scholarly journals Aircraft soot indirect effect on large-scale cirrus clouds: Is the indirect forcing by aircraft soot positive or negative?

2014 ◽  
Vol 119 (19) ◽  
pp. 11,303-11,320 ◽  
Author(s):  
Cheng Zhou ◽  
Joyce E. Penner
Cirrus ◽  
2002 ◽  
Author(s):  
Andrew J. Heymsfield ◽  
Greg M. McFarquhar

Cirrus, a principal cloud type that forms at low temperatures in the upper troposphere, is composed almost always of ice crystals (Heymsfield and Miloshevich 1989) and on average cover about 20% of the earth's surface (Hartmann et al. 1992). The purpose of this chapter is to characterize the microphysical properties of cirrus clouds. The Glossary of Meteorology (Huschke 1970) defines cirrus clouds as detached clouds in the form of white, delicate filaments, or white or mostly white patches, which are composed of ice crystals. This cloud type forms primarily in the upper troposphere, above about 8km (25,000 feet), where temperatures are generally below -30° C. There are a number of types of cirrus clouds, with the most frequent ones occurring in layers or sheets with horizontal dimensions of hundreds or even thousands of kilometers. Because horizontal dimensions are much greater than vertical extent, this particular type of cirrus cloud is called cirrostratus. Cirrus can also form in a patchy or tufted shape, when the ice crystals are large enough to acquire an appreciable fall velocity (the rate at which ice crystals fall in the vertical) so that trails of considerable vertical extent may form. These trails curve irregularly or slant, sometimes with a commalike shape, as a result of changes in the horizontal wind velocity with height and variations in the fall velocity of the ice crystals. A wispy, layered cloud that forms at the top of a cumulonimbus cloud, termed an “anvil” because of its shape, is a cirrus that consists essentially of ice debris which spreads outward from the convective parts of the storm. Anvils do not include the white, dense portions of thunderstorms or the active convective column. Anvils can spread to form large, widespread cloud layers. Tropical cirrus clouds are thought to arise primarily from cumulonimbus clouds. Unlike the thin, wispy cirrus typifying mid-latitudes, the high altitudes and extensive lateral and vertical development that often characterize tropical cirrus impose substantial large-scale radiative effects in the atmosphere and at the earth's surface (Hartmann et al. 1992; Collins et al. 1996). The cirrus-like low-level ice clouds and ice fogs of the Arctic are not considered cirrus.


2003 ◽  
Vol 3 (5) ◽  
pp. 1791-1806 ◽  
Author(s):  
W. Haag ◽  
B. Kärcher ◽  
J. Ström ◽  
A. Minikin ◽  
U. Lohmann ◽  
...  

Abstract. Factors controlling the microphysical link between distributions of relative humidity above ice saturation in the upper troposphere and lowermost stratosphere and cirrus clouds are examined with the help of microphysical trajectory simulations. Our findings are related to results from aircraft measurements and global model studies. We suggest that the relative humidities at which ice crystals form in the atmosphere can be inferred from in situ measurements of water vapor and temperature close to, but outside of, cirrus clouds. The comparison with concomitant measurements performed inside cirrus clouds provides a clue to freezing mechanisms active in cirrus. The analysis of field data taken at northern and southern midlatitudes in fall 2000 reveals distinct differences in cirrus cloud freezing thresholds. Homogeneous freezing is found to be the most likely mechanism by which cirrus form at southern hemisphere midlatitudes. The results provide evidence for the existence of heterogeneous freezing in cirrus in parts of the polluted northern hemisphere, but do not suggest that cirrus clouds in this region form exclusively on heterogeneous ice nuclei, thereby emphasizing the crucial importance of homogeneous freezing. The key features of distributions of upper tropospheric relative humidity simulated by a global climate model are shown to be in general agreement with both, microphysical simulations and field observations, delineating a feasible method to include and validate ice supersaturation in other large-scale atmospheric models, in particular chemistry-transport and weather forecast models.


