Trap-Assisted Non-Radiative Recombination in Organic-Inorganic Perovskite Solar Cells

2015 ◽  
Vol 27 (11) ◽  
pp. 1837-1841 ◽  
Author(s):  
Gert-Jan A. H. Wetzelaer ◽  
Max Scheepers ◽  
Araceli Miquel Sempere ◽  
Cristina Momblona ◽  
Jorge Ávila ◽  
...  
2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Jing Wang ◽  
Jie Zhang ◽  
Yingzhi Zhou ◽  
Hongbin Liu ◽  
Qifan Xue ◽  
...  

AbstractAll-inorganic perovskite solar cells (PVSCs) have drawn increasing attention because of their outstanding thermal stability. However, their performance is still inferior than the typical organic-inorganic counterparts, especially for the devices with p-i-n configuration. Herein, we successfully employ a Lewis base small molecule to passivate the inorganic perovskite film, and its derived PVSCs achieved a champion efficiency of 16.1% and a certificated efficiency of 15.6% with improved photostability, representing the most efficient inverted all-inorganic PVSCs to date. Our studies reveal that the nitrile (C-N) groups on the small molecule effectively reduce the trap density of the perovskite film and thus significantly suppresses the non-radiative recombination in the derived PVSC by passivating the Pb-exposed surface, resulting in an improved open-circuit voltage from 1.10 V to 1.16 V after passivation. This work provides an insight in the design of functional interlayers for improving efficiencies and stability of all-inorganic PVSCs.


Nanoscale ◽  
2019 ◽  
Vol 11 (45) ◽  
pp. 21824-21833 ◽  
Author(s):  
Jyoti V. Patil ◽  
Sawanta S. Mali ◽  
Chang Kook Hong

Controlling the grain size of the organic–inorganic perovskite thin films using thiourea additives now crossing 2 μm size with >20% power conversion efficiency.


2021 ◽  
Vol 6 (2) ◽  
pp. 778-788
Author(s):  
Sawanta S. Mali ◽  
Jyoti V. Patil ◽  
Julian A. Steele ◽  
Sachin R. Rondiya ◽  
Nelson Y. Dzade ◽  
...  

2021 ◽  
pp. 2101287
Author(s):  
Xiao Wu ◽  
Junjie Ma ◽  
Minchao Qin ◽  
Xinlu Guo ◽  
Yuhao Li ◽  
...  

Solar Energy ◽  
2021 ◽  
Vol 222 ◽  
pp. 212-218
Author(s):  
Honggang Xie ◽  
Jiannan Xu ◽  
Can Gao ◽  
Jiejing Zhang ◽  
Chunxiao Gao ◽  
...  

2021 ◽  
pp. 2106386
Author(s):  
Youchao Wei ◽  
Yao Zhao ◽  
Caiping Liu ◽  
Zhaoyu Wang ◽  
Feilong Jiang ◽  
...  

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