Isolation of Pu-isotopes from environmental samples using ion chromatography for accelerator mass spectrometry and alpha spectrometry

2008 ◽  
Vol 606 (2) ◽  
pp. 239-245 ◽  
Author(s):  
E. Chamizo ◽  
M.C. Jiménez-Ramos ◽  
L. Wacker ◽  
I. Vioque ◽  
A. Calleja ◽  
...  
2015 ◽  
Vol 4 (2) ◽  
pp. 125-130
Author(s):  
Xiongxin Dai ◽  
Marcus Christl ◽  
Sheila Kramer-Tremblay ◽  
Hans-Arno Synal

Ultra-trace analysis of actinides, such as Pu isotopes and 237Np, in bioassay samples is often needed for radiation protection programs at nuclear facilities. Accelerator mass spectrometry (AMS), particularly the compact ETH Zurich system “Tandy”, has evolved over the years as one of the most sensitive, selective, and robust techniques for actinide analysis. Employment of the AMS technique can reduce the demands on sample preparation chemistry and increase sample analysis throughput, due to very low instrumental detection limit, high rejection of interferences, and low susceptibility to adverse sample matrices. Initial research and development tests were performed to explore and demonstrate the analytical capability of AMS for Pu and Np urine bioassay. In this study, urine samples spiked with femtogram levels of Np and Pu isotopes were prepared and measured using compact ETH AMS system and the results showed excellent analytical capability for measuring Np and Pu isotopes at femtogram/litre levels in urine.


1990 ◽  
Vol 138 (2) ◽  
pp. 261-270 ◽  
Author(s):  
M. Imamura ◽  
H. Nagai ◽  
M. Honda ◽  
K. Kobayashi ◽  
K. Yoshida ◽  
...  

1995 ◽  
Vol 34 (2) ◽  
pp. 183-186 ◽  
Author(s):  
Fatma Arslan ◽  
Martin Behrendt ◽  
Werner Ernst ◽  
Eberhard Finckh ◽  
Gunther Greb ◽  
...  

The Analyst ◽  
2018 ◽  
Vol 143 (13) ◽  
pp. 3059-3067 ◽  
Author(s):  
B. Z. Cvetković ◽  
G. Salazar ◽  
D. Kunz ◽  
S. Szidat ◽  
E. Wieland

The combination of ion chromatography (IC) with accelerator mass spectrometry (AMS) was developed to determine the speciation of 14C-(radiocarbon) bearing organic compounds in the femto to pico molar concentration range.


Radiocarbon ◽  
2007 ◽  
Vol 49 (3) ◽  
pp. 1395-1402 ◽  
Author(s):  
M Youn ◽  
Y M Song ◽  
J Kang ◽  
J C Kim ◽  
M K Cheoun

The accelerator mass spectrometry (AMS) facility at Seoul National University (SNU-AMS) was accepted in December 1998 and results reported first at the Vienna AMS conference in October 1999 and at the 17th Radiocarbon Conference in Israel, June 2000. At the Vienna conference, we reported our accelerator system and sample preparation systems (Kim et al. 2000). Recent developments of the AMS facility have been regularly reported at AMS conferences (Kim et al. 2001, 2004, 2007). Meanwhile, about 1000 unknown archaeological, geological, and environmental samples have been measured every year. In this report, the archaeological and geological data carried out in 2002 are presented in terms of years BP (before present, AD 1950), following the SNU-AMS date lists I and II published in Radiocarbon (Kim et al. 2006a,b).


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