Assessment of the Low-Temperature Nonoxidative Activation of Methane over H-Galloaluminosilicate (MFI) Zeolite: A C-13 Labelling Investigation

2002 ◽  
Vol 205 (1) ◽  
pp. 217-220 ◽  
Author(s):  
Claude M. Naccache ◽  
Paul Mériaudeau ◽  
Gilbert Sapaly ◽  
Le Van Tiep ◽  
Younès Ben Taârit
Langmuir ◽  
2003 ◽  
Vol 19 (19) ◽  
pp. 7977-7988 ◽  
Author(s):  
Anastasios I. Skoulidas ◽  
David S. Sholl ◽  
Rajamani Krishna

2017 ◽  
Vol 121 (46) ◽  
pp. 25818-25826 ◽  
Author(s):  
Hui Fu ◽  
Yajun Wang ◽  
Tianhao Zhang ◽  
Chaohe Yang ◽  
Honghong Shan

2015 ◽  
Vol 1112 ◽  
pp. 201-204 ◽  
Author(s):  
Grandprix T.M. Kadja ◽  
Rino R. Mukti ◽  
I. Nyoman Marsih ◽  
Ismunandar

Zeolites are among the main catalysts in the petroleoum and fine-chemical industry. The well-defined channel framework with the acid sites have empowered this kind of material to catalyze many chemical reactions, such as alkylation, isomerization, and hydrocarbon cracking. Controlling the energy consumption towards efficient process in the synthesis of zeolite has been a great interest. In this light, we succesfully show that synthesis of MFI zeolite can be tailored by using high or low temperature heating. Synthesis via high-temperature heating (HTH) at 150 °C, resulted in conventional coffin-type morphology whereas low-temperature heating (LTH) at 90 °C, resulted in a spherical-type morphology. This phenomenon indicates that energy consumption for synthesizing MFI zeolite can be decreased. Moreover, the tetrapropylammonion ion (TPA+) amount as structure-directing agents (SDA) can be lowered, hence reducing the synthesis cost. The obtained samples were charaterized by advanced techniques to compare interesting properties between samples synthesized by HTH and LTH. This concerns on the resulting morphology, textural properties, and Si/Al framework ratio.


Author(s):  
Alessia Airi ◽  
Matteo Signorile ◽  
Francesca Bonino ◽  
Pierluigi Quagliotto ◽  
Silvia Bordiga ◽  
...  

Langmuir ◽  
2009 ◽  
Vol 25 (19) ◽  
pp. 11598-11607 ◽  
Author(s):  
L. Narasimhan ◽  
Pascal Boulet ◽  
Bogdan Kuchta ◽  
Oliver Schaef ◽  
Renaud Denoyel ◽  
...  

2016 ◽  
Vol 235 ◽  
pp. 143-150 ◽  
Author(s):  
Lin Lang ◽  
Shuheng Zhao ◽  
Junfei Jiang ◽  
Wenshen Yang ◽  
Xiuli Yin

2020 ◽  
Vol 355 ◽  
pp. 512-517 ◽  
Author(s):  
Bo Wu ◽  
Bingbing Chen ◽  
Xiaobing Zhu ◽  
Limei Yu ◽  
Chuan Shi

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