Double Atom Catalysts: Heteronuclear Transition Metal Dimer Anchored on Nitrogen‐Doped Graphene as Superior Electrocatalyst for Nitrogen Reduction Reaction

2020 ◽  
Vol 3 (12) ◽  
pp. 2000190
Author(s):  
Guokui Zheng ◽  
Lei Li ◽  
Shaoyun Hao ◽  
Xingwang Zhang ◽  
Ziqi Tian ◽  
...  
Keyword(s):  
Transition Metal ◽  
Reduction Reaction ◽  
Nitrogen Reduction ◽  
Nitrogen Doped ◽  
Nitrogen Doped Graphene ◽  
Doped Graphene

Computational screening of efficient graphene-supported transition metal single atom catalysts toward the oxygen reduction reaction

2020 ◽  
Vol 8 (37) ◽  
pp. 19319-19327 ◽  
Author(s):  
Lei Li ◽  
Rao Huang ◽  
Xinrui Cao ◽  
Yuhua Wen
Keyword(s):  
Transition Metal ◽  
Oxygen Reduction Reaction ◽  
Oxygen Reduction ◽  
Reduction Reaction ◽  
Single Atom ◽  
Nitrogen Doped ◽  
Single Atoms ◽  
Computational Screening ◽  
Nitrogen Doped Graphene ◽  
Doped Graphene

Transition metal single atoms anchored on nitrogen-doped graphene toward the oxygen reduction reaction have been screened.

scholarly journals Strain-Controlled Single Cr Embedded Nitrogen-Doped Graphene Achieve Efficient Nitrogen Reduction

2021 ◽  
Author(s):  
Chao Lin ◽  
Xiaopeng Liu ◽  
Jiale Qu ◽  
Xiang Feng ◽  
Zhi Wei Seh ◽  
...  
Keyword(s):  
Electronic State ◽  
Reduction Reaction ◽  
State Regulation ◽  
Single Atom ◽  
Nitrogen Reduction ◽  
Nitrogen Doped ◽  
Nitrogen Doped Graphene ◽  
Doped Graphene

Single atom catalysts (SACs) have received much attention in the nitrogen reduction reaction (NRR) field due to their high atomic utilization and controllable electronic state regulation. It is attractive to...

scholarly journals Nitrogen-Doped Graphene Iron-Based Particle Electrode Outperforms Activated Carbon in Three-Dimensional Electrochemical Water Treatment Systems

Water ◽  
2020 ◽  
Vol 12 (11) ◽  
pp. 3121
Author(s):  
Hosna Ghanbarlou ◽  
Nikoline Loklindt Pedersen ◽  
Morten Enggrob Simonsen ◽  
Jens Muff
Keyword(s):  
Activated Carbon ◽  
Three Dimensional ◽  
Cell Voltage ◽  
Reduction Reaction ◽  
Process Data ◽  
Nitrogen Doped ◽  
Pesticide Removal ◽  
Optimal Value ◽  
Nitrogen Doped Graphene ◽  
Doped Graphene

The synergy between electrochemical oxidation and adsorption on particle electrodes was investigated in three-dimensional (3D) systems for p-nitrosodimethylaniline (RNO) decolorization and pesticide removal. A comparison was made between granular activated carbon (GAC) and a novel synthesized nitrogen-doped graphene-based particle electrode (NCPE). Experiments on RNO decolorization show that the synergy parameter of the 3D-NCPE system was improved 3000 times compared to the studied 3D-GAC system. This was due to the specific nanostructure and composition of the NCPE material. Nitrogen-doped graphene triggered an oxygen reduction reaction, producing hydrogen peroxide that simultaneously catalyzed on iron sites of the NCPEs to hydroxyl radicals following the electro-Fenton (EF) process. Data showed that in the experimental setup used for the study, the applied cell voltage required for the optimal value of the synergy parameter could be lowered to 5V in the 3D-NCPEs process, which is significantly better than the 15–20 V needed for synergy to be found in the 3D-GAC process. Compared to previous studies with 3D-GAC, the removal of pesticides 2,6 dichlorobenzamide (BAM), 2-methyl-4-chlorophenoxyaceticacid (MCPA), and methylchlorophenoxypropionic acid (MCPP) was also enhanced in the 3D-NCPE system.

scholarly journals Oxygen Reduction Reaction Mechanism of Nitrogen-Doped Graphene Derived from Ionic Liquid

2017 ◽  
Vol 142 ◽  
pp. 1319-1326 ◽  
Author(s):  
Yiyi She ◽  
Jinfan Chen ◽  
Chengxu Zhang ◽  
Zhouguang Lu ◽  
Meng Ni ◽  
...  
Keyword(s):  
Ionic Liquid ◽  
Reaction Mechanism ◽  
Oxygen Reduction Reaction ◽  
Oxygen Reduction ◽  
Reduction Reaction ◽  
Nitrogen Doped ◽  
Nitrogen Doped Graphene ◽  
Doped Graphene
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