scholarly journals Sensitivity of modeled far-IR radiation budgets in polar continents to treatments of snow surface and ice cloud radiative properties

2014 ◽  
Vol 41 (18) ◽  
pp. 6530-6537 ◽  
Author(s):  
Xiuhong Chen ◽  
Xianglei Huang ◽  
Mark G. Flanner
Keyword(s):  
Radiative Properties ◽  
Snow Surface ◽  
Ir Radiation ◽  
Ice Cloud ◽  
Cloud Radiative Properties

Calculations of the variability of ice cloud radiative properties at selected solar wavelengths

1980 ◽  
Vol 19 (18) ◽  
pp. 3057 ◽  
Author(s):  
R. M. Welch ◽  
S. K. Cox ◽  
W. G. Zdunkowski
Keyword(s):  
Radiative Properties ◽  
Ice Cloud ◽  
Cloud Radiative Properties

scholarly journals Resolving ice cloud optical thickness biases between CALIOP and MODIS using infrared retrievals

2016 ◽  
Vol 16 (8) ◽  
pp. 5075-5090 ◽  
Author(s):  
Robert E. Holz ◽  
Steven Platnick ◽  
Kerry Meyer ◽  
Mark Vaughan ◽  
Andrew Heidinger ◽  
...  
Keyword(s):  
Optical Thickness ◽  
Spatial Scales ◽  
Radiative Properties ◽  
Radiation Balance ◽  
Data Set ◽  
Mean Values ◽  
Ice Cloud ◽  
Lidar Ratio ◽  
Cloud Optical Thickness ◽  
The Impact

Abstract. Despite its importance as one of the key radiative properties that determines the impact of upper tropospheric clouds on the radiation balance, ice cloud optical thickness (IOT) has proven to be one of the more challenging properties to retrieve from space-based remote sensing measurements. In particular, optically thin upper tropospheric ice clouds (cirrus) have been especially challenging due to their tenuous nature, extensive spatial scales, and complex particle shapes and light-scattering characteristics. The lack of independent validation motivates the investigation presented in this paper, wherein systematic biases between MODIS Collection 5 (C5) and CALIOP Version 3 (V3) unconstrained retrievals of tenuous IOT (< 3) are examined using a month of collocated A-Train observations. An initial comparison revealed a factor of 2 bias between the MODIS and CALIOP IOT retrievals. This bias is investigated using an infrared (IR) radiative closure approach that compares both products with MODIS IR cirrus retrievals developed for this assessment. The analysis finds that both the MODIS C5 and the unconstrained CALIOP V3 retrievals are biased (high and low, respectively) relative to the IR IOT retrievals. Based on this finding, the MODIS and CALIOP algorithms are investigated with the goal of explaining and minimizing the biases relative to the IR. For MODIS we find that the assumed ice single-scattering properties used for the C5 retrievals are not consistent with the mean IR COT distribution. The C5 ice scattering database results in the asymmetry parameter (g) varying as a function of effective radius with mean values that are too large. The MODIS retrievals have been brought into agreement with the IR by adopting a new ice scattering model for Collection 6 (C6) consisting of a modified gamma distribution comprised of a single habit (severely roughened aggregated columns); the C6 ice cloud optical property models have a constant g ≈ 0.75 in the mid-visible spectrum, 5–15 % smaller than C5. For CALIOP, the assumed lidar ratio for unconstrained retrievals is fixed at 25 sr for the V3 data products. This value is found to be inconsistent with the constrained (predominantly nighttime) CALIOP retrievals. An experimental data set was produced using a modified lidar ratio of 32 sr for the unconstrained retrievals (an increase of 28 %), selected to provide consistency with the constrained V3 results. These modifications greatly improve the agreement with the IR and provide consistency between the MODIS and CALIOP products. Based on these results the recently released MODIS C6 optical products use the single-habit distribution given above, while the upcoming CALIOP V4 unconstrained algorithm will use higher lidar ratios for unconstrained retrievals.

scholarly journals A test of the ability of current bulk optical models to represent the radiative properties of cirrus cloud across the mid-and far-infrared