2009 ◽  
Vol 9 (1) ◽  
pp. 93-117 ◽  
Author(s):  
D. Brunner ◽  
P. Siegmund ◽  
P. T. May ◽  
L. Chappel ◽  
C. Schiller ◽  
...  

Abstract. An aircraft measurement campaign involving the Russian high-altitude aircraft M55 Geophysica and the German DLR Falcon was conducted in Darwin, Australia in November and December 2005 as part of the European integrated project SCOUT-O3. The overall objectives of the campaign were to study the transport of trace gases through the tropical tropopause layer (TTL), mechanisms of dehydration close to the tropopause, and the role of deep convection in these processes. In this paper a detailed roadmap of the campaign is presented, including rationales for each flight, and an analysis of the local and large-scale meteorological context in which they were embedded. The campaign took place during the pre-monsoon season which is characterized by a pronounced diurnal evolution of deep convection including a mesoscale system over the Tiwi Islands north of Darwin known as "Hector". This allowed studying in detail the role of deep convection in structuring the tropical tropopause region, in situ sampling convective overshoots above storm anvils, and probing the structure of anvils and cirrus clouds by Lidar and a suite of in situ instruments onboard the two aircraft. The large-scale flow during the first half of the campaign was such that local flights, away from convection, sampled air masses downstream of the "cold trap" region over Indonesia. Abundant cirrus clouds enabled the study of active dehydration, in particular during two TTL survey flights. The campaign period also encompassed a Rossby wave breaking event transporting stratospheric air to the tropical middle troposphere and an equatorial Kelvin wave modulating tropopause temperatures and hence the conditions for dehydration.


2017 ◽  
Vol 61 (2) ◽  
pp. 202-218 ◽  
Author(s):  
Hans-Peter Y Qvist

During the last 20–30 years Western societies have witnessed large scale migration from the Global South. This has given rise to important challenges in securing the social, civic and political integration of non-Western immigrants into Western societies. Previous research has suggested that participation in volunteering in civil society can serve as a ‘stepping stone’ towards integration for immigrants. Whilst the previous studies have shown marked gaps in the propensity to participate in volunteering between immigrants and natives, little work has been done to identify the mechanisms that explain these gaps. In this study, high-quality survey data, linked with data from administrative registers, are used, with the application of logistic regression based on the Karlson–Holm–Breen method to conduct mediation analysis. The mediation analysis shows that non-Western immigrants are significantly less likely to participate in secular volunteering compared to natives; however, over half of this gap is explained by an indirect effect via socio-economic status, self-rated health, generalized trust, informal social networks and the intergenerational transmission of volunteering. Moreover, the mediation analysis suggests that non-Western immigrants are more likely to participate in religious volunteering: this is completely explained by a strong indirect effect occurring via religiosity.


Cirrus ◽  
2002 ◽  
Author(s):  
Graeme Stephens

Understanding the climate of Earth and the way climate varies in time requires a quantitative understanding of the way water cycles back and forth between the atmosphere and at the Earth's surface. The exchanges of water between the surface and atmosphere establish the hydrological cycle, and it is the influence of this cycle on the energy budget of Earth that is central not only to understanding present climate but also to the prediction of climate change. Processes relating to the smallest of the reservoirs of water—namely, the atmospheric branch of the hydrological cycle—play an especially critical role in climate change. Water in vapor phase is the critical greenhouse gas (e.g., Chahine 1992) providing much studied feedbacks on climate forcing (Lindzen 1990; Rind et al. 1991; Stephens and Greenwald 1991; Inamdar and Ramanathan 1998; Hall and Manabe 1999). Water in the form of condensed, precipitation-sized particles is an important source of energy fueling circulation systems and is the fundamental supply of fresh water to life on Earth. Liquid water cloud droplets significantly modulate the radiative budget of the planet (e.g., Wielicki et al. 1995). Water that exists as ice particles suspended in the atmosphere is perhaps the smallest of the water reservoirs of the atmosphere, yet these ice crystals when distributed as part of large-scale cirrus clouds exert a disproportionate influence on the energy and water budgets of the planet. This chapter briefly speculates on the important ways cirrus clouds affect the Earth's climate. The topics discussed are central to what is referred to as the cloud-climate problem, which might be schematically represented in terms of the coupled processes represented in figure 20.1. The two most critical scientific questions associated with the cloud-climate problem are also stated in figure 20.1. Answers to these questions require a clearer understanding of how the large-scale circulation of the atmosphere governs cloud formation and evolution, how these clouds heat and moisten the atmosphere, and how this heating and moistening effect in turn feeds back to influence the dynamical and thermodynamical properties of the atmosphere.


