonic generation to electronic dynamics and attribute it to the presence of inelastic quantum paths connecting coherently related electronic states [Kraus et al., Phys. Rev. Lett.111, 243005 (2013)]. Whereas different harmonic orders display very different sensitivities to rotational or electronic dynamics, strong-field ionization is found to be most sensitive to electronic motion. We introduce a general theoretical formalism for high-harmonic generation from coupled nuclear-electronic wave packets. We show that the unequal sensitivities of different harmonic orders to electronic or rotational dynamics result from the angle dependence of the photorecombination matrix elements which encode several autoionizing and shape resonances in the photoionization continuum of NO. We further study the dependence of rotational and electronic coherences on the intensity of the excitation pulse and support the observations with calculations.

scholarly journals Effects of nodal planes on strong-field ionization and high-order-harmonic generation in ring-type molecules

2017 ◽  
Vol 96 (4) ◽  
Author(s):  
A. F. Alharbi ◽  
A. E. Boguslavskiy ◽  
N. Thiré ◽  
G. S. Thekkadath ◽  
S. Patchkovskii ◽  
...  
Keyword(s):  
Harmonic Generation ◽  
Strong Field ◽  
High Order ◽  
Field Ionization ◽  
High Order Harmonic Generation ◽  
Ring Type ◽  
Strong Field Ionization ◽  
High Order Harmonic

THz-driven strong-field dynamics in solids: High-harmonic generation and quasiparticle collisions

2017 ◽  
Author(s):  
F. Langer ◽  
M. Hohenleutner ◽  
C.P. Schmid ◽  
S. Schlauderer ◽  
U. Huttner ◽  
...  
Keyword(s):  
Harmonic Generation ◽  
Strong Field ◽  
High Harmonic ◽  
High Harmonic Generation

Strong-field ionization and high-order-harmonic generation during polyatomic molecular dynamics of N2O4

2012 ◽  
Vol 85 (3) ◽  
Author(s):  
Michael Spanner ◽  
Jochen Mikosch ◽  
Andrey E. Boguslavskiy ◽  
Margaret M. Murnane ◽  
Albert Stolow ◽  
...  
Keyword(s):  
Molecular Dynamics ◽  
Harmonic Generation ◽  
Strong Field ◽  
High Order ◽  
Field Ionization ◽  
High Order Harmonic Generation ◽  
Strong Field Ionization ◽  
High Order Harmonic
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