2020 ◽  
Author(s):  
Richard J. Bantges ◽  
Helen E. Brindley ◽  
Jonathan E. Murray ◽  
Alan E. Last ◽  
Cathryn Fox ◽  
...  
Keyword(s):  
Compensation Effect ◽  
Far Infrared ◽  
Single Scattering ◽  
Radiative Properties ◽  
Cirrus Cloud ◽  
Atmospheric Measurements ◽  
Infrared Observations ◽  
Ice Cloud ◽  
Infrared Frequency Range ◽  
The Uk

Abstract. Measurements of mid- to far-infrared nadir radiances obtained from the UK Facility for Airborne Atmospheric Measurements (FAAM) BAe-146 aircraft during the Cirrus Coupled Cloud-Radiation Experiment (CIRCCREX) are used to assess the performance of various ice cloud bulk optical (single-scattering) property models. Through use of a minimisation approach, we find that the simulations can reproduce the observed spectra in the mid-infrared to within measurement uncertainty but are unable to simultaneously match the observations over the far-infrared frequency range. When both mid and far-infrared observations are used to minimise residuals, first order estimates of the flux differences between the best performing simulations and observations indicate a strong compensation effect between the mid and far infrared such that the absolute broadband difference is

scholarly journals Aerosol absorption and radiative forcing

2007 ◽  
Vol 7 (3) ◽  
pp. 7171-7233 ◽  
Author(s):  
P. Stier ◽  
J. H. Seinfeld ◽  
S. Kinne ◽  
O. Boucher
Keyword(s):  
Optical Depth ◽  
Radiative Forcing ◽  
Radiative Properties ◽  
Refractive Indices ◽  
Anthropogenic Aerosol ◽  
Clear Sky ◽  
Aerosol Absorption ◽  
Long Wave ◽  
Aerosol Radiative ◽  
Cloud Radiative Properties

Abstract. We present a comprehensive examination of aerosol absorption with a focus on evaluating the sensitivity of the global distribution of aerosol absorption to key uncertainties in the process representation. For this purpose we extended the comprehensive aerosol-climate model ECHAM5-HAM by effective medium approximations for the calculation of aerosol effective refractive indices, updated black carbon refractive indices, new cloud radiative properties considering the effect of aerosol inclusions, as well as by modules for the calculation of long-wave aerosol radiative properties and instantaneous aerosol forcing. The evaluation of the simulated aerosol absorption optical depth with the AERONET sun-photometer network shows a good agreement in the large scale global patterns. On a regional basis it becomes evident that the update of the BC refractive indices to Bond and Bergstrom (2006) significantly improves the previous underestimation of the aerosol absorption optical depth. In the global annual-mean, absorption acts to reduce the short-wave anthropogenic aerosol top-of-atmosphere (TOA) radiative forcing clear-sky from –0.79 to –0.53 W m−2 (33%) and all-sky from –0.47 to –0.13 W m−2 (72%). Our results confirm that basic assumptions about the BC refractive index play a key role for aerosol absorption and radiative forcing. The effect of the usage of more accurate effective medium approximations is comparably small. We demonstrate that the diversity in the AeroCom land-surface albedo fields contributes to the uncertainty in the simulated anthropogenic aerosol radiative forcings: the usage of an upper versus lower bound of the AeroCom land albedos introduces a global annual-mean TOA forcing range of 0.19 W m−2 (36%) clear-sky and of 0.12 W m−2 (92%) all-sky. The consideration of black carbon inclusions on cloud radiative properties results in a small global annual-mean all-sky absorption of 0.05 W m−2 and a positive TOA forcing perturbation of 0.02 W m−2. The long-wave aerosol radiative effects are small for anthropogenic aerosols but become of relevance for the larger natural dust and sea-salt aerosols.

scholarly journals The efficacy of aerosol–cloud radiative perturbations from near-surface emissions in deep open-cell stratocumuli

2018 ◽  
Vol 18 (23) ◽  
pp. 17475-17488 ◽  
Author(s):  
Anna Possner ◽  
Hailong Wang ◽  
Robert Wood ◽  
Ken Caldeira ◽  
Thomas P. Ackerman
Keyword(s):  
Emission Line ◽  
Radiative Properties ◽  
Radiative Effect ◽  
Radiative Effects ◽  
Near Surface ◽  
Open Cell ◽  
Detection And Attribution ◽  
Cloud Radiative Effects ◽  
Ship Tracks ◽  
Cloud Radiative Properties