2013 ◽  
Vol 70 (3) ◽  
pp. 901-915 ◽  
Author(s):  
Q. S. He ◽  
C. C. Li ◽  
J. Z. Ma ◽  
H. Q. Wang ◽  
G. M. Shi ◽  
...  

Abstract As part of the Tibet Ozone, Aerosol and Radiation (TOAR) project, a micropulse lidar was operated in Naqu (31.5°N, 92.1°E; 4508 m MSL) on the Tibetan Plateau to observe cirrus clouds continuously from 19 July to 26 August 2011. During the experiment, the time coverage of ice clouds only was 15% in the upper troposphere (above 9.5 km MSL). The cirrus top/bottom altitudes (mean values of 15.6/14.7 km) are comparable to those measured previously at tropical sites but relatively higher than those measured at midlatitude sites. The majority of the cloud layers yielded a lidar ratio between 10 and 40 sr, with a mean value of 28 ± 15 sr, characterized by a bimodal frequency distribution. Subvisible, thin, and opaque cirrus formation was observed in 16%, 34%, and 50% of all cirrus cases, respectively. A mean cirrus optical depth of 0.33 was observed over the Tibetan Plateau, slightly higher than those in the subtropics and tropics. With decreasing temperature, the lidar ratio increased slightly, whereas the mean extinction coefficient decreased significantly. The occurrence of clouds is highly correlated with the outgoing longwave radiation and the strong cold perturbations in the upper troposphere. Deep convective activity and Rossby waves are important dynamical processes that control cirrus variations over the Tibetan Plateau, where both anvil cirrus outflowing from convective cumulonimbus clouds and large-scale strong cold perturbations in the upper troposphere should play an important role in cirrus formation.


2013 ◽  
Vol 13 (8) ◽  
pp. 4235-4251 ◽  
Author(s):  
R. H. Moore ◽  
V. A. Karydis ◽  
S. L. Capps ◽  
T. L. Lathem ◽  
A. Nenes

Abstract. We use the Global Modelling Initiative (GMI) chemical transport model with a cloud droplet parameterisation adjoint to quantify the sensitivity of cloud droplet number concentration to uncertainties in predicting CCN concentrations. Published CCN closure uncertainties for six different sets of simplifying compositional and mixing state assumptions are used as proxies for modelled CCN uncertainty arising from application of those scenarios. It is found that cloud droplet number concentrations (Nd) are fairly insensitive to the number concentration (Na) of aerosol which act as CCN over the continents (∂lnNd/∂lnNa ~10–30%), but the sensitivities exceed 70% in pristine regions such as the Alaskan Arctic and remote oceans. This means that CCN concentration uncertainties of 4–71% translate into only 1–23% uncertainty in cloud droplet number, on average. Since most of the anthropogenic indirect forcing is concentrated over the continents, this work shows that the application of Köhler theory and attendant simplifying assumptions in models is not a major source of uncertainty in predicting cloud droplet number or anthropogenic aerosol indirect forcing for the liquid, stratiform clouds simulated in these models. However, it does highlight the sensitivity of some remote areas to pollution brought into the region via long-range transport (e.g., biomass burning) or from seasonal biogenic sources (e.g., phytoplankton as a source of dimethylsulfide in the southern oceans). Since these transient processes are not captured well by the climatological emissions inventories employed by current large-scale models, the uncertainties in aerosol-cloud interactions during these events could be much larger than those uncovered here. This finding motivates additional measurements in these pristine regions, for which few observations exist, to quantify the impact (and associated uncertainty) of transient aerosol processes on cloud properties.


