Highly Luminescent 2D-Type Slab Crystals Based on a Molecular Charge-Transfer Complex as Promising Organic Light-Emitting Transistor Materials

2017 ◽  
Vol 29 (36) ◽  
pp. 1701346 ◽  
Author(s):  
Sang Kyu Park ◽  
Jin Hong Kim ◽  
Tatsuhiko Ohto ◽  
Ryo Yamada ◽  
Andrew O. F. Jones ◽  
...  
Author(s):  
Haitao Zhou ◽  
Mengna Yin ◽  
Zhenhong Zhao ◽  
Yanqin Miao ◽  
Xin Jin ◽  
...  

In this work, two carbazole- and benzo[d]oxazole-based novel multifunctional materials with hybridized local and charge-transfer (HLCT) characteristic, namely OCI and OCT, which could act as deep-blue fluorophors and phosphorescent hosts,...


2021 ◽  
Author(s):  
Qi Sun ◽  
Jiajun Ren ◽  
Tong Jiang ◽  
Qian Peng ◽  
Qi Ou ◽  
...  

Superior organic light-emitting transistors (OLETs) materials require two conventionally exclusive properties: strong luminescence and high charge mobilities. We propose a three-state model through localized diabatization to quantitative analyze excited state structures for various herringbone (HB) H-aggregates and demonstrate that for some investigated systems, the low-lying intermolecular charge-transfer (CT) state couples with the bright Frenkel exciton (FE) and forms a dipole-allowed S<sub>1</sub> that lies below the dark state, proceeding strong luminescence. Specifically, such conversion in luminescence properties occurs when the electron- and hole-transfer integrals ( and ) are of the same sign and is notably larger than the excitonic coupling (<i>J</i>), i.e., . This theoretical finding can not only explain and rationalize recent experimental results on DPA and dNaAnt, both with OLET property, but also unravel an exciting scenario where strong luminescence and high charge mobilities are compatible, which will considerably broaden the aperture of novel OLET design.


2018 ◽  
Vol 6 (34) ◽  
pp. 9049-9054 ◽  
Author(s):  
Seongjin Jeong ◽  
Youngnam Lee ◽  
Joon Ki Kim ◽  
Du-Jeon Jang ◽  
Jong-In Hong

We report new TADF molecules (AmT and AmmT) for highly efficient non-doped OLEDs utilizing intra- and intermolecular charge transfer excitons.


Sign in / Sign up

Export Citation Format

Share Document