Role of multiphoton excitation and two-electron effects in high harmonic generation of H2: A TDDFT calculation

2011 ◽  
Vol 391 (1) ◽  
pp. 83-87 ◽  
Author(s):  
Xi Chu ◽  
Patrick J. Memoli
Keyword(s):  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Multiphoton Excitation ◽  
Electron Effects

scholarly journals Role of the Intramolecular Phase in High-Harmonic Generation

2002 ◽  
Vol 88 (18) ◽  
Author(s):  
M. Lein ◽  
N. Hay ◽  
R. Velotta ◽  
J. P. Marangos ◽  
P. L. Knight
Keyword(s):  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation

scholarly journals The Role of Electron Trajectories in XUV-Initiated High-Harmonic Generation

2019 ◽  
Vol 9 (3) ◽  
pp. 378 ◽  
Author(s):  
Michael Krüger ◽  
Doron Azoury ◽  
Barry Bruner ◽  
Nirit Dudovich
Keyword(s):  
Harmonic Generation ◽  
Extreme Ultraviolet ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Generation Process ◽  
Electron Trajectories ◽  
Tunneling Ionization ◽  
Spectral Frequency ◽  
And Control

High-harmonic generation spectroscopy is a powerful tool for ultrafast spectroscopy with intrinsic attosecond time resolution. Its major limitation—the fact that a strong infrared driving pulse is governing the entire generation process—is lifted by extreme ultraviolet (XUV)-initiated high-harmonic generation (HHG). Tunneling ionization is replaced by XUV photoionization, which decouples ionization from recollision. Here we probe the intensity dependence of XUV-initiated HHG and observe strong spectral frequency shifts of the high harmonics. We are able to tune the shift by controlling the instantaneous intensity of the infrared field. We directly access the reciprocal intensity parameter associated with the electron trajectories and identify short and long trajectories. Our findings are supported and analyzed by ab initio calculations and a semiclassical trajectory model. The ability to isolate and control long trajectories in XUV-initiated HHG increases the range of the intrinsic attosecond clock for spectroscopic applications.

Role of Many-Electron Dynamics in High Harmonic Generation

2006 ◽  
Vol 96 (22) ◽  
Author(s):  
Ariel Gordon ◽  
Franz X. Kärtner ◽  
Nina Rohringer ◽  
Robin Santra
Keyword(s):  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Electron Dynamics
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