scholarly journals Graphene Quantum Dots: Fundamental Understanding of the Formation Mechanism for Graphene Quantum Dots Fabricated by Pulsed Laser Fragmentation in Liquid: Experimental and Theoretical Insight (Small 38/2020)

Small ◽  
2020 ◽  
Vol 16 (38) ◽  
pp. 2070210
Author(s):  
Sukhyun Kang ◽  
Kyung Hwan Jung ◽  
Sungwook Mhin ◽  
Yong Son ◽  
Kangpyo Lee ◽  
...  
Carbon ◽  
2013 ◽  
Vol 64 ◽  
pp. 341-350 ◽  
Author(s):  
Khaled Habiba ◽  
Vladimir I. Makarov ◽  
Javier Avalos ◽  
Maxime J.F. Guinel ◽  
Brad R. Weiner ◽  
...  

2014 ◽  
Vol 4 (1) ◽  
Author(s):  
Dan Qu ◽  
Min Zheng ◽  
Ligong Zhang ◽  
Haifeng Zhao ◽  
Zhigang Xie ◽  
...  

2017 ◽  
Vol 19 (33) ◽  
pp. 22395-22400 ◽  
Author(s):  
S. R. M. Santiago ◽  
T. N. Lin ◽  
C. H. Chang ◽  
Y. A. Wong ◽  
C. A. J. Lin ◽  
...  

We report a facile, fast, and one-step approach to prepare N-doped graphene quantum dots (GQDs) using pulsed laser ablation with diethylenetriamine (DETA).


2020 ◽  
Vol 58 (11) ◽  
pp. 808-814
Author(s):  
Jung-Il Lee ◽  
Jeong Ho Ryu

Graphene oxide quantum dots (GOQDs) are nanometer-sized graphene oxide fragments that exhibit unique properties, making them interesting candidates for a range of new applications. Carbon black, one of the commercially available carbon precursors, is produced by the thermal decomposition or incomplete combustion of organic compounds. It is commonly used as a supporting material for catalysts because of its excellent electrical conductivity, high surface area, and stability. In this paper, we report the transformation of carbon black into GOQDs in 10 min using a one-step facile approach. This transformation was achieved by pulsed laser ablation (PLA) in ethanol using the earth-abundant and low-cost carbon black as precursor. Only ethanol and carbon black were used for the transformation. The carbon clusters ablated from the carbon black were completely transformed into GOQDs with a homogeneous size distribution and heights in the range of 0.3-1.7 nm. This confirmed that the transformed GOQDs consisted of only single- or few-layered graphene quantum dots. The UV-vis spectra showed absorption bands at 215, 260, and 320 nm, which were attributed to the π→π* transition of the C=C of the sp<sup>2</sup> C bond in the sp<sup>3</sup> C matrix. A distinct blue emission peak at 450 nm was evident at an excitation wavelength of 360 nm. The broader PL emission spectra are due to the oxygen-related functional groups emitting PL between 300 and 440 nm.


2020 ◽  
Vol 28 (15) ◽  
pp. 21659 ◽  
Author(s):  
Sukhyun Kang ◽  
Young Kyu Jeong ◽  
Kyung Hwan Jung ◽  
Yong Son ◽  
Won Rae Kim ◽  
...  

RSC Advances ◽  
2019 ◽  
Vol 9 (24) ◽  
pp. 13658-13663 ◽  
Author(s):  
Sukhyun Kang ◽  
Jeong Ho Ryu ◽  
Byoungsoo Lee ◽  
Kyung Hwan Jung ◽  
Kwang Bo Shim ◽  
...  

Graphene quantum dots (GQDs) and graphene oxide quantum dots (GOQDs) can be selectively produced by wavelength-modulated pulsed laser ablation in liquid (PLAL) method, which can used in different applications such as optoelectronic and biomedical applications, respectively.


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