Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural–Artificial Photosynthetic Hybrid

2016 ◽  
Vol 128 (32) ◽  
pp. 9375-9379 ◽  
Author(s):  
Wangyin Wang ◽  
Hong Wang ◽  
Qingjun Zhu ◽  
Wei Qin ◽  
Guangye Han ◽  
...  
Keyword(s):  
Photosystem Ii ◽  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Overall Water Splitting ◽  
Artificial Photosynthetic

Biomimetic electron transport via multiredox shuttles from photosystem II to a photoelectrochemical cell for solar water splitting

2017 ◽  
Vol 10 (3) ◽  
pp. 765-771 ◽  
Author(s):  
Zhen Li ◽  
Wangyin Wang ◽  
Chunmei Ding ◽  
Zhiliang Wang ◽  
Shichao Liao ◽  
...  
Keyword(s):  
Electron Transfer ◽  
Electron Transport ◽  
Photosystem Ii ◽  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Electron Transfer Pathway ◽  
Solar Water ◽  
Solar Water Splitting ◽  
Overall Water Splitting ◽  
Redox Shuttles

A CdS–PSII hybrid PEC cell for overall water splitting contains a biomimetic electron transfer pathway comprising two redox shuttles.

A silicon-based hybrid photocathode modified with an N5-chelated nickel catalyst in a noble-metal-free biomimetic photoelectrochemical cell for solar-driven unbiased overall water splitting

2021 ◽  
Author(s):  
Lunlun Gong ◽  
Peili Zhang ◽  
Guoquan Liu ◽  
Yu Shan ◽  
Mei Wang
Keyword(s):  
Water Splitting ◽  
Nickel Catalyst ◽  
Noble Metal ◽  
Photoelectrochemical Cell ◽  
Metal Free ◽  
Overall Water Splitting ◽  
Redox Catalysts ◽  
Silicon Based ◽  
Modification Of The Surface

Modification of the surface of semiconductor-based photoelectrodes with molecular redox catalysts gives a way to realize atom-efficient catalysis for photoelectrochemical (PEC) H2 and O2 evolution. However, the diversity of immobilized...

scholarly journals A molecular tandem cell for efficient solar water splitting

2020 ◽  
Vol 117 (24) ◽  
pp. 13256-13260 ◽  
Author(s):  
Degao Wang ◽  
Jun Hu ◽  
Benjamin D. Sherman ◽  
Matthew V. Sheridan ◽  
Liang Yan ◽  
...  
Keyword(s):  
Water Splitting ◽  
Water Oxidation ◽  
Photoelectrochemical Cell ◽  
Applied Bias ◽  
Tandem Cell ◽  
Solar Water Splitting ◽  
Dye Sensitized ◽  
Solar Conversion ◽  
Artificial Photosynthetic ◽  
Natural Photosynthesis

Artificial photosynthesis provides a way to store solar energy in chemical bonds. Achieving water splitting without an applied external potential bias provides the key to artificial photosynthetic devices. We describe here a tandem photoelectrochemical cell design that combines a dye-sensitized photoelectrosynthesis cell (DSPEC) and an organic solar cell (OSC) in a photoanode for water oxidation. When combined with a Pt electrode for H2evolution, the electrode becomes part of a combined electrochemical cell for water splitting, 2H2O → O2+ 2H2, by increasing the voltage of the photoanode sufficiently to drive bias-free reduction of H+to H2. The combined electrode gave a 1.5% solar conversion efficiency for water splitting with no external applied bias, providing a mimic for the tandem cell configuration of PSII in natural photosynthesis. The electrode provided sustained water splitting in the molecular photoelectrode with sustained photocurrent densities of 1.24 mA/cm2for 1 h under 1-sun illumination with no applied bias.

Photoassisted Overall Water Splitting in a Visible Light-Absorbing Dye-Sensitized Photoelectrochemical Cell

2009 ◽  
Vol 131 (3) ◽  
pp. 926-927 ◽  
Author(s):  
W. Justin Youngblood ◽  
Seung-Hyun Anna Lee ◽  
Yoji Kobayashi ◽  
Emil A. Hernandez-Pagan ◽  
Paul G. Hoertz ◽  
...  
Keyword(s):  
Visible Light ◽  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Dye Sensitized ◽  
Overall Water Splitting

A Molecular Relay-Modified CdS-Sensitized Photoelectrochemical Cell for Overall Water Splitting

2016 ◽  
Vol 3 (9) ◽  
pp. 1471-1477 ◽  
Author(s):  
Chao Shen ◽  
Chin Sheng Chua ◽  
Yee-Fun Lim ◽  
Jie Liu ◽  
Xingzhu Wang ◽  
...  
Keyword(s):  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Overall Water Splitting

scholarly journals Earth-Abundant Molecular Z-Scheme Photoelectrochemical Cell for Overall Water-Splitting

2019 ◽  
Vol 141 (24) ◽  
pp. 9593-9602 ◽  
Author(s):  
Christopher D. Windle ◽  
Hiromu Kumagai ◽  
Masanobu Higashi ◽  
Romain Brisse ◽  
Sebastian Bold ◽  
...  
Keyword(s):  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Overall Water Splitting ◽  
Earth Abundant

Self-Biasing Photoelectrochemical Cell for Spontaneous Overall Water Splitting under Visible-Light Illumination

ChemSusChem ◽  
2013 ◽  
Vol 6 (7) ◽  
pp. 1276-1281 ◽  
Author(s):  
Quanpeng Chen ◽  
Jinhua Li ◽  
Xuejin Li ◽  
Ke Huang ◽  
Baoxue Zhou ◽  
...  
Keyword(s):  
Visible Light ◽  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Light Illumination ◽  
Overall Water Splitting ◽  
Visible Light Illumination

Reversible electron storage in tandem photoelectrochemical cell for light driven unassisted overall water splitting

2020 ◽  
Vol 275 ◽  
pp. 119094 ◽  
Author(s):  
Yanhu Wang ◽  
Huihui Shi ◽  
Kang Cui ◽  
Lina Zhang ◽  
Shenguang Ge ◽  
...  
Keyword(s):  
Water Splitting ◽  
Photoelectrochemical Cell ◽  
Electron Storage ◽  
Overall Water Splitting
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