1997 ◽  
Vol 36 (6) ◽  
pp. 664-675 ◽  
Author(s):  
V. Giraud ◽  
J. C. Buriez ◽  
Y. Fouquart ◽  
F. Parol ◽  
G. Seze

Abstract An algorithm that allows an automatic analysis of cirrus properties from Advanced Very High Resolution Radiometer (AVHRR) observations is presented. Further investigations of the information content and physical meaning of the brightness temperature differences (BTD) between channels 4 (11 μm) and 5 (12 μm) of the radiometer have led to the development of an automatic procedure to provide global estimates both of the cirrus cloud temperature and of the ratio of the equivalent absorption coefficients in the two channels, accounting for scattering effects. The ratio is useful since its variations are related to differences in microphysical properties. Assuming that cirrus clouds are composed of ice spheres, the effective diameter of the particle size distribution can be deduced from this microphysical index. The automatic procedure includes first, a cloud classification and a selection of the pixels corresponding to the envelope of the BTD diagram observed at a scale of typically 100 × 100 pixels. The classification, which uses dynamic cluster analysis, takes into account spectral and spatial properties of the AVHRR pixels. The selection is made through a series of tests, which also guarantees that the BTD diagram contains the necessary information, such as the presence of both cirrus-free pixels and pixels totally covered by opaque cirrus in the same area. Finally, the cloud temperature and the equivalent absorption coefficient ratio are found by fitting the envelope of the BTD diagram with a theoretical curve. Note that the method leads to the retrieval of the maximum value of the equivalent absorption coefficient ratio in the scene under consideration. This, in turn, corresponds to the minimum value of the effective diameter of the size distribution of equivalent Mie particles. The automatic analysis has been applied to a series of 21 AVHRR images acquired during the International Cirrus Experiment (ICE’89). Although the dataset is obviously much too limited to draw any conclusion at the global scale, it is large enough to permit derivation of cirrus properties that are statistically representative of the cirrus systems contained therein. The authors found that on average, the maximum equivalent absorption coefficient ratio increases with the cloud-top temperature with a jump between 235 and 240 K. More precisely, for cloud temperatures warmer than 235 K, the retrieved equivalent absorption coefficient ratio sometimes corresponds to very small equivalent spheres (diameter smaller than 20 μm). This is never observed for lower cloud temperatures. This change in cirrus microphysical properties points out that ice crystal habits may vary from one temperature regime toanother. It may be attributed to a modification of the size and/or shape of the particles.


2006 ◽  
Vol 6 (1) ◽  
pp. 1579-1617 ◽  
Author(s):  
J. E. Penner ◽  
J. Quaas ◽  
T. Storelvmo ◽  
T. Takemura ◽  
O. Boucher ◽  
...  

Abstract. Modeled differences in predicted effects are increasingly used to help quantify the uncertainty of these effects. Here, we examine modeled differences in the aerosol indirect effect in a series of experiments that help to quantify how and why model-predicted aerosol indirect forcing varies between models. The experiments start with an experiment in which aerosol concentrations, the parameterization of droplet concentrations and the autoconversion scheme are all specified and end with an experiment that examines the predicted aerosol indirect forcing when only aerosol sources are specified. Although there are large differences in the predicted liquid water path among the models, the predicted aerosol indirect effect for the first experiment is rather similar. Changes to the autoconversion scheme can lead to large changes in the liquid water path of the models and to the response of the liquid water path to changes in aerosols. Nevertheless, these changes do not necessarily lead to large changes in the radiative forcing. The parameterization of cloud fraction within models is not sensitive to the aerosol concentration, and, therefore, the response of the modeled cloud fraction within the present models appears to be smaller than that which would be associated with model ''noise''. The prediction of aerosol concentrations, given a fixed set of sources, leads to some of the largest differences in the predicted aerosol indirect radiative forcing among the models. Thus, this aspect of modeling requires significant improvement in order to improve the prediction of aerosol indirect effects.


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