Proton Relaxometry of Long-Lived Spin Order

ChemPhysChem ◽  
2019 ◽  
Vol 20 (5) ◽  
pp. 766-772 ◽  
Author(s):  
Alexey S. Kiryutin ◽  
Mikhail S. Panov ◽  
Alexandra V. Yurkovskaya ◽  
Konstantin L. Ivanov ◽  
Geoffrey Bodenhausen
ChemPhysChem ◽  
2021 ◽  
Vol 22 (12) ◽  
pp. 1148-1148
Author(s):  
Ewoud Vaneeckhaute ◽  
Sophie De Ridder ◽  
Jean‐Max Tyburn ◽  
James G. Kempf ◽  
Francis Taulelle ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
O. Yu. Gorobtsov ◽  
L. Ponet ◽  
S. K. K. Patel ◽  
N. Hua ◽  
A. G. Shabalin ◽  
...  

AbstractThe spin-phonon interaction in spin density wave (SDW) systems often determines the free energy landscape that drives the evolution of the system. When a passing energy flux, such as photoexcitation, drives a crystalline system far from equilibrium, the resulting lattice displacement generates transient vibrational states. Manipulating intermediate vibrational states in the vicinity of the critical point, where the SDW order parameter changes dramatically, would then allow dynamical control over functional properties. Here we combine double photoexcitation with an X-ray free-electron laser (XFEL) probe to control and detect the lifetime and magnitude of the intermediate vibrational state near the critical point of the SDW in chromium. We apply Landau theory to identify the mechanism of control as a repeated partial quench and sub picosecond recovery of the SDW. Our results showcase the capabilities to influence and monitor quantum states by combining multiple optical photoexcitations with an XFEL probe. They open new avenues for manipulating and researching the behaviour of photoexcited states in charge and spin order systems near the critical point.


1984 ◽  
Vol 49 (12) ◽  
pp. 1147-1151 ◽  
Author(s):  
S. Kawarazaki ◽  
N. Kunitomi ◽  
Y. Morii ◽  
H. Suzuki ◽  
R.M. Moon ◽  
...  

2021 ◽  
Vol 104 (17) ◽  
Author(s):  
I. Panneer Muthuselvam ◽  
K. Saranya ◽  
Deepa Kasinathan ◽  
R. N. Bhowmik ◽  
R. Sankar ◽  
...  
Keyword(s):  

2018 ◽  
Vol 4 (11) ◽  
pp. eaau3402 ◽  
Author(s):  
R. Takagi ◽  
J. S. White ◽  
S. Hayami ◽  
R. Arita ◽  
D. Honecker ◽  
...  

Multiple-q spin order, i.e., a spin texture characterized by a multiple number of coexisting magnetic modulation vectors q, has recently attracted attention as a source of nontrivial magnetic topology and associated emergent phenomena. One typical example is the triple-q skyrmion lattice state stabilized by Dzyaloshinskii-Moriya interactions in noncentrosymmetric magnets, while the emergence of various multiple-q states of different origins is expected according to the latest theories. Here, we investigated the magnetic structure of the itinerant polar hexagonal magnet Y3Co8Sn4, in which several distinctive mechanisms favoring multiple-q states are allowed to become active. Small-angle neutron-scattering experiments suggest the formation of incommensurate triple-q magnetic order with an in-plane vortex-like spin texture, which can be most consistently explained in terms of the novel four-spin interaction mechanism inherent to itinerant magnets. The present results suggest a new route to realizing exotic multiple-q orders and that itinerant hexagonal magnets, including the R3M8Sn4 family with wide chemical tunability, can be a unique material platform to explore their rich phase diagrams.


ChemInform ◽  
2016 ◽  
Vol 47 (43) ◽  
Author(s):  
Taito Murakami ◽  
Takafumi Yamamoto ◽  
Cedric Tassel ◽  
Hiroshi Takatsu ◽  
Clemens Ritter ◽  
...  
Keyword(s):  

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