Abstract. Aerosol–cloud radiative effects are determined and quantified in simulations of deep open-cell stratocumuli observed during the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) campaign off the west coast of Chile. The cloud deck forms in a boundary layer 1.5 km deep, with cell sizes reaching 50 km in diameter. Global databases of ship tracks suggest that these linear structures are seldom found in boundary layers this deep. Here, we quantify the changes in cloud radiative properties to a continuous aerosol point source moving along a fixed emission line releasing 1017 particles per second. We show that a spatially coherent cloud perturbation is not evident along the emission line. Yet our model simulates an increase in domain-mean all-sky albedo of 0.05, corresponding to a diurnally averaged cloud radiative effect of 20 W m−2, given the annual mean solar insolation at the VOCALS-REx site. Therefore, marked changes in cloud radiative properties in precipitating deep open cells may be driven by anthropogenic near-surface aerosol perturbations, such as those generated by ships. Furthermore, we demonstrate that these changes in cloud radiative properties are masked by the naturally occurring variability within the organised cloud field. A clear detection and attribution of cloud radiative effects to a perturbation in aerosol concentrations becomes possible when sub-filtering of the cloud field is applied, using the spatio-temporal distribution of the aerosol perturbation. Therefore, this work has implications for the detection and attribution of effective cloud radiative forcing in marine stratocumuli, which constitutes one of the major physical uncertainties within the climate system. Our results suggest that ships may sometimes have a substantial radiative effect on marine clouds and albedo, even when ship tracks are not readily visible.

scholarly journals Deposition of brown carbon onto snow: changes in snow optical and radiative properties

2020 ◽  
Vol 20 (10) ◽  
pp. 6095-6114 ◽  
Author(s):  
Nicholas D. Beres ◽  
Deep Sengupta ◽  
Vera Samburova ◽  
Andrey Y. Khlystov ◽  
Hans Moosmüller
Keyword(s):  
Optical Properties ◽  
Organic Carbon ◽  
Total Organic Carbon ◽  
Radiative Forcing ◽  
Radiative Properties ◽  
Unit Mass ◽  
Small Scale ◽  
Snow Surface ◽  
Brown Carbon ◽  
Snow Albedo

Abstract. Light-absorbing organic carbon aerosol – colloquially known as brown carbon (BrC) – is emitted from combustion processes and has a brownish or yellowish visual appearance, caused by enhanced light absorption at shorter visible and ultraviolet wavelengths (0.3 µm≲λ≲0.5 µm). Recently, optical properties of atmospheric BrC aerosols have become the topic of intense research, but little is known about how BrC deposition onto snow surfaces affects the spectral snow albedo, which can alter the resulting radiative forcing and in-snow photochemistry. Wildland fires in close proximity to the cryosphere, such as peatland fires that emit large quantities of BrC, are becoming more common at high latitudes, potentially affecting nearby snow and ice surfaces. In this study, we describe the artificial deposition of BrC aerosol with known optical, chemical, and physical properties onto the snow surface, and we monitor its spectral radiative impact and compare it directly to modeled values. First, using small-scale combustion of Alaskan peat, BrC aerosols were artificially deposited onto the snow surface. UV–Vis absorbance and total organic carbon (TOC) concentration of snow samples were measured for samples with and without artificial BrC deposition. These measurements were used to first derive a BrC (mass) specific absorption (m2 g−1) across the UV–Vis spectral range. We then estimate the imaginary part of the refractive index of deposited BrC aerosol using a volume mixing rule. Single-particle optical properties were calculated using Mie theory, and these values were used to show that the measured spectral snow albedo of snow with deposited BrC was in general agreement with modeled spectral snow albedo using calculated BrC optical properties. The instantaneous radiative forcing per unit mass of total organic carbon deposited to the ambient snowpack was found to be 1.23 (+0.14/-0.11) W m−2 per part per million (ppm). We estimate the same deposition onto a pure snowpack without light-absorbing impurities would have resulted in an instantaneous radiative forcing per unit mass of 2.68 (+0.27/-0.22) W m−2 per ppm of BrC deposited.

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